RESUMEN
We address the problem of thermalization in the presence of a time-dependent disorder in the framework of the nonlinear Schrödinger (or Gross-Pitaevskii) equation with a random potential. The thermalization to the Rayleigh-Jeans distribution is driven by the nonlinearity. On the other hand, the structural disorder is responsible for a relaxation toward the homogeneous equilibrium distribution (particle equipartition), which thus inhibits thermalization (energy equipartition). On the basis of the wave turbulence theory, we derive a kinetic equation that accounts for the presence of strong disorder. The theory unveils the interplay of disorder and nonlinearity. It unexpectedly reveals that a nonequilibrium process of condensation and thermalization can take place in the regime where disorder effects dominate over nonlinear effects. We validate the theory by numerical simulations of the nonlinear Schrödinger equation and the derived kinetic equation, which are found in quantitative agreement without using any adjustable parameter. Experiments realized in multimode optical fibers with an applied external stress evidence the process of thermalization in the presence of strong disorder.
RESUMEN
Light can be used to modify and control properties of media, as in the case of electromagnetically induced transparency or, more recently, for the generation of slow light or bright coherent XUV and X-ray radiation. Particularly unusual states of matter can be created by light fields with strengths comparable to the Coulomb field that binds valence electrons in atoms, leading to nearly-free electrons oscillating in the laser field and yet still loosely bound to the core [1,2]. These are known as Kramers-Henneberger states [3], a specific example of laser-dressed states [2]. Here, we demonstrate that these states arise not only in isolated atoms [4,5], but also in rare gases, at and above atmospheric pressure, where they can act as a gain medium during laser filamentation. Using shaped laser pulses, gain in these states is achieved within just a few cycles of the guided field. The corresponding lasing emission is a signature of population inversion in these states and of their stability against ionization. Our work demonstrates that these unusual states of neutral atoms can be exploited to create a general ultrafast gain mechanism during laser filamentation.
RESUMEN
We evaluate the linearity of three electric measurement techniques of the initial electron density in laser filaments by comparing their results for a pair of filaments and for the sum of each individual filament. The conductivity measured between two plane electrodes in a longitudinal configuration is linear within 2 % provided the electric field is kept below 100 kV/m. Furthermore, simulations show that the signal behaves like the amount of generated free electrons. The slow ionic current measured with plane electrodes in a parallel configuration is representative of the ionic charge available in the filament, after several µs, when the free electrons have recombined. It is linear within 2 % with the amount of ions and is insensitive to misalignment. Finally, the fast polarization signal in the same configuration deviates from linearity by up to 80 % and can only be considered as a semi-qualitative indication of the presence of charges, e.g., to characterize the filament length.
RESUMEN
The influence of aerosols on climate is highly dependent on the particle size distribution, concentration, and composition. In particular, the latter influences their ability to act as cloud condensation nuclei, whereby they impact cloud coverage and precipitation. Here, we simultaneously measured the concentration of aerosols from sea spray over the North Atlantic on board the exhaust-free solar-powered vessel "PlanetSolar", and the sea surface physico-chemical parameters. We identified organic-bearing particles based on individual particle fluorescence spectra. Organic-bearing aerosols display specific spatio-temporal distributions as compared to total aerosols. We propose an empirical parameterization of the organic-bearing particle concentration, with a dependence on water salinity and sea-surface temperature only. We also show that a very rich mixture of organic aerosols is emitted from the sea surface. Such data will certainly contribute to providing further insight into the influence of aerosols on cloud formation, and be used as input for the improved modeling of aerosols and their role in global climate processes.
RESUMEN
We measured the chemical composition and the size distribution of aerosols generated by femtosecond-Terawatt laser pulses in the atmosphere using an aerosol mass spectrometer (AMS). We show that nitric acid condenses in the form of ammonium nitrate, and that oxidized volatile organics also contribute to particle growth. These two components account for two thirds and one third, respectively, of the dry laser-condensed mass. They appear in two different modes centred at 380 nm and 150 nm. The number concentration of particles between 25 and 300 nm increases by a factor of 15. Pre-existing water droplets strongly increase the oxidative properties of the laser-activated atmosphere, substantially enhancing the condensation of organics under laser illumination.