Statistical assessment of natural radioactivity, radon activity, and associated radiological exposure due to artisanal mining in Atiwa West district of the Eastern region, Ghana.

The activity concentration of natural radionuclides, radon activity concentration, mass and area exhalation rates have been studied in soils from gold mining communities in Atiwa West district. The natural radionuclides were determined by gamma ray spectrometry method while radon concentrations were measured using CR-39 detectors. The mean activity concentrations were found to be 26.9 ± 1.7 Bq/kg, 57.5 ± 3.6 Bq/kg, 237.5 ± 17.6 Bq/kg and 560.0 ± 54 Bq/m3 for Ra-226, Th-232, K-40 and Rn-222 respectively. The evaluated mass exhalation rates ranged from 2.8 ± 0.3 to 6.5 ± 0.7 × 10-5 Bq/kg/h while the area exhalation rates were from 0.8 ± 0.09 to 2.0 ± 0.21 × 10-3 Bq/m2/h. Some mining and farming areas recorded high exhalation rates indicating that the use of soils as building materials from such areas could pose a level of radiation hazard to the population. The evaluated radiological risks were below reference levels. A good linear correlation was observed between Ra-226 and Rn-222 activity concentrations and in the investigated soils. The Pearson correlation coefficient, cluster analysis and principal component analysis were used to study the relationship between the determined parameters of the study.

Validation of a new sampler for radon gas measurements in surface water.

Radon gas (Rn-222) in water poses health risks due to radiation exposure, yet it's also an important tracer for studying natural systems. Sampling procedures for Rn-222 analysis are very sensitive to potential losses of the gas to the atmosphere. It requires a well-defined and properly validated protocol to ensure accuracy and reliability. A novel sampler was developed to collect surface water from a distance (e.g. from bridges), addressing logistic challenges posed by topography. The sampler, manually operated, ensures precise depth-specific sampling throughout the water column. A three-stage validation process (technical performance test, uncertainty estimations and preliminary test) was followed to validate the protocol.•The comparison of the technical procedure for analysis and measurement through Liquid Scintillation Counting is statistically robust (one-way ANOVA p-value = 0.96).•For the protocol proposed for Rn-222 determination, the estimated sampling and measurement uncertainties (k = 2) are respectively 5% and 15%. These are compatible with the literature and the laboratory's precision.•Preliminary tests, with meaningful patterns identified and possibly related to the river's hydrodynamics, revealed a very reliable protocol, even in low Rn-222 concentrations.Therefore, the sampler has demonstrated a good analytical reproducibility and was considered validated for Rn-222 determination in surface waters.

Evaluation of Indoor Radon Activity Concentrations and Controls in Dwellings Surrounding the Gold Mine Tailings in Gauteng Province of South Africa.

Radon in dwellings is recognized as the primary source of natural radiation exposure to members of the public. In the West Rand District and Soweto in the Gauteng Province (South Africa), indoor radon (222Rn) mapping was carried out to assess the exposure levels of radon in dwellings around gold and uranium mining tailings dams. This study was conducted predominately during warm and cold seasons, using the solid-state nuclear track detectors. In summer months, the indoor radon levels measured in all areas ranged from below the lower limit of detection to 71 Bq/m3, with a mean value of 29 Bq/m3, whereas in winter, the levels ranged between 11 and 124 Bq/m3, with a mean value of 46 Bq/m3. Higher indoor radon levels are found in colder months (winter season) than warmer months (summer season). However, no dwellings with indoor radon levels that exceed the WHO (2009) recommended reference level of 100 Bq/m3 were found, except for one that was constructed directly on soil mixed with tailings material. It is recommended that residents should keep their indoor radon levels low through continuous ventilation so as to minimize the buildup of radon and the likelihood of increased health hazards associated with radon exposure.

Radon and thoron exhalation rate in the soil of Western Haryana, India.

This study reports the exhalation rates of radon and thoron from surface soil collected from 60 rural sites of district Hisar, Haryana, India. The exhalation rates of Rn222 (radon) and Rn220 (thoron) were measured by portable SMART RnDuo (AQTEK SYSTEMS) using a mass accumulation chamber which was equipped with a scintillation material-coated cell. Dose rates due to natural gamma radiations ranged from 0.526 to 1.139 mSv y-1. The Rn222 mass exhalation rate in soil samples varied from 0.14 to 94.65 mBq kg-1 h-1. Thoron surface exhalation rates ranged from 46.42 to 619.88 Bq m-2 h-1. This study gives an idea about the differences in Rn222 and Rn220 exhalation at different locations which may be due to variations in geological features of the locations and characteristics of the topsoil. The findings show that usage of study area soil as building material is safe.

A straightforward approach for assessing the effectiveness of membrane materials as radon (222Rn) barriers.

The ubiquitous presence of the radioisotope radon (222Rn) and its short-lived progeny (218Po, 214Pb, 214Bi, 214Po) is challenging in two respects: (i) Radon is a major issue regarding health-related problems due to potentially elevated radiation exposure of humans in dwellings, and (ii) due to the mobility of radon the short-lived progeny may cause complications in radionuclide detection in laboratories. Polymer membranes are an appropriate means for effectively preventing unwanted radon migration. However, most of the published literature focusses on robust membranes made for the large-scale sealing of dwelling substructures. Membranes that are suitable (at small-scale) for sealing purposes in radionuclide detection applications are only rarely discussed. In this paper, we present a straightforward practical approach that allows the effectiveness of any membrane to be assessed for any purpose related to radon sealing. Executing the approach requires only (i) a suitable container with inlet and outlet ports, (ii) a mobile radon detector, and (iii) any type of radon source material. The approach provides a tool that allows testing any available membrane for its applicability as radon barrier sheeting.

Numerical analysis of two-filter method for continuous measurement of airborne Rn-222.

The two-filter method enables the continuous measurement of airborne Rn-222 via simultaneously sampling and counting. However, the slow time response of the two-filter detector and the overlapping counting data derived from the intervallic data acquisition make the interpretation of measurement results complicated. A valid data analysis to exactly match the series of counting data with the corresponding radon concentrations is desired. In this work, the continuous sampling and counting processes of the two-filter method is depicted numerically and the calculation of radon concentration from the raw counting data is given with detailed formulas. The numerical model is used to quantitatively investigate the influences of several key factors, including the volume of the radon delay chamber (5-10 000 l), the flow rate of air sampling (2.5-1000 l min-1) and the interval time of data acquisition (5-120 min), on the measurement sensitivity and accuracy, which provides an approach for the optimization of the design and measurement settings of a specific two-filter detector in relation to these aspects.

Identification of earthquake precursors in soil radon-222 data of Kutch, Gujarat, India using empirical mode decomposition based Hilbert Huang Transform.

Soil radon (Rn-222) has been continuously monitored at Badargadh station (23.47°N, 70.62°E) in Kutch region of Gujarat to study the pre-seismic anomalies prior to occurrence of local earthquakes. This monitoring site is in close proximity to the South Wagad Fault, a seismically active fault in the study area. The raw data of radon along with meteorological parameters such as temperature, pressure and humidity in soil of this station for the period of January 01 to December 31, 2017 with a sampling interval of 10 min were used in the analysis. The wind speed and rainfall data of the corresponding period were collected from the nearest weather station. From descriptive statistics, we found an average soil radon concentration of 343 Bq.m-3. It is observed that radon has a maximum concentration during the rainy season compared to the other two seasons. We found that radon emission rate is less during mid-nights and early morning, whereas, the radon emission is more during afternoon hours when the sun light intensity is more. In order to identify and extract the periodic oscillations in the radon time series, the Empirical Mode Decomposition (EMD) was applied to the soil radon (Rn-222) time series by decomposing it into different oscillatory modes known as the Intrinsic Mode Function (IMF). Several interesting non-linear features emerged from the analysis after applying Hilbert Huang Transform (HHT) on significant IMFs. The temporal variation of the instantaneous energy is well correlated with four local earthquakes during the study period. Most interestingly, intermittencies in the temporal evolution of the instantaneous energy function have been observed prior to these local earthquakes. We present the results of the seismic and aseismic periods as well as a brief discussion of the analysis of radon data which can be used as a precursor of seismic activity. It is now possible to identify anomalies in radon time series using EMD based HHT method even for small-magnitude earthquakes.

Nitrate loads in sub-tropical headwater streams driven by intensive horticulture.

Nitrogen runoff from fertiliser intensive land uses has become an issue worldwide, contributing to algal blooms, hypoxic waters and aquatic biodiversity losses. This study assessed potential nutrient pollution from blueberry farms in subtropical Australia and examines whether nutrient loads were driven by groundwater discharge and/or surface water runoff. Streams downstream of eight blueberry farms were compared to eight nearby control sites without any blueberry activity. In the 90 day sample period, there were three rain events >90 mm day-1 that produced runoff sufficient to create flooding. Overall, the results revealed a clear link between blueberry farming and nitrogen runoff in headwater streams. While NOX (nitrate + nitrite) was the dominant nitrogen species downstream of blueberry farms, dissolved organic nitrogen (DON) was the dominant species in control sites. The concentrations and loads of NOx were one order of magnitude lower in the eight non-blueberry (6.3 ±â€¯2.0 µmol L-1; 1.6 ±â€¯1.2 kg N-NOX ha-1 yr-1) than the eight blueberry (56.9 ±â€¯14.2 µmol L-1; 21.8 ±â€¯8.0 kg N-NOX ha-1 yr-1) sites. NOX concentrations and loads were highest following rain events. Radon (222Rn, a natural groundwater tracer) observations and low nitrogen concentration in groundwater samples further suggest that surface runoff dominates the delivery of nitrogen to the creeks investigated. NOX concentrations and loads in creeks correlated with blueberry farm density. At >15% of blueberry land use in a catchment, there was a detectable influence in NOX concentrations and loads in the headwater streams. Assuming that our load estimates can be up-scaled to annual nitrogen creek exports, and that local farmers use the recommended amount of fertiliser (121 kg N ha-1 yr-1), between 18 and 25% of the used fertiliser was lost to the creeks. This implies that there are opportunities for decreasing the use of fertilisers in this catchment and managing any nitrogen that escapes to the creeks.

Simulation and experimental measurement of radon activity using a multichannel silicon-based radiation detector.

In this study, high-precision radiation detector (HIPRAD), a new-generation semiconductor microstrip detector, was used for detecting radon (Rn-222) activity. The aim of this study was to detect radon (Rn-222) activity experimentally by measuring the energy of particles in this detector. Count-ADC channel, eta-charge, and dose-response values were experimentally obtained using HIPRAD. The radon simulation in the radiation detector was theoretically performed using the Geant4 software package. The obtained radioactive decay, energy generation, energy values, and efficiency values of the simulation were plotted using the root program. The new-generation radiation detector proved to have 95% reliability according to the obtained dose-response graphs. The experimental and simulation results were found to be compatible with each other and with the radon decays and literature studies.

Bias in the measurement of radon gas using ionization chambers: Application to SIR.

Two main non-destructive techniques can be used to measure standard 222Rn gas ampoules: well-type ionization chambers and gamma-ray spectrometry, the former being used in the Système International de Référence (SIR) for international comparison purposes. The reliability of these techniques requires that the variability of the flame-sealed gas glass ampoules used have a negligible influence on the detector response. This variability is studied in this work by considering three parameters: the volume of the ampoule, the position of the sealing point and the thickness of the glass. Results showed that variability of the gas ampoules induced measurement bias larger than the uncertainty of the standard sources.

Activity measurement of 222Rn gas for a key comparison.

The Korea Research Institute of Standards and Science (KRISS) participated, in 2015, in an international Key Comparison (KC) of gaseous radon-222 activity named CCRI (II) -K2.Rn-222 to confirm international equivalence of KRISS-established gaseous radon-222 measurement standards. LNHB acted as KC pilot laboratory. This paper describes the KC measurement procedure followed at KRISS using the defined solid angle counting method together with auxiliary relative measurement methods and presents the results.

Radioactivity measurements and risk assessments of spa waters in some areas in Turkey.

The current study presents the results of the activity of radionuclides in spa waters, and evaluates their radiological influences on the population consuming these waters in the Central and Eastern Black Sea regions of Turkey. Since these waters are used for therapy and consumption purposes unconsciously, their radiological impact on the people was computed by taking into consideration the annual intake through ingestion of 226Ra, 232Th, 40K, 137Cs and 222Rn. The mean activities were estimated to be 11.35 for gross alpha, 6.23 for gross beta, 2.96 for 226Ra, 0.42 for 232Th, 0.069 for 137Cs, 0.19 for 40K, and 267 Bq L-1 for 222Rn, respectively. The estimated effective doses from spa water were found to be 49.77 µSv a-1 (226Ra), 5.95 µSv a-1 (232Th), 0.07 µSv a-1 (137Cs), 0.83 µSv a-1 (40K) and 56.03 µSv a-1 (222Rn). These values were evaluated and compared with related verified values from literature. Also, physico-chemical characterizations of spa water samples considered in the current study were investigated. This study would be useful for consumers and official authorities for the assessment of radiation exposure risk due to usage of the considered spa waters.

An absolute radon 222 activity measurement system at LNE-LNHB.

A good metrological traceability of radon and progenies is necessary to accurately measure the radon concentration. In 1995, at the LNE-LNHB, J.L. Picolo developed a reference method using a defined-solid-angle (DSA) alpha spectrometer to measure a frozen radon source. With this method it was possible to measure radon standards with a relative standard uncertainty of 0.5%. This paper presents the design and the characterization of a new upgraded measurement system; all parameters and their uncertainties are discussed. This new system allows the measurement of radon sources from 100Bq to 4MBq with a relative standard uncertainty of 0.3%.

A new thoron atmosphere reference measurement system.

A new thoron reference ((220)Rn) in air measurement system is developed at the LNE-LNHB with the collaboration of the IRSN. This measurement system is based on a reference volume with an alpha detector which is able to directly measure thoron and its decay products at atmospheric pressure. In order to improve the spectrum quality of the thoron progenies, we have applied an electric field to catch the decay products on the detector surface. The developed system is a portative device which can be used to measure reference thoron atmosphere such as the BACCARA chamber at IRSN (Picolo et al., 1999). As this system also allows the measurement of radon ((222)Rn) in air, it was validated using the radon primary standards made at the LNE-LNHB. This thoron measurement system will be used, at IRSN, as a reference instrument in order to calibrate the thoron activity concentration in the BACCARA facility.

Unusual Childhood Waking as a Possible Precursor of the 1995 Kobe Earthquake.

Nearly 1,100 young students living in Japan at a range of distances up to 500 km from the 1995 Kobe M7 earthquake were interviewed. A statistically significant abnormal rate of early wakening before the earthquake was found, having exponential decrease with distance and a half value approaching 100 km, but decreasing much slower than from a point source such as an epicentre; instead originating from an extended area of more than 100 km in diameter. Because an improbably high amount of variance is explained, this effect is unlikely to be simply psychological and must reflect another mechanism-perhaps Ultra-Low Frequency (ULF) electromagnetic waves creating anxiety-but probably not (222)Rn excess. Other work reviewed suggests these conclusions may be valid for animals in general, not just children, but would be very difficult to apply for practical earthquake prediction.

Standardization of Rn-222 at the Australian Radiation Laboratory.

The standardization of Rn-222 at the Australian Radiation Laboratory involves the calibration of scintillation cells by two methods using standard Ra-226 solutions traceable to the National Institute of Standards and Technology. One of these methods, namely the injection method, involves direct transfer of Rn-222 into a scintillation cell. In the other method, known as the volumetric method, the Rn-222 is flushed into a large container and the scintillation cell calibrated by sampling from this container. A comparison of the two methods showed that similar results were obtained, with the overall random uncertainty being 3.4% for one standard deviation. Using better estimates of the true calibration factors, the overall random uncertainty was reduced to 1.8% for one standard deviation.