Noninvasive characterization methods for ultra-short laser pulse induced volume modifications.

We present two noninvasive characterization methods to investigate laser induced modifications in bulk fused silica glasses. The methods discussed are immersion microscopy and scanning acoustic microscopy (SAM). SAM shows merits in measuring the distance from sample surface to the first detectable density change of the modification, while immersion microscopy offers a look into the modification. Both noninvasive methods are preferred over conventional polishing or etching techniques due to the facts, that multiple investigations can be done with only one sample and lower time expenditure. The type II modifications were introduced by focusing laser pulses with high repetition rates into the fused silica.

Rapidly tunable femtosecond near-UV pulses from a non-collinear optical parametric oscillator.

Broadband tunable femtosecond laser pulses are of great interest in numerous fields, such as spectroscopy or imaging. Here, we report on the generation of rapidly tunable radiation in the near UV by using intracavity non-collinear sum-frequency mixing between the visible pulses of a non-collinear optical parametric oscillator (NOPO) and a near-infrared beam. The NOPO is pumped by the third harmonic of an Yb-based master oscillator fiber amplifier (MOFA). For sum-frequency mixing, remaining fundamental pulses at 1030 nm are used. With this approach, near-UV pulses in a range of 333-413 nm with average output powers up to 90 mW and pulse durations from 158-240 fs are achieved. Fast tunability is demonstrated over the whole tuning range by varying just the cavity length. The system also allows for the generation of two simultaneous synchronized output pulse trains in the visible and the near-UV spectral range.

Third and fifth order nonlinear susceptibilities in thin HfO2 layers.

Third harmonic generation (THG) from dielectric layers is investigated. By forming a thin gradient of HfO2 with continuously increasing thickness, we are able to study this process in detail. This technique allows us to elucidate the influence of the substrate and to quantify the layered materials third χ(3)(3ω: ω, ω, ω) and even fifth order χ(5)(3ω: ω, ω, ω, ω, - ω) nonlinear susceptibility at the fundamental wavelength of 1030 nm. This is to the best of our knowledge the first measurement of the fifth order nonlinear susceptibility in thin dielectric layers.

Photonic molecule state transition by collision.

We investigate the impact of collisions with two-frequency photonic molecules aiming to observe internal dynamic behavior and challenge their strong robustness. Versatile interaction scenarios show intriguing state changes expressed through modifications of the resulting state such as temporal compression and unknown collision-induced spectral tunneling. These processes show potential for efficient coherent supercontinuum generation and all-optical manipulation.

4D spatio-temporal electric field characterization of ultrashort light pulses undergoing filamentation.

We present an experimental method capable of capturing the complete spatio-temporal dynamics of filamenting ultrashort laser pulses. By employing spatially resolved Fourier transform spectrometry in combination with the capability to terminate the filament at any length, we can follow the nonlinear dynamics in four dimensions, i.e. the transverse domain, time and filament length. Our method thus not only enables the full characterization of the filamentation process throughout its evolution, but also allows to identify and select laser pulses with desired parameters.

Potential hazards and mitigation of X-ray radiation generated by laser-induced plasma from research-grade laser systems.

A large range of laser-matter applications employ ultrashort pulses and high laser intensity. Such processes can lead to unrequired X-ray generation, which represents a hazardous radiation factor even for common laboratory research-grade laser systems. We present here an analysis of the radiation dose rate and X-ray spectrum emitted during ablation of a rotating copper cylinder with respect to several laser parameters. The results show that focused sub-picosecond pulses with intensity above 1013 W/cm2 can exceed the annual irradiation limit even in one hour, requiring appropriate shielding for the safety of the researchers.

Generation of 15 nJ pulse energy by a sub-150 fs thulium-doped fiber Mamyshev oscillator.

Mamyshev oscillators have pushed the frontiers in output parameters of ytterbium- and erbium-based ultrafast fiber oscillators in the spectral region around 1 µm and 1.5 µm within the last few years tremendously. In order to expand the superior performance toward the 2 µm spectral region, we present in this Letter an experimental investigation of the generation of high-energy pulses by a thulium-doped fiber Mamyshev oscillator. Generating highly energetic pulses is enabled by a tailored redshifted gain spectrum in a highly doped double-clad fiber. The oscillator emits pulses with an energy of up to 15 nJ, which can be compressed to 140 fs.

Fast-tunable femtosecond visible radiation via sum-frequency generation from a high power NIR NOPO.

We report on a high power ultra-broadband, quickly tunable non-collinear parametric oscillator with highly efficient intra-cavity sum-frequency generation. It simultaneously delivers femtosecond pulses in two synchronized output beams: up to 4.9 W tunable from 650 to 1050 nm in the near infrared and up to 1.9 W from 380 to 500 nm in the visible spectral range. The (to our knowledge) novel source is ideally suited for spectroscopy or multi-color imaging. First results of two-color functional microscopy are presented.

Single-cycle pulse compression in dense resonant media.

We propose here a new approach for compression and frequency up-conversion of short optical pulses in the regime of extreme nonlinear optics in optically dense absorbing media, providing an alternative route to attosecond-scale pulses at high frequencies. This method is based on dynamics of self-induced transparency (SIT) pulses of nearly single cycle duration, leading to single-cycle-scale Rabi oscillations in the medium. The sub-cycle components of an incident pulse behave as separate SIT-pulses, approaching each other and self-compressing, resulting in the threefold compression in time and frequency up-conversion by the same factor. As we show, the scheme can be cascaded, staying at the subsequent stage with nearly the same compression and up-conversion ratio. In this way, as our simulations show, after only few micrometers of propagation, a 700 nm wavelength single cycle pulse can be compressed to a pulse of 200 attoseconds duration located in XUV frequency range.

Real-time stimulated Raman spectroscopy with a non-collinear optical parametric oscillator.

Ultrafast detection of microplastic particles is becoming a vital problem, as these particles are found in water sources worldwide. Ideally, a live analysis in flow is desirable to directly monitor the water quality for contaminations. Therefore, coherent Raman spectroscopy techniques require fast and broadband tunable lasers to address all relevant spectral regions of the investigated samples. In our work, we combine a high power non-collinear optical parametric oscillator with a real-time stimulated Raman scattering spectroscopy setup. The light source is continously tunable from 700 nm to 1030 nm in less than 10 ms, delivering an average output power of more than 500 mW with sub-ps pulses. We show the immediate observation of mixing processes and the detection of microplastic particles in water solution with a spectral window of more than 2000 cm-1.

Role of frequency dependence of the nonlinearity on a soliton's evolution in photonic crystal fibers.

We reveal the crucial role played by the frequency dependence of the nonlinear parameter on the evolution of femtosecond solitons inside photonic crystal fibers (PCFs). We show that the conventional approach based on the self-steepening effect is not appropriate when such fibers have two zero-dispersion wavelengths, and several higher-order nonlinear terms must be included for realistic modeling of the nonlinear phenomena in PCFs. These terms affect not only the Raman-induced wavelength shift of a soliton but also impact its shedding of dispersive radiation.

Dynamic focus shaping with mixed-aperture coherent beam combining.

A novel concept for dynamic focus shaping based on highly efficient coherent beam combining with micro-lens arrays (MLAs) as the combining element is presented. This concept allows us to control the power weights of diffraction orders by varying the absolute phases of an array of input beams. A proof-of-principle experiment is supported by simulations. For this, an input beam matrix of 5×5 beams is combined proving both the ability for further power scaling and dynamic focus shaping.

Mode-locked pulses from a Thulium-doped fiber Mamyshev oscillator.

We present experimental results of the generation of ultrashort pulses in the 2 µm wavelength region by a fiber Mamyshev oscillator, along with the simulation of the pulse propagation in the cavity. The Mamyshev oscillator emitted pulses with energies of 3.55 nJ at a repetition rate of 15 MHz and optical spectra with bandwidths of 48 nm. The pulses propagated in anomalous dispersive Thulium-doped fiber sections with dispersion compensation sections of normal dispersive fibers.

Selective ultrafast control of multi-level quantum systems by subcycle and unipolar pulses.

The most typical way to optically control population of atomic and molecular systems is to illuminate them with radiation, resonant to the relevant transitions. Here we consider a possibility to control populations with the subcycle and even unipolar pulses, containing less than one oscillation of electric field. Despite the spectrum of such pulses covers several levels at once, we show that it is possible to selectively excite the levels of our choice by varying the driving pulse shape, duration or time delay between consecutive pulses. The pulses which are not unipolar, but have a peak of electric field of one polarity much higher (and shorter) than of the opposite one, are also capable for such control.

High-repetition rate, mid-infrared, picosecond pulse generation with µJ-energies based on OPG/OPA schemes in 2-µm-pumped ZnGeP2.

We report on two different concepts to generate µJ-level mid-infrared laser pulses with sub-10 ps pulse duration via nonlinear parametric generation at high pulse repetition rates. Both schemes rely on the recent development of compact and efficient CPA-free, Ho:YLF-based 2-µm laser sources pumping the highly nonlinear crystal ZnGeP2 used for parametric amplification. The first concept comprises a simplified OPG/OPA scheme efficiently producing signal and idler radiation at fixed wavelengths of 3.0 and 6.5 µm, respectively. In the second concept, we demonstrate a wide spectral tunability of the picosecond, µJ pulses over the entire tuning range between 2.5 and 12 µm maintaining a constant bandwidth of sub-20 cm-1 by integrating a two-color pumping scheme and a spectral shaper into the setup. The presented compact and efficient mid-IR picosecond radiation sources offer a way towards low-cost mid-IR material processing and spectroscopic applications.

Higher-order dispersion and the spectral behavior in a doubly resonant optical parametric oscillator.

In doubly resonant optical parametric oscillators (DROPOs), it is possible to generate, enhance, and phase lock two frequencies at once. Following intracavity phase conditions, a complex tuning behavior of the signal and idler spectra takes place in DROPOs, cumulating into degeneracy with phase self-locking and coherent wavelength doubling. In this work, we identify group delay matching as the important parameter determining the global tuning behavior and demonstrate the key role of higher-order dispersion in the spectral dependencies. Applicationwise, we suggest a simple way to control the phase self-locking region by varying the intracavity third-order dispersion.

Coherent beam combining with micro-lens arrays.

A novel, to the best of our knowledge, concept for coherent beam combining is presented based on a simple setup with micro-lens arrays. These standard components are used in a proof-of-principle experiment for both coherent beam splitting and a combination of 5×5 beams. Here a combination efficiency above 90% is achieved. We call this novel concept "mixed aperture."

Manipulation of infrared dispersive waves in customized microstructured optical fibers for 1.7 and 2.0 µm light sources.

We demonstrate the controllable generation of infrared dispersive waves (DWs) from customized, in-house fabricated silica microstructured optical fibers (MOFs) by manipulating the location of zero dispersion wavelength (ZDW) through the structure of the fibers. The highly enriched shaping mechanism of arrested soliton in the MOFs with two ZDWs provides a technique for efficient energy transfer into the targeted eye-safe wavelengths at 1.7 and 2.0 µm by the virtue of DW formation.

Generating Ultrabroadband Deep-UV Radiation and Sub-10 nm Gap by Hybrid-Morphology Gold Antennas.

We experimentally investigate the interaction between hybrid-morphology gold optical antennas and a few-cycle Ti:sapphire laser up to ablative intensities, demonstrating rich nonlinear plasmonic effects and promising applications in coherent frequency upconversion and nanofabrication technology. The two-dimensional array of hybrid antennas consists of elliptical apertures combined with bowties in its minor axis. The plasmonic resonance frequency of the bowties is red-shifted with respect to the laser central frequency and thus mainly enhances the third harmonic spectrum at long wavelengths. The gold film between two neighboring elliptical apertures forms an hourglass-shaped structure, which acts as a "plasmonic lens" and thus strongly reinforces surface currents into a small area. This enhanced surface current produces a rotating magnetic field that deeply penetrates into the substrate. At resonant frequency, the magnetic field is further intensified by the bowties. The resonant frequency of the hourglass is blueshifted with respect to the laser central frequency. Consequently, it spectacularly extends the third harmonic spectrum toward short wavelengths. The resultant third harmonic signal ranges from 230 to 300 nm, much broader than the emission from a sapphire crystal. In addition, the concentration of surface current within the neck of the hourglass antenna results in a structural modification through laser ablation, producing sub-10 nm sharp metallic gaps. Moreover, after laser illumination the optical field hotspots are imprinted around the antennas, allowing us to confirm the subwavelength enhancement of the electric near-field intensity.

Rapid phase retrieval of ultrashort pulses from dispersion scan traces using deep neural networks.

The knowledge of the temporal shape of femtosecond pulses is of major interest for all their applications. The reconstruction of the temporal shape of these pulses is an inverse problem for characterization techniques, which benefit from an inherent redundancy in the measurement. Conventionally, time-consuming optimization algorithms are used to solve the inverse problems. Here, we demonstrate the reconstruction of ultrashort pulses from dispersion scan traces employing a deep neural network. The network is trained with a multitude of artificial and noisy dispersion scan traces from randomly shaped pulses. The retrieval takes only 16 ms enabling video-rate reconstructions. This approach reveals a great tolerance against noisy conditions, delivering reliable retrievals from traces with signal-to-noise ratios down to 5.