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1.
ACS Appl Mater Interfaces ; 16(40): 54435-54444, 2024 Oct 09.
Artículo en Inglés | MEDLINE | ID: mdl-39330975

RESUMEN

Advances in artificial general intelligence (AGI) necessitate the integration of diverse functionalities to address complex tasks. Carbon nanotubes (CNTs), with their unique physical properties, have broad applications in emerging research fields, providing a foundation for next-generation devices that could overcome the limits of Moore's Law. This work demonstrates a novel intelligent device that integrates five functions─sensors, memory, neuromorphic computing, logic, and communication─using CNT field-effect transistors (CNFETs) compatible with CMOS processes. Through passivation and annealing techniques, we have significantly enhanced the optoelectronic performance of CNFETs, leading to the development of multifunctional optoelectronic synaptic transistors. These optimized CNFETs enable dual-mode weight-tunable synaptic functions, including long-term plasticity and multilevel storage. Additionally, a CNT-based neural network has achieved high recognition accuracy on the MNIST data set, showcasing the potential of in-memory computing. This research also innovates by integrating logic functions with optoelectronic communication capabilities, paving the way for next-generation intelligent computing and communication integrated systems.

2.
Adv Mater ; : e2302658, 2023 Aug 31.
Artículo en Inglés | MEDLINE | ID: mdl-37652463

RESUMEN

In the era of the Internet of Things, vast amounts of data generated at sensory nodes impose critical challenges on the data-transfer bandwidth and energy efficiency of computing hardware. A near-sensor computing (NSC) architecture places the processing units closer to the sensors such that the generated data can be processed almost in situ with high efficiency. This study demonstrates the monolithic three-dimensional (M3D) integration of a photosensor array, analog computing-in-memory (CIM), and Si complementary metal-oxide-semiconductor (CMOS) logic circuits, named M3D-SAIL. This approach exploits the high-bandwidth on-chip data transfer and massively parallel CIM cores to realize an energy-efficient NSC architecture. The 1st layer of the Si CMOS circuits serves as the control logic and peripheral circuits. The 2nd layer comprises a 1 k-bit one-transistor-one-resistor (1T1R) array with InGaZnOx field-effect transistor (IGZO-FET) and resistive random-access memory (RRAM) for analog CIM. The 3rd layer comprises multiple IGZO-FET-based photosensor arrays for wavelength-dependent optical sensing. The structural integrity and function of each layer are comprehensively verified. Furthermore, NSC is implemented using the M3D-SAIL architecture for a typical video keyframe-extraction task, achieving a high classification accuracy of 96.7% as well as a 31.5× lower energy consumption and 1.91× faster computing speed compared to its 2D counterpart.

3.
iScience ; 16: 368-377, 2019 Jun 28.
Artículo en Inglés | MEDLINE | ID: mdl-31220760

RESUMEN

Oxide-based resistive switching devices, including ferroelectric tunnel junctions and resistance random access memory, are promising candidates for the next-generation non-volatile memory technology. In this work, we propose a ferroionic tunnel junction to realize a giant electroresistance. It functions as a ferroelectric tunnel junction at low resistance state and as a Schottky junction at high resistance state, due to interface engineering through the field-induced migration of oxygen vacancies. An extremely large electroresistance with ON/OFF ratios of 5.1×107 at room temperature and 2.1×109 at 10 K is achieved, using an ultrathin BaTiO3-δ layer as the ferroelectric barrier and a semiconducting Nb-doped SrTiO3 substrate as the bottom electrode. The results point toward an appealing way for the design of high-performance resistive switching devices based on ultrathin oxide heterostructures by ionic controlled interface engineering.

4.
Adv Mater ; : e1801548, 2018 Jul 04.
Artículo en Inglés | MEDLINE | ID: mdl-29974526

RESUMEN

Considering that the human brain uses ≈1015 synapses to operate, the development of effective artificial synapses is essential to build brain-inspired computing systems. In biological synapses, the voltage-gated ion channels are very important for regulating the action-potential firing. Here, an electrolyte-gated transistor using WO3 with a unique tunnel structure, which can emulate the ionic modulation process of biological synapses, is proposed. The transistor successfully realizes synaptic functions of both short-term and long-term plasticity. Short-term plasticity is mimicked with the help of electrolyte ion dynamics under low electrical bias, whereas the long-term plasticity is realized using proton insertion in WO3 under high electrical bias. This is a new working approach to control the transition from short-term memory to long-term memory using different gate voltage amplitude for artificial synapses. Other essential synaptic behaviors, such as paired pulse facilitation, the depression and potentiation of synaptic weight, as well as spike-timing-dependent plasticity are also implemented in this artificial synapse. These results provide a new recipe for designing synaptic electrolyte-gated transistors through the electrostatic and electrochemical effects.

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