GaAs-chip-based mid-infrared supercontinuum generation.

The mid-infrared spectral region opens up new possibilities for applications such as molecular spectroscopy with high spatial and frequency resolution. For example, the mid-infrared light provided by synchrotron sources has helped for early diagnosis of several pathologies. However, alternative light sources at the table-top scale would enable better access to these state-of-the-art characterizations, eventually speeding up research in biology and medicine. Mid-infrared supercontinuum generation in highly nonlinear waveguides pumped by compact fiber lasers represents an appealing alternative to synchrotrons. Here, we introduce orientation-patterned gallium arsenide waveguides as a new versatile platform for mid-infrared supercontinuum generation. Waveguides and fiber-based pump lasers are optimized in tandem to allow for the group velocities of the signal and the idler waves to match near the degeneracy point. This configuration exacerbates supercontinuum generation from 4 to 9 µm when waveguides are pumped at 2750 nm with few-nanojoule energy pulses. The brightness of the novel mid-infrared source exceeds that of the third-generation synchrotron source by a factor of 20. We also show that the nonlinear dynamics is strongly influenced by the choice of waveguide and laser parameters, thus offering an additional degree of freedom in tailoring the spectral profile of the generated light. Such an approach then opens new paths for high-brightness mid-infrared laser sources development for high-resolution spectroscopy and imaging. Furthermore, thanks to the excellent mechanical and thermal properties of the waveguide material, further power scaling seems feasible, allowing for the generation of watt-level ultra-broad frequency combs in the mid-infrared.

Optical parametric generation in OP-GaAs waveguides pumped by a femtosecond fluoride fiber laser.

We report on mid-infrared optical parametric generation in the 4-5 µm and 9-12 µm bands by pumping custom-designed orientation-patterned gallium arsenide (OP-GaAs) rib waveguides with an ultrafast femtosecond fiber laser system. This pump source is seeded by a mode-locked fluoride fiber laser with 59 MHz repetition rate and can be tuned between 2.8 and 3.2 µm using a soliton self-frequency shifting stage. The single TE and TM modes OP-GaAs crystals feature quasi-phase-matched grating periods of 85 and 90 µm and different transverse sizes thus allowing a wide spectral tunability.

Actively Q-switched tunable single-longitudinal-mode 2†µm Tm:YAP laser using a transversally chirped volume Bragg grating.

A pulsed, single longitudinal mode, wavelength-tunable Tm:YAP laser is reported. We demonstrate 1 kHz stable operation with 230 µJ, 50 ns pulses and a spectrum linewidth narrowed below 4 pm (FWHM) close to the Fourier transform limit by use of a volume Bragg grating and a YAG etalon. The output wavelength was tuned from 1940 to 1960 nm owing to a transverse chirp of the period of the Bragg grating.

Near-infrared to visible upconversion imaging using a broadband pump laser.

We present an upconversion imaging experiment from the near-infrared to the visible spectrum. Using a dedicated broadband pump laser to increase the number of resolved elements converted in the image we obtain up to 56x64 spatial elements with a 2.7 nm wide pump spectrum, more than 10 times the number of elements accessible with a narrowband laser. Results in terms of field of view, resolution and conversion efficiency are in good agreement with simulations. The computed sensitivity of our experiment favorably compares with direct InGaAs camera detection.

140 W peak power laser system tunable in the LWIR.

We present a high peak power rapidly tunable laser system in the long-wave infrared comprising an external-cavity quantum cascade laser (EC-QCL) broadly tunable from 8 to 10 µm and an optical parametric amplifier (OPA) based on quasi phase-matching in orientation-patterned gallium arsenide (OP-GaAs) of fixed grating period. The nonlinear crystal is pumped by a pulsed fiber laser system to achieve efficient amplification in the OPA. Quasi phase-matching remains satisfied when the EC-QCL wavelength is swept from 8 to 10 µm with a crystal of fixed grating period through tuning the pump laser source around 2 µm. The OPA demonstrates parametric amplification from 8 µm to 10 µm and achieves output peak powers up to 140 W with spectral linewidths below 3.5 cm-1. The beam profile quality (M2) remains below 3.4 in both horizontal and vertical directions. Compared to the EC-QCL, the linewidth broadening is attributed to a coupling with the OPA.

High sensitivity narrowband wavelength mid-infrared detection at room temperature.

We report an upconversion experiment using an orientation-patterned gallium arsenide (OP-GaAs) crystal to detect small mid-infrared signals on an InGaAs avalanche photodiode. A conversion efficiency up to 20% with a nonpolarized pulsed fiber pump is demonstrated. Our uncooled setup is favorably compared in terms of noise equivalent power, dynamic range, and response time to cryogenically cooled HgCdTe detectors. Its dependence on the polarization of both the pump and signal beams is also investigated.

Optical parametric generation by a simultaneously Q-switched mode-locked single-oscillator thulium-doped fiber laser in orientation-patterned gallium arsenide.

Optical parametric generation is demonstrated in orientation-patterned gallium arsenide, pumped by a novel single-oscillator simultaneously Q-switched and mode-locked thulium-doped fiber laser, downconverting the pump radiation into the mid-infrared wavelength regime. The maximum output energy reached is greater than 2.0 µJ per pump pulse.

Nonlinear diffraction in orientation-patterned semiconductors.

This work represents experimental demonstration of nonlinear diffraction in an orientation-patterned semiconducting material. By employing a new transverse geometry of interaction, three types of second-order nonlinear diffraction have been identified according to different configurations of quasi-phase matching conditions. Specifically, nonlinear Cerenkov diffraction is defined by the longitudinal quasi-phase matching condition, nonlinear Raman-Nath diffraction satisfies only the transverse quasi-phase matching condition, and nonlinear Bragg diffraction fulfils the full vectorial quasi-phase matching conditions. The study extends the concept of transverse nonlinear parametric interaction toward infrared frequency conversion in semiconductors. It also offers an effective nondestructive method to visualise and diagnose variations of second-order nonlinear coefficients inside semiconductors.

Multi-kW peak power acousto-optically tunable thulium-doped fiber laser system.

We demonstrate a core-pumped Q-switched thulium-doped fiber laser system with fast tunability capability over 100 nm without any movable part. With up to 7 kW peak power in a diffraction-limited beam, this source is well adapted for pumping a frequency agile mid-IR parametric oscillator or amplifier based on Quasi-Phase-Match single-period crystals.

Robust, frequency-stable and accurate mid-IR laser spectrometer based on frequency comb metrology of quantum cascade lasers up-converted in orientation-patterned GaAs.

We demonstrate a robust and simple method for measurement, stabilization and tuning of the frequency of cw mid-infrared (MIR) lasers, in particular of quantum cascade lasers. The proof of principle is performed with a quantum cascade laser at 5.4 µm, which is upconverted to 1.2 µm by sum-frequency generation in orientation-patterned GaAs with the output of a standard high-power cw 1.5 µm fiber laser. Both the 1.2 µm and the 1.5 µm waves are measured by a standard Er:fiber frequency comb. Frequency measurement at the 100 kHz-level, stabilization to sub-10 kHz level, controlled frequency tuning and long-term stability are demonstrated.

Optical parametric amplification of a distributed-feedback quantum-cascade laser in orientation-patterned GaAs.

We demonstrate what is to our knowledge the first realization of an optical parametric amplifier in orientation-patterned GaAs amplifying the emission of a quantum-cascade laser (QCL) with a distributed-feedback (DFB) structure. We report a gain as high as 53 dB at 4.5 mum, in good agreement with theoretical calculations. The narrow spectral linewidth and the good beam quality of this source are imposed by the DFB-QCL, while high-peak-power emission is achieved through the parametric amplification. These characteristics are of valuable interest for long-range spectroscopy.

Near-infrared active polarimetric and multispectral laboratory demonstrator for target detection.

We report on the design and exploitation of a real-field laboratory demonstrator combining active polarimetric and multispectral functions. Its building blocks, including a multiwavelength pulsed optical parametric oscillator at the emission side and a hyperspectral imager with polarimetric capability at the reception side, are described. The results obtained with this demonstrator are illustrated on some examples and discussed. In particular it is found that good detection performances rely on joint use of intensity and polarimetric images, with these images exhibiting complementary signatures in most cases.

Broadly tunable single-frequency cw mid-infrared source with milliwatt-level output based on difference-frequency generation in orientation-patterned GaAs.

A narrow-linewidth mid-IR source based on difference-frequency generation of an amplified 1.5 microm diode laser and a cw Tm-doped fiber laser in orientation-patterned (OP) GaAs has been developed and evaluated for spectroscopic applications. The source can be tuned to any frequency in the 7.6-8.2 microm range with an output power of 0.5 mW. The measured characteristics of the OP-GaAs sample demonstrate a high quality of the material.