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1.
Sci Total Environ ; 919: 170895, 2024 Apr 01.
Artículo en Inglés | MEDLINE | ID: mdl-38346652

RESUMEN

Turbulent motion is the essential difference between the atmospheric boundary layer and the free atmosphere. Due to the lack of detection methods for vertical turbulent structures, commonly used methods usually focus on material distribution, thermal effects, or dynamic effects, and they fail to reflect the boundary layer objectively in terms of turbulence. Therefore, to date, the acquisition and characteristic analysis of the atmospheric boundary layer height under turbulent angles have not been achieved. This study proposes a method for obtaining the height of the boundary layer based on the power-law exponent of atmospheric turbulence. The proposed method is validated and analyzed with data from radiosondes obtained under sunny, cloudy, and light rain weather conditions, demonstrating its advantages. With the proposed method, the first published acquisition of boundary layer height characteristics based on turbulent motion is achieved, including a statistical analysis of the daily and monthly variation characteristics of the boundary layer height over the Shenzhen area in China. Moreover, different oscillation frequencies of the boundary layer height under different wind directions are revealed. The results of this study break the traditional bottleneck of not being able to obtain the height of the boundary layer based on turbulence, and provide a new perspective for the acquisition and research of the boundary layer height.

2.
Heliyon ; 9(8): e18641, 2023 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-37560661

RESUMEN

Based on the simulation of the fluid-structure interaction response, the cause of an overturning of a gantry crane induced by a downburst in Shenzhen is studied in this paper. According to the results, (1) Vicroy's downburst model could establish the steady-state wind field of the downburst more reasonably when there was only low-level wind speed observation data, and its simulation results were close to the two-dimensional downburst numerical simulation results; (2) Compared with the normal exponential vertical profile of wind speed, the disturbance caused by the front girder of the double-girder gantry crane structure under the downburst wind field was more severe, which increases the probability of the gantry crane overturning. (3) The downwind displacement of the main girder of the gantry crane under the condition of downburst is far greater than that under the normal condition. At the same time, under the condition of downburst, the pressure difference on the surface of the gantry crane was greater, and the distribution of the support reaction force was more uneven, resulting in a stronger overturning tendency of the gantry crane. (4) Under the condition of downburst, the overturning moment and the shearing force borne by the foundation of gantry crane exceeded the critical value to maintain the stability of the gantry crane by the gravity, resulting in the overturning of the gantry crane.

3.
Sci Total Environ ; 902: 166001, 2023 Dec 01.
Artículo en Inglés | MEDLINE | ID: mdl-37536585

RESUMEN

Extremely high-temperature lightning generates NOx by electrolyzing nitrogen and oxygen molecules, regulating ozone concentration. The Pearl River Delta (PRD) is located in the world's high-value area of lightning density, and lightning-generated NOx (LNOx) cannot be ignored. Using the flash data from Guangdong-Hong Kong-Macao Lightning Location System and multi-site atmospheric composition data, we estimate the NOx variations in lightning activity and its impact on O3 across the PRD region. The cloud-to-groud (CG) frequency from 2013 to 2021 shows a decreasing trend driven by urban regions. We observe that the lightning density is steadily decreasing from the south-central part of Guangzhou City to the surrounding area. A comparison of the different sites with lightning days and non-lightning days shows that a significant amount (13. 84-20. 47 %) of ground-level NOx concentration at urban stations can be attributed to lightning NOx emissions. A lower lightning frequency and low background concentration observed at suburban sites indicated a limited contribution of LNOx. The average decrease in O3 concentration at urban stations (15.92-25.06 %) was significantly higher than that at suburban stations (5.34-8.95 %) due to the influence of titration and lower actinic radiation. There was a greater fluctuation in NOx and O3 concentrations during the cases, and the surface NOx concentration displayed the most significant responsiveness to LNOx under direct lightning striking in the tall tower. This phenomenon has not been reported, however, it is consistent with the laboratory-based observations suggesting the amount of LNO increases with peak current. LNOx significantly impacts air quality in the PRD during the high convective season. Further in situ and vertical distribution observations are necessary to explore the ground-level impact of LNOx.

4.
Huan Jing Ke Xue ; 44(6): 3117-3129, 2023 Jun 08.
Artículo en Chino | MEDLINE | ID: mdl-37309931

RESUMEN

The short-term reduction of air pollutant emissions is an important emergency control measure for avoiding air pollution exceedances in Chinese cities. However, the impacts of short-term emission reductions on the air qualities in southern Chinese cities in spring has not been fully explored. We analyzed the changes in air quality in Shenzhen, Guangdong before, during, and after a city-wide lockdown associated with COVID-19 control during March 14 to 20, 2022. Stable weather conditions prevailed before and during the lockdown, such that local air pollution was strongly affected by local emissions. In-situ measurements and WRF-GC simulations over the Pearl River Delta (PRD) both showed that, due to reductions in traffic emissions during the lockdown, the concentrations of nitrogen dioxide (NO2), respirable particulate matter (PM10), and fine particulate matters (PM2.5) in Shenzhen decreased by (-26±9.5)%, (-28±6.4)%, and (-20±8.2)%, respectively. However, surface ozone (O3) concentration did not change significantly[(-1.0±6.5)%]. TROPOMI satellite observations of formaldehyde and nitrogen dioxide column concentrations indicated that the ozone photochemistry in the PRD in spring 2022 was mainly controlled by the volatile organic compound (VOCs) concentrations and was not sensitive to the reduction in nitrogen oxide (NOx) concentrations. Reduction in NOx may even have increased O3, because the titration of O3 by NOx was weakened. Due to the small spatial-temporal extent of emission reductions, the air quality effects caused by this short-term urban-scale lockdown were weaker than the air quality effects across China during the widespread COVID-19 lockdown in 2020. Future air quality management in South China cities should consider the impacts of NOx emission reduction on ozone and focus on the co-reduction scenarios of NOx and VOCs.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , COVID-19 , Ozono , Compuestos Orgánicos Volátiles , Humanos , Dióxido de Nitrógeno , Control de Enfermedades Transmisibles , Óxido Nítrico , Material Particulado
5.
Opt Express ; 30(15): 27462-27471, 2022 Jul 18.
Artículo en Inglés | MEDLINE | ID: mdl-36236917

RESUMEN

Sea fog changes widely and rapidly, and existing Lidar scanning speeds are insufficient to detect such changes. Therefore, we developed a Lidar system with a fast scanning speed and long detection distance. Experimental results show that at high scanning speeds, the maximum correlation between the Lidar's visibility results and those from two forward scattering visibility meters reaches 0.9537, with a minimum relative error less than 15.31%. The results also show that the visibility of the proposed Lidar system has high accuracy when fast scanning. During the tests, the Lidar system successfully captured sea fog many times and closely tracked the changes of sea visibility, which verifies the feasibility and reliability of the developed Lidar system for obtaining visibility measurements and sea fog detection.

6.
Sci Total Environ ; 853: 158657, 2022 Dec 20.
Artículo en Inglés | MEDLINE | ID: mdl-36096219

RESUMEN

Black carbon (BC) is a vital climate forcer in the atmosphere, but measurements of BC vertical profiles near the surface remain limited. This study investigates time-resolved vertical profiling of BC in both dry (December 2017) and wet (August 2018) seasons in Shenzhen, China, at a 356-m meteorological tower. In the dry season, five micro-aethalometers were deployed at different heights (2, 50, 100, 200, and 350 m), while four heights (2, 100, 200, and 350 m) were measured in the wet season. The concentrations of equivalent BC (eBC) showed a decreasing trend with altitude in the dry season, while a weaker vertical gradient was observed in the wet season. The diurnal variability of eBC in the dry season is also more significant than in the wet season. Correlation analysis between eBC concentrations at the ground and those at the upper levels suggest a better vertical mixing of eBC in the wet season than in the dry season. In the wet season when south wind prevailed, eBC concentration at ground level was likely reduced by the large amount of vegetation cover south to the sampling site. In the dry season, eBC concentrations at 350 m show little dependence on wind speed, implying that local emissions have a limited effect on eBC concentrations at 350 m. In the wet season when brown carbon influence was weak, higher wind speed leads to a higher Ångström exponent (AAE) at 350 m, likely associated with more aged BC particles. Cluster analysis of backward trajectories suggests that high eBC concentration was associated with air masses from Central China in both seasons. This study provides a better understanding on the influencing factors that affect the vertical distributions of BC in the lower part of the boundary layer.


Asunto(s)
Contaminantes Atmosféricos , Estaciones del Año , Contaminantes Atmosféricos/análisis , Aerosoles/análisis , Monitoreo del Ambiente , Hollín/análisis , Carbono/análisis , China
7.
Atmos Environ (1994) ; 276: 119068, 2022 May 01.
Artículo en Inglés | MEDLINE | ID: mdl-35342324

RESUMEN

The outbreak of the 2019 novel coronavirus (COVID-19) had a large impact on human health and socio-economics worldwide. The lockdown implemented in China beginning from January 23, 2020 led to sharp reductions in human activities and associated emissions. The declines in primary pollution provided a unique opportunity to examine the relationship between anthropogenic emissions and air quality. This study reports on air pollutant and meteorological measurements at different heights from a tall tower in the Pearl River Delta. These measurements were used to investigate the vertical scale response of pollutants to understand reductions in human activities. Compared to that in the pre-lockdown period (from December 16, 2019), the concentrations of surface layer nitric oxide (NOx), fine particulate matter (PM2.5), and daily maximum 8 h average ozone (MDA8O3) declined significantly during the lockdown by 76.8%, 49.4%, and 18.6%, respectively. Although the vertical profiles of NOx and O3 changed during the lockdown period, those of PM2.5 remained the same. During the lockdown period, there were statistically significant correlations between PM2.5 and O3 but not between PM2.5 and NOx at four heights, indicating that the main composition of PM2.5 have dramatically changed, during which the impact of NOx on PM2.5 became insignificant. Additionally, O3 concentrations were also insensitive to NOx concentrations during the lockdown, implying that O3 levels were more of a representative of regional background level. In this case, local photochemical formation is no longer a significant ozone source. This evidence suggests that it is possible to mitigation of PM2.5 and O3 levels simultaneously by significant reductions in anthropogenic emissions.

8.
Sci Total Environ ; 801: 149689, 2021 Dec 20.
Artículo en Inglés | MEDLINE | ID: mdl-34425446

RESUMEN

Existing studies on vertical profiling of black carbon (BC) and ozone (O3) were mainly conducted in the rural areas, leading to limited knowledge of their vertical distributions in the urban area. To fill this knowledge gap, vertical profiling (0-500 m and 0-900 m, AGL) of BC and O3 was conducted in a highly urbanized area of Shenzhen in subtropical South China using a multicopter unmanned aerial vehicle (UAV) platform. In total 32 flights were conducted from the 10th to 15th, December 2017 (winter campaign) and 42 flights from the 19th to 28th, August 2018 (summer campaign) with 4 time slots per day, including morning, afternoon, evening, and midnight. In general, equivalent BC (eBC) concentration decreased as the height increased with an overall slope of -0.13 µg m-3 per 100 m in the winter campaign and -0.08 µg m-3 per 100 m in the summer campaign. On the contrary, an increase of O3 level with altitude was observed (7.8 ppb per 100 m). Absorption Ångström exponent (AAE) exhibits a slightly increasing trend with height. Seasonality of eBC vertical profiles was observed in morning, afternoon and midnight flights, but not for evening flights. The analysis showed the shape of vertical profiles of eBC and O3 can be affected by planetary boundary layer height (PBLH) and air mass origin. Calculated heating rates due to BC show distinct seasonal variability for morning but not for afternoon, because of the counteracting effects by solar irradiance in the subtropical afternoon and eBC concentration in urban South China influenced by the monsoon climate.


Asunto(s)
Contaminantes Atmosféricos , Ozono , Contaminantes Atmosféricos/análisis , Carbono/análisis , China , Monitoreo del Ambiente , Ozono/análisis , Estaciones del Año
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