Quantized Fields for Optimal Control in the Strong Coupling Regime.

We tailor the quantum statistics of a bosonic field to deterministically drive a quantum system into a target state. Experimentally accessible states of the field achieve good control of multilevel or multiqubit systems, notably also at coupling strengths beyond the rotating-wave approximation. This extends optimal control theory to the realm of fully quantized, strongly coupled control and target degrees of freedom.

Many-Body Interference at the Onset of Chaos.

We unveil the signature of many-body interference across dynamical regimes of the Bose-Hubbard model. Increasing the particles' indistinguishability enhances the temporal fluctuations of few-body observables, with a dramatic amplification at the onset of quantum chaos. By resolving the exchange symmetries of partially distinguishable particles, we explain this amplification as the fingerprint of the initial state's coherences in the eigenbasis.

Pulse area dependence of multiple quantum coherence signals in dilute thermal gases.

In the general framework of open quantum systems, we assess the impact of the pulse area on single and double quantum coherence (1QC and 2QC) signals extracted from fluorescence emitted by dilute thermal gases. We show that 1QC and 2QC signals are periodic functions of the pulse area, with distinctive features that reflect the particles' interactions via photon exchange, the polarizations of the laser pulses, and the observation direction.

Optimization of selective two-photon absorption in cavity polaritons.

We investigate optimal states of photon pairs to excite a target transition in a multilevel quantum system. With the help of coherent control theory for two-photon absorption with quantum light, we infer the maximal population achievable by optimal entangled vs separable states of light. Interference between excitation pathways as well as the presence of nearby states may hamper the selective excitation of a particular target state, but we show that quantum correlations can help to overcome this problem and enhance the achievable "selectivity" between two energy levels, i.e., the relative difference in population transferred into each of them. We find that the added value of optimal entangled states of light increases with broadening linewidths of the target states.

Chaos and Ergodicity across the Energy Spectrum of Interacting Bosons.

We identify the chaotic phase of the Bose-Hubbard Hamiltonian by the energy-resolved correlation between spectral features and structural changes of the associated eigenstates as exposed by their generalized fractal dimensions. The eigenvectors are shown to become ergodic in the thermodynamic limit, in the configuration space Fock basis, in which random matrix theory offers a remarkable description of their typical structure. The distributions of the generalized fractal dimensions, however, are ever more distinguishable from random matrix theory as the Hilbert space dimension grows.

Wave-Particle Duality in Complex Quantum Systems.

Stunning progress in the experimental resolution and control of natural or man-made complex systems at the level of their quantum mechanical constituents raises the question, across diverse subdisciplines of physics, chemistry, and biology, whether the fundamental quantum nature may condition the dynamical and functional system properties on mesoscopic if not macroscopic scales. However, which are the distinctive signatures of quantum properties in complex systems, notably when modulated by environmental stochasticity and dynamical instabilities? It appears that, to settle this question across the above communities, a shared understanding is needed of the central feature of quantum mechanics: wave-particle duality. In this Perspective, we elaborate how randomness induced by this very quantum property can be discerned from the stochasticity ubiquitous in complex systems already on the classical level. We argue that in the study of increasingly complex systems, such distinction requires the analysis of single incidents of quantum dynamical processes.

Robust Asymptotic Entanglement under Multipartite Collective Dephasing.

We derive an analytic solution for the ensemble-averaged collective dephasing dynamics of N noninteracting atoms in a fluctuating homogeneous external field. The obtained Kraus map is used to specify families of states whose entanglement properties are preserved at all times under arbitrary field orientations, even for states undergoing incoherent evolution. Our results apply to arbitrary spectral distributions of the field fluctuations.