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Using all-optical time-resolved magneto-optical Kerr effect measurements we demonstrate an efficient modulation of the spin-wave (SW) dynamics via the bias magnetic field orientation around nanoscale diamond shaped antidots that are arranged on a square lattice within a [Co(0.75 nm)/Pd(0.9 nm)]8multilayer with perpendicular magnetic anisotropy (PMA). Micromagnetic modeling of the experimental results reveals that the SW modes in the lower frequency regime are related to narrow shell regions around the antidots, where in-plane (IP) domain structures are formed due to the reduced PMA, caused by Ga+ion irradiation during the focused ion beam milling process of antidot fabrication. The IP direction of the shell magnetization undergoes a striking change with magnetic field orientation, leading to the sharp variation of the edge localized (shell) SW modes. Nevertheless, the coupling between such edge localized and bulk SWs for different orientations of bias field in PMA systems gives rise to interesting Physics and attests to new prospects for developing energy efficient and hybrid-system-based next-generation nanoscale magnonic devices.
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Magnetic nanomaterials record information as fast as picoseconds in computer memories but retain it for millions of years in ancient rocks. This exceedingly broad range of times is covered by hopping over a potential energy barrier through temperature, ultrafast optical excitation, mechanical stress, or microwaves. As switching depends on nanoparticle size, shape, orientation, and material properties, only single-nanoparticle studies can eliminate the ensemble heterogeneity. Here, we push the sensitivity of photothermal magnetic circular dichroism down to individual 20 nm magnetite nanoparticles. Single-particle magnetization curves display superparamagnetic to ferromagnetic behaviors, depending on the size, shape, and orientation. Some nanoparticles undergo thermally activated switching on time scales of milliseconds to minutes. Surprisingly, the switching barrier varies with time, leading to dynamical heterogeneity, a phenomenon familiar in protein dynamics and supercooled liquids. Our observations will help to identify the external parameters influencing magnetization switching and, eventually, to control it, an important step for many applications.
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The intricate interplay between light and matter provides effective tools for manipulating topological phenomena. Here, we theoretically propose and computationally show that circularly polarized light holds the potential to transform the axion insulating phase into a quantum anomalous Hall state in MnBi2Te4 thin films, featuring tunable Chern numbers (ranging up to ±2). In particular, we reveal the spatial rearrangement of the hidden layer-resolved anomalous Hall effect under light-driven Floquet engineering. Notably, upon Bi2Te3 layer intercalation, the anomalous Hall conductance predominantly localizes in the nonmagnetic Bi2Te3 layers that hold zero Berry curvature in the intact state, suggesting a significant magnetic proximity effect. Additionally, we estimate variations in the magneto-optical Kerr effect, giving a contactless method for detecting topological transitions. Our work not only presents a strategy to investigate emergent topological phases but also sheds light on the possible applications of the layer Hall effect in topological antiferromagnetic spintronics.
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Recent advances in single-particle photothermal circular dichroism (PT CD) and photothermal magnetic circular dichroism (PT MCD) microscopy have shown strong promise for diverse applications in chirality and magnetism. Photothermal circular dichroism microscopy measures direct differential absorption of left- and right-circularly polarized light by a chiral nanoobject and thus can measure a pure circular dichroism signal, which is free from the contribution of circular birefringence and linear dichroism. Photothermal magnetic circular dichroism, which is based on the polar magneto-optical Kerr effect, can probe the magnetic properties of a single nanoparticle (of sizes down to 20 nm) optically. Single-particle measurements enable studies of the spatiotemporal heterogeneity of magnetism at the nanoscale. Both PT CD and PT MCD have already found applications in chiral plasmonics and magnetic nanomaterials. Most importantly, the advent of these microscopic techniques opens possibilities for many novel applications in biology and nanomaterial science.
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Magnetic topological insulators are a fertile platform for studying the interplay between magnetism and topology. The unique electronic band structure can induce exotic transport and optical properties. However, a comprehensive optical study at both near-infrared and terahertz frequencies has been lacking. Here, we report magneto-optical effects from a heterostructure of a Cr-incorporated topological insulator, CBST. By measuring the magneto-optical Kerr effect, we observe a high temperature ferromagnetic transition (160 K) in the CBST film. We also use time-domain terahertz polarimetry to reveal a terahertz Faraday rotation of 1.5 mrad and a terahertz Kerr rotation of 3.6 mrad at 2 K. The calculated terahertz Hall conductance is 0.42 e2/h. Our work shows the optical responses of an artificially layered magnetic topological insulator, paving the way toward a high-temperature quantum anomalous Hall effect via heterostructure engineering.
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The magneto-optical Kerr effect (MOKE) is a powerful probe of magnetism and has recently gained new attention in antiferromagnetic (AFM) materials. Through extensive first-principles calculations and group theory analysis, we have identified Fe2CX2 (X = F, Cl) and Janus Fe2CFCl monolayers as ideal A-type collinear AFM materials with high magnetic anisotropy and Néel temperatures. By applying a vertical external electrical field (Ef) of 0.2 V/Å, the MOKE is activated for Fe2CF2 and Fe2CCl2 monolayers without changing their magnetic ground state, and the maximum Kerr rotation angles are 0.13 and 0.08°, respectively. Due to the out-of-plane spontaneous polarization, the intrinsic and nonvolatile MOKE is found in the Janus Fe2CFCl monolayer and the maximal Kerr rotation angle without external electronic field is 0.25°. Moreover, the intrinsic built-in electronic field also gives origin to more robust A-type AFM ordering and reversible Kerr angle against external Ef. Our study suggests that Ef is an effective tool for controlling MOKE in two-dimensional (2D) AFM materials. This research opens the possibility of related studies and applications in AFM spintronics.
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The magneto-optical (MO) Kerr effects for ZnO and ZnO:Ni-doped nanolaminate structures prepared using atomic layer deposition (ALD) have been investigated. The chemical composition and corresponding structural and morphological properties were studied using XRD and XPS and compared for both nanostructures. The 2D array gradient maps of microscale variations of the Kerr angle polarization rotation were acquired by means of MO Kerr microscopy. The obtained data revealed complex behavior and broad statistical dispersion and showed distinct qualitative and quantitative differences between the undoped ZnO and ZnO:Ni-doped nanolaminates. The detected magneto-optical response is extensively inhomogeneous in ZnO:Ni films, and a giant Kerr polarization rotation angle reaching up to ~2° was established. This marks the prospects for further development of magneto-optical effects in ALD ZnO modified by transition metal oxide nanostructures.
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The fundamental mechanisms of ultrafast demagnetization and magnetization recovery processes in ferromagnetic materials remain incompletely understood. The investigation of different dynamic features which depend on various physical quantities requires a more systematic approach. Here, the femtosecond laser-induced demagnetization and recovery dynamics in L10-Fe0.5Pt0.5 alloy film are studied by utilizing time-resolved magneto-optical Kerr measurements, focusing on their dependences of excitation fluence and ambient temperature over broad ranges. Ultrafast demagnetization dominated by Elliott-Yafet spin-flip scattering, and two-step magnetization recovery processes are found to be involved in all observations. The fast recovery time corresponding to spin-lattice relaxation is much shorter than that of many ferromagnets and increase with excitation fluence. These can be ascribed to the strong spin-orbit coupling (SOC) demonstrated in FePt and the reduction of transient magnetic anisotropy, respectively. Surprisingly, the demagnetization time exhibits no discernible correlation with ambient temperature. Two competitive factors are proposed to account for this phenomenon. On the other hand, the spin-lattice relaxation accelerates as temperature decreases due to enhanced SOC at lower ambient temperature. A semiquantitative analysis is given to get a visualized understanding. These results offer a comprehensive understanding of the dynamic characteristics of ultrafast demagnetization and recovery processes in iron-based materials with strong SOC, highlighting the potential for regulating the magnetization recovery process through temperature and laser fluence adjustments.
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Thin films of BaM hexaferrite (BaFe12O19) were grown on α-Al2O3(0001) substrates by laser molecular beam epitaxy. Structural, magnetic, and magneto-optical properties were studied using medium-energy ion scattering, energy dispersive X-ray spectroscopy, atomic force microscopy, X-ray diffraction, magneto-optical spectroscopy, and magnetometric techniques, and the dynamics of magnetization by ferromagnetic resonance method. It was shown that even a short time annealing drastically changes the structural and magnetic properties of films. Only annealed films demonstrate magnetic hysteresis loops in PMOKE and VSM experiments. The shape of hysteresis loops depends on thickness of films showing practically rectangular loops and high value of remnant magnetization (Mr/Ms~99%) for thin films (50 nm) and much broader and sloped loops in thick (350-500 nm) films. The magnitude of magnetization 4πMs ≈ 4.3 kG in thin films corresponds to that in bulk BaM hexaferrite. Photon energy and sign of bands in magneto-optical spectra of thin films correspond to ones observed earlier in bulk samples and films of BaM hexaferrite. FMR spectra of 50 nm films at 50 GHz consist of a number of narrow lines. The width of main line ΔH~20 Oe is lower than has been reported up to now.
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We studied the magneto-optical Kerr effect (MOKE) of two-dimensional (2D) heterostructure CrI3/In2Se3/CrI3 using density functional theory calculations and symmetry analysis. The spontaneous polarization in the In2Se3 ferroelectric layer and the antiferromagnetic ordering in CrI3 layers break the mirror and the time-reversal symmetry, thus activating MOKE. We show that the Kerr angle can be reversed by either the polarization or the antiferromagnetic order parameter. Our results suggest that ferroelectric and antiferromagnetic 2D heterostructures could be exploited for ultracompact information storage devices, where the information is encoded by the two ferroelectric or the two time-reversed antiferromagnetic states and the read-out is performed optically by MOKE.
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Introducing magnetism to two-dimensional topological insulators is a central issue in the pursuit of magnetic topological materials in low dimensionality. By means of low-temperature growth at 80 K, we succeeded in fabricating a monolayer stanene on Co/Cu(111) and resolving ferromagnetic spin contrast by field-dependent spin-polarized scanning tunneling microscopy (SP-STM). Increases of both remanence to saturation magnetization ratio (Mr/Ms) and coercive field (Hc) due to an enhanced perpendicular magnetic anisotropy (PMA) are further identified by out-of-plane magneto-optical Kerr effect (MOKE). In addition to ultraflat stanene fully relaxed on bilayer Co/Cu(111) from density functional theory (DFT), characteristic topological properties including an in-plane s-p band inversion and a spin-orbit coupling (SOC) induced gap about 0.25 eV at the ΓÌ point have also been verified in the Sn-projected band structure. Interfacial coupling of single-atomic-layer stanene with ferromagnetic Co biatomic layers allows topological band features to coexist with ferromagnetism, facilitating a conceptual design of atomically thin magnetic topological heterostructures.
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Following the demonstration of laser-induced ultrafast demagnetization in ferromagnetic nickel, several theoretical and phenomenological propositions have sought to uncover its underlying physics. In this work we revisit the three temperature model (3TM) and the microscopic three temperature model (M3TM) to perform a comparative analysis of ultrafast demagnetization in 20 nm thick cobalt, nickel and permalloy thin films measured using an all-optical pump-probe technique. In addition to the ultrafast dynamics at the femtosecond timescales, the nanosecond magnetization precession and damping are recorded at various pump excitation fluences revealing a fluence-dependent enhancement in both the demagnetization times and the damping factors. We confirm that the Curie temperature to magnetic moment ratio of a given system acts as a figure of merit for the demagnetization time, while the demagnetization times and damping factors show an apparent sensitivity to the density of states at the Fermi level for a given system. Further, from numerical simulations of the ultrafast demagnetization based on both the 3TM and the M3TM, we extract the reservoir coupling parameters that best reproduce the experimental data and estimate the value of the spin flip scattering probability for each system. We discuss how the fluence-dependence of inter-reservoir coupling parameters so extracted may reflect a role played by nonthermal electrons in the magnetization dynamics at low laser fluences.
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The weak magneto-optical (MO) signal of traditional MO materials is indeed an important issue for their further practical applications. Although many strategies have been proposed to improve the MO effect, hybridization with noble metal nanostructures is a promising route in recent years due to the high localized-surface plasmon resonances (LSPR) effect. A new magneto-optical surface plasmon resonance (MOSPR) structure hybrid with Au bowtie arrays is proposed to increase the measuring range of the polar magneto-optical Kerr effect (PMOKE) and the quality factor through the LSPR effect. It is verified by a numerical simulation of the finite element method (FEM). The optimized parameters were found by modulating the shape and geometric dimensions. Owing to the significant LSPR from the Au bowties, a PMOKE amplification signal spectrum with narrow linewidth, and a high amplitude with high-sensing performance was achieved. Compared with the bare magnetic film alone, by optimizing the relevant parameters of the LSPR structure, the maximum signal increases 3255 times, and the quality factor can be greatly improved, which would provide important guidance and help for the practical application of MO devices.
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Superdiffusive spin transport has been proposed as a new mechanism of ultrafast demagnetization in layered magnetic nanostructures and demonstrated experimentally. However, it is unknown if it is possible for phonon transport to occur and manipulate ultrafast demagnetization. Here, we explore the ultrafast dynamics of demagnetization of an antiferromagnet/ferromagnet bilayer nanostructure, of a FeMn/MnGa bilayer film prepared by molecular beam epitaxy. Ultrafast dynamics of a two-step demagnetization were observed through the time-resolved magneto-optical Kerr effect. The first-step fast component of the two-step demagnetization occurred within ~200 fs, while the second-step slow component emerged in a few tens of picoseconds. For a single MnGa film, only the ultrafast dynamics of the first-step fast demagnetization were observed, revealing that the second-step slow demagnetization originates from interlayer phonon transport. A four-temperature model considering phonon transport was developed and used to effectively reproduce the observed ultrafast dynamics of two-step demagnetization. Our results reveal the effect of phonon transport on demagnetization for the first time and open up a new route to manipulate ultrafast demagnetization in layered magnetic structures.
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A series of Pd1- x Fe x alloy epitaxial films (x = 0, 0.038, 0.062, and 0.080), a material promising for superconducting spintronics, was prepared and studied with ultrafast optical and magneto-optical laser spectroscopy in a wide temperature range of 4-300 K. It was found that the transition to the ferromagnetic state causes a qualitative change of both the reflectivity and the magneto-optical Kerr effect transients. A nanoscale magnetic inhomogeneity of the ferromagnet/paramagnet type inherent in the palladium-rich Pd1- x Fe x alloys reveals itself through the occurrence of a relatively slow, 10-25 ps, photoinduced demagnetization component following a subpicosecond one; the former vanishes at low temperatures only in the x = 0.080 sample. We argue that the 10 ps timescale demagnetization originates most probably from the diffusive transport of d electrons under the condition of nanoscale magnetic inhomogeneities. The low-temperature fraction of the residual paramagnetic phase can be deduced from the magnitude of the slow reflectivity relaxation component. It is estimated as ≈30% for x = 0.038 and ≈15% for x = 0.062 films. The minimal iron content ensuring the magnetic homogeneity of the ferromagnetic state in the Pd1- x Fe x alloy at low temperatures is about 7-8 atom %.
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Deep insights into microstructures and domain wall behaviors in the evaluation of different material statuses under elastic and plastic stress ranges have essential implications for magnetic sensing and nondestructive testing and evaluation (NDT&E). This paper investigates the repeatability and stability of residual magnetic field (RMF) signals using a magneto-optical Kerr effect microscope for the stress characterization of silicon steel sheets beyond their elastic limit. Real-time domain motion is used for RMF characterization, while both the repeatability under plastic ranges after the cyclic stress rounds and stability during relaxation time are studied in detail. The distinction between elastic and plastic materials is discussed in terms of their spatio-temporal properties for further residual stress measurement since both ranges are mixed. During the relaxation time, the RMF of the plastic material shows a two-stage change with apparent recovery, which is contrasted with the one-stage change in the elastic material. Results show that the grain boundary affects the temporal recovery of the RMF. These findings concerning the spatio-temporal properties of different RMFs in plastic and elastic materials can be applied to the design and development of magnetic NDT&E for (residual) stress measurement and material status estimation.
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Ultrafast demagnetization in diverse materials has sparked immense research activities due to its captivating richness and contested underlying mechanisms. Among these, the two most celebrated mechanisms have been the spin-flip scattering (SFS) and spin transport (ST) of optically excited carriers. In this work, we have investigated femtosecond laser-induced ultrafast demagnetization in perpendicular magnetic anisotropy-based synthetic antiferromagnets (p-SAFs) where [Co/Pt]n-1/Co multilayer blocks are separated by Ru or Ir spacers. Our investigation conclusively shows that the ST of optically excited carriers can have a significant contribution to the ultrafast demagnetization in addition to SFS processes. Moreover, we have also achieved an active control over the individual mechanisms by specially designing the SAF samples and altering the external magnetic field and excitation fluence. Our study provides a vital understanding of the underlying mechanism of ultrafast demagnetization in synthetic antiferromagnets, which will be crucial in future research and applications of antiferromagnetic spintronics.
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The magnetic properties and the atomic scale morphology of bimetallic two-dimensional nanoislands, epitaxially grown on fcc(111) metal surfaces, have been studied by means of Magneto-Optical Kerr Effect and Scanning Tunneling Microscopy. We investigate the effect on blocking temperature of one-dimensional interlines appearing in core-shell structures, of two-dimensional interfaces created by capping, and of random alloying. The islands are grown on Pt(111) and contain a Co-core, surrounded by Ag, Rh, and Pd shells, or capped by Pd. The largest effect is obtained by Pd capping, increasing the blocking temperature by a factor of three compared to pure Co islands. In addition, for Co-core Fe-shell and Co-core FexCo1-x-shell islands, self-assembled into well ordered superlattices on Au(11,12,12) vicinal surfaces, we find a strong enhancement of the blocking temperature compared to pure Co islands of the same size. These ultra-high-density (15 Tdots/in2) superlattices of CoFe nanodots, only 500 atoms in size, have blocking temperature exceeding 100 K. Our findings open new possibilities to tailor the magnetic properties of nanoislands.
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We study how to enhance the transverse magneto-optical Kerr effect (TMOKE) of ultra-thin magnetic dielectric films through the excitation of strong magnetic resonances on metasurface with a metal nanowire array stacked above a metal substrate with an ultra-thin magnetic dielectric film spacer. The plasmonic hybridizations between the Au nanowires and substrate result in magnetic resonances. The periodic arrangement of the Au nanowires can excite propagating surface plasmon polaritons (SPPs) on the metal surface. When the SPPs and the magnetic resonances hybridize, they can strongly couple to form two strong magnetic resonances, which are explained by a coupled oscillator model. Importantly, benefitting from the strong magnetic resonances, we can achieve a large TMOKE signal up to 26% in the ultra-thin magnetic dielectric film with a thickness of only 30 nm, which may find potential applications in nanophotonics, magnonics, and spintronics.
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Anti-perovskite transition metal nitrides exhibit a variety of magnetic properties-such as ferromagnetic, ferrimagnetic, and paramagnetic-depending on the 3dtransition metal. Fe4N and Co4N are ferromagnetic at room temperature (RT), and the minority spins play a dominant role in the electrical transport properties. However, Mn4N is ferrimagnetic at RT and exhibits a perpendicular magnetic anisotropy caused by tensile strain. Around the magnetic compensation in Mn4N induced by impurity doping, researchers have demonstrated ultrafast current-induced domain wall motion reaching 3000 m s-1at RT, making switching energies lower and switching speed higher compared with Mn4N. In this review article, we start with individual magnetic nitrides-such as Fe4N, Co4N, Ni4N, and Mn4N; describe the nitrides' features; and then discuss compounds such as Fe4-xAxN (A = Co, Ni, and Mn) and Mn4-xBxN (B = Ni, Co, and Fe) to evaluate nitride properties from the standpoint of spintronics applications. We pay particular attention to preferential sites of A and B atoms in these compounds, based on x-ray absorption spectroscopy and x-ray magnetic circular dichroism.
