Ultrabroadband coherence-domain imaging using parametric downconversion and superconducting single-photon detectors at 1064 nm.

Coherence-domain imaging systems can be operated in a single-photon-counting mode, offering low detector noise; this in turn leads to increased sensitivity for weak light sources and weakly reflecting samples. We have demonstrated that excellent axial resolution can be obtained in a photon-counting coherence-domain imaging (CDI) system that uses light generated via spontaneous parametric downconversion (SPDC) in a chirped periodically poled stoichiometric lithium tantalate (chirped-PPSLT) structure, in conjunction with a niobium nitride superconducting single-photon detector (SSPD). The bandwidth of the light generated via SPDC, as well as the bandwidth over which the SSPD is sensitive, can extend over a wavelength region that stretches from 700 to 1500 nm. This ultrabroad wavelength band offers a near-ideal combination of deep penetration and ultrahigh axial resolution for the imaging of biological tissue. The generation of SPDC light of adjustable bandwidth in the vicinity of 1064 nm, via the use of chirped-PPSLT structures, had not been previously achieved. To demonstrate the usefulness of this technique, we construct images for a hierarchy of samples of increasing complexity: a mirror, a nitrocellulose membrane, and a biological sample comprising onion-skin cells.

Photon-counting optical coherence-domain reflectometry using superconducting single-photon detectors.

We consider the use of single-photon counting detectors in coherence-domain imaging. Detectors operated in this mode exhibit reduced noise, which leads to increased sensitivity for weak light sources and weakly reflecting samples. In particular, we experimentally demonstrate the possibility of using superconducting single-photon detectors (SSPDs) for optical coherence-domain reflectometry (OCDR). These detectors are sensitive over the full spectral range that is useful for carrying out such imaging in biological samples. With counting rates as high as 100 MHz, SSPDs also offer a high rate of data acquisition if the light flux is sufficient.

Submicron axial resolution in an ultrabroadband two-photon interferometer using superconducting single-photon detectors.

We generate ultrabroadband biphotons via the process of spontaneous parametric down-conversion in a quasi-phase-matched nonlinear grating that has a linearly chirped poling period. Using these biphotons in conjunction with superconducting single-photon detectors (SSPDs), we measure the narrowest Hong-Ou-Mandel dip to date in a two-photon interferometer, having a full width at half maximum (FWHM) of approximately 5.7 fsec. This FWHM corresponds to a quantum optical coherence tomography (QOCT) axial resolution of 0.85 ?m. Our results indicate that a high flux of nonoverlapping biphotons may be generated, as required in many applications of nonclassical light.

Ultrabroadband biphotons generated via chirped quasi-phase-matched optical parametric down-conversion.

We generate ultrabroadband biphotons via the process of spontaneous parametric down-conversion (SPDC) in quasi-phase-matched nonlinear gratings that have a linearly chirped wave vector. By using these ultrabroadband biphotons (300-nm bandwidth), we measure the narrowest Hong-Ou-Mandel dip to date, having a full width at half maximum of 7.1 fs. This enables the generation of a high flux of nonoverlapping biphotons with ultrabroad bandwidth, thereby promoting the use of SPDC light in many nonclassical applications.

Spatial coherence effects on second- and fourth-order temporal interference.

We report the results of two experiments performed with two-photon light, produced via collinear degenerate optical spontaneous parametric downconversion (SPDC), in which both second-order (one-photon) and fourth-order (two-photon) interferograms are recorded in a Mach-Zehnder interferometer (MZI). In the first experiment, high-visibility fringes are obtained for both the second- and fourth-order interferograms. In the second experiment, the MZI is modified by the removal of a mirror from one of its arms; this leaves the fourth-order interferogram unchanged, but extinguishes the second-order interferogram. A theoretical model that takes into consideration both the temporal and spatial degrees-of-freedom of the two-photon state successfully explains the results. While the temporal interference in the MZI is independent of the spatial coherence of the source, that of the modified MZI is not.

Experimental violation of Bell's inequality in spatial-parity space.

We report the first experimental violation of Bell's inequality in the spatial domain using the Einstein-Podolsky-Rosen state. Two-photon states generated via optical spontaneous parametric down-conversion are shown to be entangled in the parity of their one-dimensional transverse spatial profile. Superpositions of Bell states are prepared by manipulation of the optical pump's transverse spatial parity-a classical parameter. The Bell-operator measurements are made possible by devising simple optical arrangements that perform rotations in the one-dimensional spatial-parity space of each photon of an entangled pair and projective measurements onto a basis of even-odd functions. A Bell-operator value of 2.389+/-0.016 is recorded, a violation of the inequality by more than 24 standard deviations.

Synthesis and analysis of entangled photonic qubits in spatial-parity space.

We present the novel embodiment of a photonic qubit that makes use of one continuous spatial degree of freedom of a single photon and relies on the parity of the photon's transverse spatial distribution. Using optical spontaneous parametric down-conversion to produce photon pairs, we demonstrate the controlled generation of entangled-photon states in this new space. Specifically, two Bell states, and a continuum of their superpositions, are generated by simple manipulation of a classical parameter, the optical-pump spatial parity, and not by manipulation of the entangled photons themselves. An interferometric device, isomorphic in action to a polarizing beam splitter, projects the spatial-parity states onto an even-odd basis. This new physical realization of photonic qubits could be used as a foundation for future experiments in quantum information processing.

Selective functionalization of 3-D polymer microstructures.

We demonstrate the selective functionalization of 3-D polymer microstructures that were created using multiphoton absorption polymerization. By fabricating different portions of the structures with acrylic and methacrylic polymers, we are able to take advantage of the differential reactivities of these materials to perform functionalization chemistry on a single polymeric component. We demonstrate the selective deposition of metal to create structures, such as a functional microinductor. Our strategy is quite general and can be extended readily to the deposition of materials, such as metal oxides and biomolecules.

Broadband light generation by noncollinear parametric downconversion.

Broadband light generation is demonstrated by noncollinear spontaneous parametric downconversion with a cw pump laser. By use of a suitable noncollinear phase-matching geometry and a tightly focused pump beam, downconverted signals that feature a bell-shaped spectral distribution with a bandwidth approaching 200 nm are obtained. As an application of the generated broadband light, submicrometer axial resolution in an optical coherence tomography scheme is demonstrated; a free-space resolution down to 0.8 microm was achieved.

Non-collinear and non-degenerate polarization-entangled photon generation via concurrent type-I parametric downconversion in PPLN.

A periodically poled lithium niobate (PPLN) crystal has been used as an efficient source of non-collinearly generated polarization-entangled photon pairs at 810 and 1550 nm. The PPLN crystal was endowed with a specially designed poling pattern and the entangled photons were generated via the nonlinear optical process of spontaneous parametric down conversion (SPDC). A novel design based on overlapping two concurrent type-I quasi-phase-matching structures in a single PPLN crystals produced correlated pairs of alternatively polarized photons in largely separated spectral regions. The phase of the resulting two-photon state is directly linked to parameters of the nonlinear grating. Continuous tunability of the generated Bell state, from Phi(+) to Phi(-), has been demonstrated by translating a slightly wedged crystal perpendicular to the pump beam.

Wolf equations for two-photon light.

The spatiotemporal two-photon probability amplitude that describes light in a two-photon entangled state obeys equations identical to the Wolf equations, which are satisfied by the mutual coherence function for light in any quantum state. Both functions therefore propagate similarly through optical systems. A generalized van Cittert-Zernike theorem explains the predicted enhancement in resolution for entangled-photon microscopy and quantum lithography. The Wolf equations provide a particularly powerful analytical tool for studying three-dimensional imaging and lithography since they describe propagation in continuous inhomogeneous media.

Entangled-photon imaging of a pure phase object.

We demonstrate experimentally and theoretically that a coherent image of a pure phase object [implemented by a microelectromechanical system (MEMS) micromirror array] may be obtained by use of a spatially incoherent illumination beam. This is accomplished by employing a two-beam source of entangled photons generated by spontaneous parametric down-conversion. One of the beams probes the phase object while the other is scanned. Though each of the beams is, in and of itself, spatially incoherent, the pair of beams exhibits higher-order interbeam coherence.

Enhancing the axial resolution of quantum optical coherence tomography by chirped quasi-phase matching.

We show theoretically that a chirped quasi-phase-matching nonlinear crystal structure can significantly enhance the axial resolution in quantum optical coherence tomography by increasing the spectral width of the generated entangled photon pairs. For pulsed pumps we show how the pump-pulse duration affects the maximum resolution attainable.

Demonstration of dispersion-canceled quantum-optical coherence tomography.

We present an experimental demonstration of quantum-optical coherence tomography. The technique makes use of an entangled twin-photon light source to carry out axial optical sectioning. It is compared to conventional optical coherence tomography. The immunity of the quantum version to dispersion, as well as a factor of 2 enhancement in resolution, is experimentally demonstrated.

Decoherence-free subspaces in quantum key distribution.

We demonstrate that two recent innovations in the field of practical quantum key distribution (one-way autocompensation and passive detection) are closely related to the methods developed to protect quantum computations from decoherence. We present a new scheme that combines these advantages, and propose a practical implementation of this scheme that is feasible using existing technology.