Estimation of radiological health risks due to 226Ra, 232Th, and 40K in foods consumed in Iraqi Kurdistan Region.

This study investigates the activity concentration of natural radionuclides in a diverse range of food samples in the Koya district markets food baskets, including both domestic and imported products. The samples cover annual crops (e.g. coffee, tea, kidney beans), tree nuts (e.g. almonds, pistachios), and other items (e.g. beef, fish, milk) by using a high-purity germanium (HPGe) detector. This research addresses a notable gap by providing baseline data on radionuclide concentrations and assessing potential health risks. Average activity concentrations for ²²6Ra, ²³²Th, and 4°K were 0.943, 0.367, and 191.8 Bq kg-1, respectively. Radium equivalent activity values ranged from 2.88-58.48 Bq kg-1, all below the safety limit. The average excess lifetime cancer risk (ELCR) was 0.154 mSv a-1, indicating safety for most samples, though coffee and tea showed higher levels. This study provides new data crucial for future research and regulatory monitoring, underscoring the need for further investigation into geological impacts on radionuclide levels.

Mineral exploration and environmental impact assessment in the Jabal Hamadat Area, Central Eastern Desert, Egypt, using remote sensing and airborne radiometric data.

Mineral exploration is essential for economic growth, but it must be conducted with careful consideration of health and environmental impacts. This study focuses on mapping potential mineralization areas and evaluating environmental consequences in the Jabal Hamadat area. By integrating ASTER, Landsat-9 and airborne radiometric data, the study includes: (1) identification of alteration mineral indicators including iron oxides (gossanized zone), chlorite (propylitic zone), kaolinite, sericite, montmorillonite/illite (argillic zone), and alunite (advanced argillic zone) via the Band Ratio (BR) technique; (2) preparation of a lineament density map through an automated lineament extraction technique; and (3) identification of areas with elevated F-parameter values exceeding 10. Ten areas with high mineralization potential are delineated for further exploration. Additionally, the study assesses environmental radiation exposure, finding that certain areas exceed the safe radiation limit of 1.0 mSv/year. Peak radiation levels range from 0.75 to 1.25 mSv/year, with mining sites showing the highest readings at 1.25 mSv/year and 0.64 mSv/year. These findings highlight elevated radiological hazards, emphasizing the need for comprehensive monitoring and effective mitigation strategies to protect human health and minimize environmental impact. The methodology's success in this area indicates its potential applicability to other mining areas, contributing to enhanced safety and environmental protection.

Natural radionuclide profiles and radiological risks in soils and rocks of the Koytash-Ugam Range, Uzbekistan.

This investigation quantifies the activity concentrations of natural radionuclides (226Ra, 232Th, and 40K) in the soils and certain rocks of the Koytash-Ugam Range, Uzbekistan, and assesses their radiological risks. Gamma-spectrometric analysis of soil and rock samples revealed activity concentrations ranging from 456.2 ± 56.0 to 813.9 ± 76.0 Bq kg-1 for 40K, 18.2 ± 6.3 to 70.0 ± 12.0 Bq kg-1 for 226Ra, and 30.1 ± 2.9 to 57.9 ± 10 Bq kg-1 for 232Th. This data indicates a heterogeneous distribution of radionuclides, informing radiation safety and health risk assessments on a global scale. The calculation of radiological hazard indices, including the alpha-index (ranging from 0.09 to 0.35), gamma-index (ranging from 0.40 to 0.73), and both internal (ranging from 0.40 to 0.54) and external (ranging from 0.36 to 0.54) hazard indices, was undertaken to ascertain potential health risks. The radium equivalent activity ranged from 108.4 to 199.3 Bq kg-1, and the absorbed dose rates were 51.0-93.3 nGy h-1 indoors and 96.6-178.2 nGy h-1 outdoors. These metrics underlie the estimated annual effective dose of 536.5-988.5 × 10-3 mSv y-1, highlighting the variability in radiation exposure. Additionally, the potential lifetime cancer risk was projected at 1770.4 to 3262.0 per million, with an annual gonadal dose equivalent of 361.9 to 655.5 µSv y-1, reflecting natural background radiation influence. The results underscore the importance of safe material use in construction and the necessity for routine natural radioactivity monitoring. Radon flux density (RFD) values within acceptable construction limits (26-176 mBq m-2 s-1) suggest the area's suitability for development, considering recommended safety guidelines. This study not only aids local environmental and public health frameworks but also enriches the international knowledge base, facilitating comparative studies for the advancement of global radiation protection standards. Through a detailed examination of radionuclide distribution in an under-researched area, our research highlights the critical need for integrated international approaches to natural radiological hazard assessment.

Assessment of potential human health, radiological and ecological risks around mining areas in northeastern Brazil.

Mining is responsible for the release of metallic pollutants and radioactive materials into the environment, which have the potential to disrupt ecosystems and pose significant risks to human health. Significant mining activity is concentrated in the municipality of Caetité (northeastern Brazil), where Latin America's only active uranium mine and significant iron ore deposits are located. Although previous studies have shown that the regional soil and water resources are highly contaminated by various toxic elements and that exposure to these elements is known to have adverse effects on human health, the health risks in this mining region have never been assessed. The aim of this unprecedented comprehensive investigation was to assess the health, radiological and ecological risks in this mining region, which is home to nearly 100,000 people. To achieve our goal, soil and water samples were collected in the vicinity of the mines and in the main settlements in the region. Fifteen metallic toxic elements were determined using Instrumental Neutron Activation Analysis and Inductively Coupled Plasma Optical Emission Spectrometry. The HERisk code, which follows the main methodological guidelines for risk assessment, was used to quantify human health, radiological and ecological indices. The average values of the total risk and cancer risk indices indicated that region falls into the moderate risk category (1.0 ≤ HItot < 4.0). However, 63% of the sites had high risk values, with Fe, Co and As being the metals contributing most to total and cancer risk, respectively. Near the mining areas, the potential ecological risk can be considered extreme (PERI ≥ 600). The values of the calculated radiological indices correspond to typical values ​​in natural uranium areas. However, in the communities near the mine, the dose values are slightly above the permissible limit (1 mSv y-1), so they must be continuously monitored, and risk mitigation measures must be taken.

Natural radionuclides and radiological risk assessment in the stream and river sediments of a high background natural radiation area Kanyakumari, India.

The Kanyakumari coast is known to be a high background natural radiation area due to the placer deposits of heavy minerals such as ilmenite, monazite, and rutile. The Kanyakumari river sediments that could be the source of the elevated amounts of natural radionuclides in the coastal sands have been studied in this paper. The activity concentrations of primordial radionuclides 226Ra, 232Th, and 40K were determined using high-purity germanium (HPGe) gamma-ray spectrometry. The mean activity concentrations of 226Ra, 232Th, and 40K were found to be 75 Bq kg-1, 565 Bq kg-1, and 360 Bq kg-1, respectively. The mean absorbed dose rate was 395 nGy h-1. Radiological hazard parameters were studied and compared with the world average values. The contribution of 232Th to the total dose rate was found to be higher than that of the two other radionuclides. The high mean ratio of 232Th/226Ra suggested an enrichment of 232Th and the occurrence of 226Ra leaching due to an oxidizing environment. Principal component analysis (PCA) was carried out for the radionuclides in order to discriminate the source of the sediments. This study provides new insights into the distribution of natural radionuclides in sediments of rivers and streams.

Radionuclides distribution and radiation hazards assessment of black sand separation plant's minerals: a case study.

This study assessed the radioactivity levels and associated risks in the black sand-separated products obtained from the black sand separation plant in Delta, Egypt. A total of sixteen samples were taken from hot spots during and after the separation process. These include water samples and other samples that represent monazite, rutile, zircon, granite, ilmenite, and silica products. The hot spots included the area where the ore was stored. The activity concentrations of 232 T h , 226 R a , and 40 K were determined in these samples using a p-type HPGe detector. Based on gamma spectrometric analysis, samples of rutile, zircon, and monazite had the highest amounts of radioactivity because they contained the highest NORM's activity concentrations. In addition, it indicated that the radiological hazard indices of the collected samples were higher than the average world limits for sand texture. These findings suggest that the black sand separation process reveals potential risks to human health and the environment, and therefore, appropriate measures need to be taken to mitigate these risks, especially for the safety of the workers on-site. Reducing the risk associated with those sites should be controlled by implementing the recommendations declared for the series of International Basic Safety Standards of the International Atomic Energy Agency (GSR) Part 3, as affirmed in Document No. 103 of 2007 by the International Commission on Radiological Protection (ICRP) as will be presented in the paper body.

Radiological hazard assessment of 210Po in freshwater mussels (Sinanodonta jourdyi) and golden apple snail (Pomacea canaliculata) in Vietnam.

210Po is a significant source of ionizing radiation that people are exposed to through food globally. This paper presents the wide range of accumulation level of 210Po in the organs of two species of shellfish including freshwater mussel (Sinanodonta jourdyi) and golden apple snail (Pomacea canaliculata), common freshwater species in Vietnam. There was a significant correlation between 210Po activity in muscle to their mass and size of freshwater mussels. In contrast, there was no relation between other organs of both species with their mass and size. The annual effective dose due to consumption of freshwater mussels ranged from 68.7 to 291 µSv year-1 with a mean value of 138 µSv year-1 for muscle and from 321 to 4560 µSv year-1 with a mean value of 1422 µSv year-1 for the hepatopancreas. Meanwhile, the AED for golden apple snail was recorded to be higher with values ranging from 105 to 2189 µSv year-1 with mean value of 673 µSv year-1 for muscle and from 468 to 4155 µSv year-1 with a mean value of 2332 µSv year-1 for hepatopancreas. Thus, the consumption of these two types of shellfish is considered relatively safe, but the hepatopancreas gland must be removed before processing.

Evaluation of radioactivity in soil and rock samples from an undiscovered sea beach in the southeastern coastline of Bangladesh and associated health risk.

This study marks the first-ever assessment of radiological hazards linked to the sands and rocks of Patuartek Sea Beach, situated along one of the world's longest sea beaches in Cox' Bazar of Bangladesh. Through the utilization of an HPGe detector, a comprehensive analysis of the activity concentrations of 226Ra, 232Th, and 40 K was conducted, and their activity ranged from 7 to 23 Bq/kg, 9-58 Bq/kg, and 172-340 Bq/kg, respectively, in soils, and 19-24 Bq/kg, 27-39 Bq/kg, and 340-410 Bq/kg, respectively, in rocks. Some sand samples exhibited elevated levels of 232Th, while the rock samples displayed higher levels of 40 K compared to the global average. The radiological hazard parameters were assessed, and no values surpassed the recommended limits set by several international organizations. Hence, the sands and rocks of Patuartek sea beach pose no significant radiological risk to the residents or tourists. The findings of this study provide crucial insights for the development of a radiological baseline map in the country, which is important due to the commissioning of the country's first nuclear power plant Rooppur Nuclear Power Plant. The data may also stimulate interest in the rare-earth minerals present in the area, which is important for the electronics industry, thorium-based nuclear fuel cycles.

Distribution of natural radionuclides in NORM samples from North Abu Rusheid area, Egypt.

The North Abu Rusheid area in Egypt is a well-known high background natural radiation area (HBNRA) due to the existence of naturally occurring radioactive materials (NORMs) in mylonitic rocks. In this study, 27 rock samples were selected for dose estimation studies. 238U and 232Th were measured using inductively coupled plasma mass spectrometry (ICP-MS) and 40K was measured using sodium iodide (thallium) gamma-ray spectroscopy. The ranges of activity concentrations (Bq/kg) of 238U, 232Th and 40K in the samples varied from 270 ± 2 to 2120 ± 29, 350 ± 2 to 1840 ± 27 and 20 ± 2 to 1390 ± 35 with mean values of 980 ± 349, 770 ± 351, and 640 ± 402 Bq/kg, respectively. The radiological hazard parameters were estimated from activity concentrations of 238U, 232Th and 40K and compared to United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) values. The present study revealed that the hazard parameters were several times higher than the worldwide averages. The U/Th concentration ratio ranged from 0.7 to 3 and could be attributed to the presence of kasolite, uranothorite, zircon, and columbite in mylonitic rocks. From the radiological protection viewpoint, it is necessary to monitor natural radionuclides in these rocks prior to their use in residential and commercial construction materials.

Radiological assessment in beach sediment of coastline, Ghana.

The natural and artificial radioactivity in beach sediment sampled from the coastline of Ghana were analyzed using High Purity Germanium gamma ray detector. The overall average activity concentrations of 226Ra, 232Th, 40K and 137Cs were estimated to be 43 ± 6, 22 ± 1, 393 ± 74 and 8.4 ± 0.5 Bqkg-1, respectively. Apart from 226Ra the mean activity concentrations of the measured radionuclides were below the world averages of 32, 45, 412 and 18.2 Bqkg-1 respectively. High 137Cs mean concentration of 109.8 Bqkg-1 was observed for one of the locations, which might be due to the occurrence of a nuclear incidence or other factors. The evaluated radiological parameters also had values below world averages, except for some coastal areas which recorded Annual Gonadal Dose Equivalent (AGDE) values higher than the reference level of 300 µSvy-1. There was no significant risk associated with the radionuclide activities evaluated along the coast of Ghana. The correlation between the radionuclides and the radiological parameters were analyzed with the Pearson correlation matrix, cluster and PCA analysis, and they all showed similar outcomes. Spatial distribution maps were also created using ArcGIS software for a pictorial view of the distribution of radionuclides along the study area.

Radiological risk assessment of outdoor222Rn and220Rn around rare earth element and uranium mines from northern Vietnam.

The outdoor222Rn and220Rn concentrations at 320 sampling points at 1 m above the ground in different sites surrounding rare earth element (REE) and uranium mines from northern Vietnam were measured using the RAD7. Results showed that222Rn concentrations were always higher than220Rn concentrations with large variation ranges from 25.7 to 573 Bq m-3and from 18.5 to 385 Bq m-3, respectively. The high correlation between220Rn and228Ra concentrations in surface soil of the studied sites were observed. The highest220Rn and222Rn concentrations are found at the sampling points of the REE NX-Lai Chau site. The220Rn and222Rn activities surrounding the REE mines were found to be higher than those surrounding the uranium mines. The average annual committed effective doses originated from the inhalation of220Rn and222Rn outdoor concentrations is about five times higher than the worldwide average value.

Natural radioactivity for soil samples in primary schools at Najaf city, Iraq.

Natural radiation is the most significant contribution to the annual exposure of the world population, making it essential to assess the quantity of natural radiation in soil. This research aims to assess the level of natural radioactivity within the soil samples taken from primary schools in Al-Najaf, Iraq using gamma-ray spectroscopy. Specific activity was determined for the 238U series (214Bi), 232Th series (218Tl), 40K, and 235U. Twelve radiological hazard indices were computed. SPSS software version 23.0 was employed for data statistical analyzes to include average, standard error, standard deviation, box plot, frequency distribution, and Pearson's correlation coefficient. The results of the concentrations of 238U, 232Th, and 40K, were drawn using a geographic information system (GIS) technique. The results showed that the average values and standard error of 238U, 232Th, 40K, and 235U were 20.1 ± 0.65 Bq/kg, 11.5 ± 0.22 Bq/kg, 330.9 ± 7.1 Bq/kg, and 0.926 ± 0.03 Bq/kg, respectively. The results of 238U, 232Th, 40K, and 235U were compared to the average world value. This indicates that some schools' 238U and 40K levels had exceeded the acceptable worldwide levels. At the same time, the results of radiological hazard indices were seen to be within the permissible worldwide levels. As a result, the elementary schools under study can be argued that they are relatively free of natural radiation threats. The resulted data of the current research might be contributed to the database of natural radioactivity levels and radiation doses received by those who come into touch with these schools.

Estimation of radiological impact of the activities of Olusosun Dump Site on workers and dwellers of Olusosun, in Lagos Southwest Nigeria.

This study assessed the potential radiological risks associated with the activities on Olusosun dump site on workers and dwellers of Olusosun community. The activity concentrations of 238U, 232Th and 40K from of soil and water samples were determined using High-Purity Germanium (HPGe) detector. The background radiation level of Olusosun dump site was measured using a portable Geiger-Müller counter-Radeye B20 survey meter. The mean value of background radiation was 1.46 mSv/yr. This value is about 46% higher than the recommended reference level of 1.0 mSv/yr for the public. The mean activity concentrations of 238U, 232Th and 40K in the soil samples were 19.1 ± 3.2, 29.1 ± 4.4 and 171.5 ± 6.1 Bq/kg respectively which are about 45.4%, 35.3% and 59.2% lower than the world's average levels. For the water samples, the mean activity concentrations obtained for 238U, 232Th and 40K are 0.4 ± 0.4, 0.8 ± 0.2 and 0.8 ± 0.3 Bq/l respectively. These are about 99.9% and 20% lower than WHO reference levels for 238U and 232Th. The mean absorbed dose rate in air (D), Annual effective dose (AED) outdoor, Radium Equivalent (Req), External hazard index (Hex) internal hazard index (Hin) and Excess lifetime cancer risk (ELCR) from soil samples were 33.6 nGy/h, 41.0 µSv/yr, 73.1 Bq/kg and 0.2, 0.3 and $1.4\times{10}^{-4}$, respectively. Absorbed dose in air D, AED outdoor, Req, Hex, Hin and ELCR are 41.1%, 41.4%, 80.3%, 80%, 75% and 50% lower than their corresponding world's average and references. The estimated AEDw from ingestion of water is 148.9 ± 50.4 µSv/yr, this is about 49% higher than the WHO reference level of 100.0 µSv/y from ingestion of water. The radiological hazard indices estimated from soil samples do not indicate any potential risks to the users. The elevated background radiation level of the dump site, and AEDw from ingestion of water, however, suggest that the activities on Olusosun dump site pose potential radiological risks on workers on the site and the public from consumption of water from Olusosun community.

Study of activity concentrations of 40K, 238U and 232Th for assessment of radiation dose in agricultural soils of southwestern Nigeria.

Gamma spectrometric measurement of natural radionuclides activity concentrations by HPGe detectors was conducted in 150 agricultural soil samples collected from six states of southwestern Nigeria. The overall activity concentrations of radionuclides ranged from 15.27 to 972.00 Bqkg-1 for 40K, 0.66 to 336.19 Bqkg-1 for 232Th and 1.32 to 123.01 Bqkg-1 for 238U, with mean values of 143.95, 17.02 and 22.92 Bqkg-1, respectively. The overall averages results from this study were generally lower than worldwide average value of 420, 33 and 45 Bqkg-1 for 40K, 238U and 232Th, respectively, thus minimal transfer to plant may be expected. The estimated radiation dose levels of the soil indicated acceptable limits for general public exposure. The radioactivity levels of 40K, 232Th and 238U in the investigated agricultural soil of southwestern Nigeria are within acceptable limits. Therefore, stochastic radiological health effects of radiation exposure by farmers may not be feasible at the current moment.

Natural radioactivity and its radiological implications from soils and rocks in Jaintiapur area, North-east Bangladesh.

Natural radioactivity concentrations in recent alluvial soils from swampy areas and Tertiary rocks from Jaintiapur were measured using gamma-ray spectrometer equipped with HPGe detector. The average radioactivity concentration of 226Ra, 232Th and 40K were 47 ± 6, 64 ± 5 and 762 ± 40 Bqkg-1 in soils, whereas, 25 ± 2, 37 ± 4 and 884 ± 41 Bqkg-1 in rock samples, respectively. Average radioactivity concentrations of studied soil and rock samples exceeded the world average except 226Ra for rocks. Radio-elemental ratios suggest that an oxic depositional environment with low uranium and high thorium content. Regarding radiological hazard indices, radium equivalent activities (Raeq), external hazard index (H ex) and internal hazard index (H in) was found to be below the world permissible limits. Whereas, absorbed dose rate (D), and annual effective dose equivalent (AEDE) averages exceeded the world admissible values. Statistical studies show that radioactivity for 226Ra and 232Th linked to a source enriched in radioactive minerals and 40K related to a different sources high in K enriched minerals.

Distribution of Radionuclides and Radiological Health Assessment in Seih-Sidri Area, Southwestern Sinai.

The current contribution goal is to measure the distribution of the radionuclide within the exposed rock units of southwestern Sinai, Seih-Sidri area, and assess the radiological risk. Gneisses, older granites, younger gabbro, younger granites, and post granitic dikes (pegmatites) are the main rock units copout in the target area. Radioactivity, as well as radiological implications, were investigated for forty-three samples from gneisses (seven hornblende biotite gneiss and seven biotite gneiss), older granites (fourteen samples), and younger granites (fifteen samples of syenogranites) using NaI (Tl) scintillation detector. External and internal hazard index (Hex, Hin), internal and external level indices (Iα, Iγ), absorbed dose rates in the air (D), the annual effective dose equivalent (AED), radium equivalent activity (Raeq), annual gonadal dose (AGDE), excess lifetime cancer risk (ELCR), and the value of Upper Continental Core 232Th/238U mass fractions were determined from the obtained values of 238U, 232Th and 40K for the examined rocks of Seih-Sidri area. The average 238U mg/kg in hornblende biotite gneiss and biotite gneiss, older granites, and syenogranites is 2.3, 2.1, 2.7, and 8.4 mg/kg, respectively, reflecting a relatively higher concentration of uranium content in syenogranites. The results suggest that using these materials may pose risks to one's radiological health.

Hazards of Radioactive Mineralization Associated with Pegmatites Used as Decorative and Building Material.

The present study aimed to assess the radiological hazards associated with applying the investigated granite in the building materials and the infrastructures applications. The investigated granites are classified into four categories: El-Urf, barren, colourful and opaque. El Urf monzogranite intrudes metagabbro diorite complex with sharp contacts. Based on the activity concentrations, the environmental parameters such as absorbed dose rate (Dair), annual effective dose (AED), radium equivalent activity (Raeq), external (Hex) and internal (Hin) hazard indices were measured. The mineralized pegmatite is located in the southwestern foothill of the Gabal El Urf younger granite. It displays well-defined zonation of three zones: outer, middle and inner zones represented by potash feldspar, quartz and mica, respectively. The isorad map showed that El Urf monzogranite is barren (Up to 100 cps) surrounding an excavation of the studied pegmatite that exhibits moderate colorful mineralization (phase-I = 500-1500 cps) and anomalous opaque mineralization (phase-II = 1500-3500 cps) pegmatites. The obtained results of radionuclides activity concentrations illustrated that the Opaque granites have the highest values of 238U (561 ± 127 Bq kg-1), 232Th (4289 ± 891 Bq kg-1) and 40K (3002 ± 446 Bq kg-1) in the granites, which are higher than the recommended worldwide average. Many of the radiological hazard parameters were lesser than the international limits in the younger granites and barren pegmatites. All of these parameters were higher in the colorful and opaque mineralized pegmatites. The high activity and the elevated radiological hazard parameters in the mineralized pegmatites are revised to the presence of radioactive and radioelements bearing minerals, such as thorite, meta-autunite, kasolite, phurcalite, columbite, fergusonite, Xenotime and fluorapatite. Other instances of mineralization were also recorded as cassiterite, atacamite, galena, pyrite and iron oxide minerals. Thus, the granites with high radioactivity concentration cannot be applied in the different applications of building materials and ornamental stones.

Radiological Hazard Evaluation of Some Egyptian Magmatic Rocks Used as Ornamental Stone: Petrography and Natural Radioactivity.

Magmatic rocks represent one of the most significant rocks due to their abundance, durability and appearance; they can be used as ornamental stones in the construction of dwellings. The current study is concerned with the detailed petrography and natural radioactivity of seven magmatic rocks. All are commercial granitic rocks and are identified as black Aswan, Nero Aswan, white Halayeb, Karnak, Verdi, red Hurghada and red Aswan. Their respective mineralogical compositions are classified as porpheritic granodiorite, granodiorite, tonalite, monzogranite, syenogranite, monzogranite and syenogranite. A total of nineteen samples were prepared from these seven rock types in order to assess their suitability as ornamental stones. Concentrations of 226Ra, 232Th and 40K radionuclides were measured using NaI (Tl) scintillation gamma-ray spectrometry. Among the studied magmatic rocks, white Halayeb had the lowest average values of 226Ra (15.7 Bq/kg), 232Th (4.71 Bq/kg) and 40K (~292 Bq/kg), all below the UNSCEAR reported average world values or recommended reference limits. In contrast, the other granitic rocks have higher values than the recommended limit. Except for the absorbed dose rate, other radiological hazard parameters including radium equivalent activity, annual effective dose equivalent, external, and internal hazard indices reflect that the White Halyeb rocks are favorable for use as ornamental stone in the construction of luxurious and high-demand residential buildings.

Heavy metals concentrations and naturally occurring radionuclides in soils affected by and around a solid waste dumpsite in Osogbo metropolis, Nigeria.

The presence of heavy metals and naturally occurring radioactive materials (NORMs) in high concentrations in soils can be hazardous to exposed humans. This study is aimed at measuring the concentrations of heavy metals (Cu, Pb, Ni, Zn, Cd, Co, and Cr) and activity concentration of 232Th, 238U, and 40K in soils affected by and around a solid waste dumpsite in Osogbo metropolis, Nigeria. Atomic absorption spectrometry and gamma-ray spectrometric techniques were used to determine the concentrations of metals and NORMs, respectively. Possible environmental impact of the heavy metal content and the probable radiological hazard by the NORMs to the general public were assessed. The calculated pollution indices reported in this work for Co, Cr, Pb, and Ni show low pollution status. Geoaccumulation indices for Cu, Zn, and Cd indicated that the area under study is strongly contaminated by these metals. Evaluated ecological risk index narrowed down Cd as the poisonous metal with high concentration. The measured radionuclides' mean activity concentrations and the evaluated mean of radium equivalent and absorbed dose rate values are higher than the recommended safe limit, an indication of possible radiological hazard. The principal factor analysis results explained 76% of the collection of data and described chips of galvanized/chrome metals, scrap metals, waste from electronics, Cr, and Cd-containing waste as sources of the heavy metals. The practice of land cultivation around the dumpsite should be deterred to prevent the transportation of these vicious heavy metals into the food chain.

Assessment of radiation hazard indices due to natural radioactivity in soil samples from Orlu, Imo State, Nigeria.

The use of a Radiation Alert Inspector device and a gamma-spectrometry system fitted with a Sodium Iodide (NaI) detector was used to determine the radioactivity concentration level of natural radionuclides 238U, 232Th, and 40K in soil in several locations in Orlu, Imo State, Nigeria. 19 soil samples were collected for analysis from several locations of factories, agricultural farming-lands, gullies and water eroded areas, and soil deposits very close to flowing waters from rocks, due to environmental concerns arising from human activities in this region. The activity concentration values for 238U, 232Th, and 40K were found to range from 0.14 to 9.34 Bq.kg-1, 0.03-3.75 Bq.kg-1, and 16.83-783.06 Bq.kg-1, respectively, with average mean values of 4.15, 1.64, and 134.13 Bq.kg-1. Radium equivalent activity, absorbed dose rate, and gamma index mean values for the samples were 16.822 Bq.kg-1, 8.528 nGyh-1, and 0.133 mSv respectively, the obtained values were below the safe limit values set by the United Nations Scientific Committee on the Effects of Atomic Radiation of 370.0 Bq.kg-1, 59.0nGyh-1, and 1.0 mSv. According to the findings, the regions under study are reasonably safe for human outdoor activities such as agriculture, construction, and factory operations.