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1.
Proc Natl Acad Sci U S A ; 120(51): e2314775120, 2023 Dec 19.
Artículo en Inglés | MEDLINE | ID: mdl-38085781

RESUMEN

Transition metal dichalcogenide (TMD) moiré superlattices provide an emerging platform to explore various light-induced phenomena. Recently, the discoveries of novel moiré excitons have attracted great interest. The nonlinear optical responses of these systems are however still underexplored. Here, we report investigation of light-induced shift currents (a second-order response generating DC current from optical illumination) in the WSe2/WS2 moiré superlattice. We identify a striking phenomenon of the formation of shift current vortex crystals-i.e., two-dimensional periodic arrays of moiré-scale current vortices and associated magnetic fields with remarkable intensity under laboratory laser setup. Furthermore, we demonstrate high optical tunability of these current vortices-their location, shape, chirality, and magnitude can be tuned by the frequency, polarization, and intensity of the incident light. Electron-hole interactions (excitonic effects) are found to play a crucial role in the generation and nature of the shift current intensity and distribution. Our findings provide a promising all-optical control route to manipulate nanoscale shift current density distributions and magnetic field patterns, as well as shed light on nonlinear optical responses in moiré quantum matter and their possible applications.

2.
Proc Natl Acad Sci U S A ; 120(31): e2307611120, 2023 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-37490531

RESUMEN

Manipulating quantum states through light-matter interactions has been actively pursued in two-dimensional materials research. Significant progress has been made toward the optical control of the valley degrees of freedom in semiconducting monolayer transition-metal dichalcogenides, based on doubly degenerate excitons from their two distinct valleys in reciprocal space. Here, we introduce a type of optically controllable doubly degenerate exciton states that come from a single valley, dubbed as single-valley exciton doublet (SVXD) states. They are unique in that their constituent holes originate from the same valence band, making possible the direct optical control of the spin structure of the excited constituent electrons. Combining ab initio GW plus Bethe-Salpeter equation (GW-BSE) calculations and a theoretical analysis method, we demonstrate such SVXD in substrate-supported monolayer bismuthene-which has been successfully grown using molecular beam epitaxy. In each of the two distinct valleys in the Brillouin zone, strong spin-orbit coupling and [Formula: see text] symmetry lead to a pair of degenerate 1s exciton states (the SVXD states) with opposite spin configurations. Any coherent linear combinations of the SVXD in a single valley can be excited by light with a specific polarization, enabling full manipulation of their internal spin configurations. In particular, a controllable net spin magnetization can be generated through light excitation. Our findings open routes to control quantum degrees of freedom, paving the way for applications in spintronics and quantum information science.

3.
Psychopharmacology (Berl) ; 237(4): 1043-1053, 2020 Apr.
Artículo en Inglés | MEDLINE | ID: mdl-31912191

RESUMEN

RATIONALE AND OBJECTIVE: Alcohol is a recreational substance that is generally socially acceptable and legal in most areas worldwide. An alcohol overdose will produce an inhibitory effect on the brain and impair cognition and memory. In this study, we examined the effect of alcohol on the acquisition, consolidation, and reconsolidation of drug reward memory induced by morphine and cocaine in rats. METHODS: Rats were trained to acquire morphine sulfate (10 mg/kg, s.c.) and cocaine (10 mg/kg, i.p.) conditioned place preference (CPP) via an unbiased CPP paradigm. Vehicle or alcohol (0.25, 0.75, 1.5 g/kg, i.p.) was administered at various time-points, including 30 min before each CPP conditioning session (acquisition), immediately after each CPP conditioning session (consolidation), immediately after the reactivation of CPP (reconsolidation with re-exposure), or without reactivation to the drug-paired context (reconsolidation without re-exposure). Conditioning scores were recorded before or after each conditioning session or memory reactivation. RESULTS: Alcohol at a dose of 1.5 g/kg but not 0.25 g/kg or 0.75 g/kg significantly inhibited the acquisition and reconsolidation of morphine- and cocaine-associated memory. In contrast, alcohol had no effect on the consolidation of morphine- or cocaine-induced CPP. CONCLUSIONS: The results suggested that pre-exposure alcohol dose-dependently attenuated morphine- or cocaine-induced place preference and prevented drug reinstatement in rats by disrupting memory reconsolidation, which may be explained by the inhibitory effect of alcohol on dopaminergic and glutamatergic neurotransmission.


Asunto(s)
Cocaína/farmacología , Condicionamiento Clásico/efectos de los fármacos , Etanol/farmacología , Memoria/efectos de los fármacos , Morfina/farmacología , Recompensa , Animales , Condicionamiento Clásico/fisiología , Relación Dosis-Respuesta a Droga , Inyecciones Intraperitoneales , Masculino , Memoria/fisiología , Ratas , Ratas Sprague-Dawley
4.
Phys Rev Lett ; 123(19): 195503, 2019 Nov 08.
Artículo en Inglés | MEDLINE | ID: mdl-31765180

RESUMEN

Topological insulators (TIs), featured by a symmetry-protected gapless surface Dirac cone(s) in their complete energy band gaps, have been extended from condensed-matter physics to classical bosonic systems in the last decade. However, acoustic TIs in three dimensions remain elusive because of a lack of a spin or polarization degree of freedom for longitudinal airborne sound. Here, we experimentally demonstrate a feasible way to hybridize an acoustic TI in three dimensions based on band inversion through a three-dimensional (3D) hybrid Dirac point (HDP). Such a 3D HDP, with linear dispersion in the layer plane while quadratic out of the layer, is distinct from a general point with linear dispersion in all directions. Interestingly, a single nearly gapless conical-like dispersion for acoustic surface states can be achieved at both zigzag and armchair interfaces, supporting robust sound transport. Our findings can serve as a tabletop platform for exploring unique acoustic applications based on the two-dimensional topological interfaces.

5.
Phys Rev E ; 98(1-1): 012127, 2018 Jul.
Artículo en Inglés | MEDLINE | ID: mdl-30110722

RESUMEN

We consider the triangular kagome XXZ-Ising model (TKL XXZ-Ising model) formed by inserting small triangles ("a-trimers") with XXZ spin-1 inside the triangles of the kagome lattice ("b-trimers"). It is a mixed spin system and can be solved exactly by transforming into the kagome lattice with the general transformation method for decorated spin systems. In the absence of an external field, we integrate out the quantum spins of the a-trimers and map the TKL model to the kagome Ising model exactly. We obtain the full phase diagram and their zero-temperature entropies (e.g., s_{max}=5.48895 per unit cell is given for the phase with the maximum entropy). When an external field is applied, 20 phases are found due to the quantum fluctuations of a-trimers. Moreover, the high spins in the a-trimers can lead to a stable quantized growth of the magnetization process in the Heisenberg limit.

6.
Phys Rev Lett ; 116(22): 226801, 2016 Jun 03.
Artículo en Inglés | MEDLINE | ID: mdl-27314733

RESUMEN

Weyl semimetals are new states of matter which feature novel Fermi arcs and exotic transport phenomena. Based on first-principles calculations, we report that the chalcopyrites CuTlSe_{2}, AgTlTe_{2}, AuTlTe_{2}, and ZnPbAs_{2} are ideal Weyl semimetals, having largely separated Weyl points (∼0.05 Å^{-1}) and uncovered Fermi arcs that are amenable to experimental detections. We also construct a minimal effective model to capture the low-energy physics of this class of Weyl semimetals. Our discovery is a major step toward a perfect playground of intriguing Weyl semimetals and potential applications for low-power and high-speed electronics.

7.
Nat Commun ; 7: 11136, 2016 Apr 01.
Artículo en Inglés | MEDLINE | ID: mdl-27033588

RESUMEN

Ideal Weyl semimetals with all Weyl nodes exactly at the Fermi level and no coexisting trivial Fermi surfaces in the bulk, similar to graphene, could feature deep physics such as exotic transport phenomena induced by the chiral anomaly. Here, we show that HgTe and half-Heusler compounds, under a broad range of in-plane compressive strain, could be materials in nature realizing ideal Weyl semimetals with four pairs of Weyl nodes and topological surface Fermi arcs. Generically, we find that the HgTe-class materials with nontrivial band inversion and noncentrosymmetry provide a promising arena to realize ideal Weyl semimetals. Such ideal Weyl semimetals could further provide a unique platform to study emergent phenomena such as the interplay between ideal Weyl fermions and superconductivity in the half-Heusler compound LaPtBi.

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