Second-harmonic generation in a high-index doped silica micro-ring resonator.

We report the first, to the best of our knowledge, observation of second-harmonic generation (SHG) in a high-index doped silica micro-ring resonator, due to the symmetry-breaking-induced χ(2) at the core and cladding interface of the waveguide. The generated SH power is shown to have quadratic dependence on the in-cavity power of the fundamental pump at around 1550 nm. The pumping wavelength sweep method is adopted to fulfill the phase-matching condition for maximum conversion efficiency of SHG. This work offers a new approach to generate a visible source for the visible-light integrated optical platform from infrared-visible light conversion.

Third-harmonic generation in CMOS-compatible highly doped silica micro-ring resonator.

We present the first demonstration of visible emission from highly doped silica glass micro-ring resonators (MRRs) through a third-harmonic generation (THG) nonlinear process. We obtain green light conversion efficiency of 2.7×10-5 W-2 in a MRR with loaded Q-factor of 1.4×106 pumped in the telecom band. A thermal nonlinear model is developed to account for the in-cavity power dependence of the resonance detuning. Using the extracted thermal nonlinear coefficients, the measured TH resonance shift is calibrated by subtracting the thermal nonlinear-induced phase mismatch to obtain the theoretical threefold wavelength relationship along with the measured cubic power relationship.

Integrating temporal and spatial control of electronic transitions for bright multiphoton upconversion.

The applications of lanthanide-doped upconversion nanomaterials are limited by unsatisfactory brightness currently. Herein, a general strategy is proposed for boosting the upconversion efficiency in Er3+ ions, based on combined use of a core-shell nanostructured host and an integrated optical waveguide circuit excitation platform. A NaErF4@NaYF4 core-shell nanoparticle is constructed to host the upconversion process for minimizing non-radiative dissipation of excitation energy by surface quenchers. Furthermore, an integrated optical microring resonator is designed to promote absorption of excitation light by the nanoparticles, which alleviates quenching of excited states due to cross-relaxation and phonon-assisted energy transfer. As a result, multiphoton upconversion emission with a large anti-Stokes shift (greater than 1150 nm) and a high energy conversion efficiency (over 5.0%) is achieved under excitation at 1550 nm. These advances in controlling photon upconversion offer exciting opportunities for important photonics applications.