Human health impacts attributable to inhalation exposure of particulate matter (PM10 and PM2.5) during the Holi festival.

OBJECTIVE: The present study focuses on residential areas of Delhi to identify the elevated levels of ambient PM10 and PM2.5 due to biomass burning followed by the coloring activity in the Holi festival celebrated at the end of the winter season. This study also focuses on the health risk assessment and mortality among different age groups due to the change in particulate matter levels during the Holi festival in Delhi, India. MATERIALS AND METHODS: Secondary data of particulate matters have been procured from the Central Pollution Control Board (CPCB), Delhi Pollution Control Committee (DPCC), and Indian Institute of Tropical Meteorology (IITM), Pune for the period of the pre-, during, and post-Holi period for the year 2018-2020 at four selected residential locations in Delhi, India. The health impacts of particle inhalation were quantified using the AirQ + models. RESULTS: The results indicated the levels of PM10 and PM2.5 rise about 3-4 times higher during the Holi festival than on normal days, resulting in health risks and causing an excess number of mortality and Asthma cases in Delhi. Such cases were also found to be higher in 2018, followed by 2019 and 2020 at all the selected locations in Delhi. CONCLUSIONS: The study linked the increasing particulate levels in the Holi festival with the increased health risk through short-term exposure of the population. The excess number of cases (ENCs) of mortality, all causes of mortality among adults (age > 30 years) associated with short-term exposure to particulate were also identified.

Profile of atmospheric particulate PAHs near busy roadway in tropical megacity, India.

Objective: This study focuses on the profile of ambient particulate polycyclic aromatic hydrocarbons (PAHs), their seasonal distribution, source identification and human health risk assessment due to inhalation exposure of ambient PAHs in Delhi, India.Materials and Methods: Two sampling sites were chosen, one at roadway (MH) and other at urban background (JNU) site in Delhi. Determination of PAHs was carried with the help of HPLC with UV detector. Principal component analysis and Molecular diagnostic ratios were used for the source apportionment of PAHs. Health risks associated with inhalation of particulate PAHs were assessed using benzo(a)pyrene equivalent concentration and incremental lifetime cancer risk (ILCR) approach.Results: The results showed that the average mass concentration of Σ16 PAHs near roadway (67.8 ± 40.2 ng m-3) is significantly higher than urban background site (56 ± 30 ng m-3). Moreover, source apportionment study indicated that major PAH-emission sources in Delhi NCR are traffic and coal combustion. ILCR values at both the sites fall in the range of 10-2-10-4 that corresponds to the priority risk level (10-3) and higher than the acceptable risk level (10-6).conclusions: The high PAHs concentration at MH site was due to it's nearness to busy traffic area. Thus, the spatial variations in PAHs were influenced by local emission sources. The high PAHs level during the winter season can be due to their higher emissions from local heating sources, shift of gas/particle partitioning toward the particulate phase at low temperature and reduced photochemical degradation of some PAHs in winter. The low level of PAHs in monsoon season can be attributed to their wet scavenging and higher percentage in vapor phase. PCA showed that the emissions from vehicles predominate at MH site; whereas, coal combustion and traffic both are the significant PAHs sources at JNU site. Health risk assessment revealed that the highest exposure risks occur at busy traffic site, thereby indicating a significantly higher health risk to the population of Delhi.

Impact of crop residue burning in Haryana on the air quality of Delhi, India.

Crop residue burning (CRB) over northern India is a major air quality and human health issue. The present study assesses the impact of PM10, PM2.5, NO2 and SO2, emitted during CRB activities in Haryana on the air quality of Delhi. The transition from pre-burning to burning period, in both rabi and kharif seasons, shows considerable increase in pollutant concentrations. PM10 and PM2.5 concentrations exceeded NAAQS limits by 2-3 times, while NO2 and SO2 stayed within the limits. MODIS fire observations used to estimate CRB fire counts (confidence ≥80%) shows that rabi (burning period) fires in Haryana are ~3 times higher and more intense than in kharif. Furthermore, backward trajectories shows air mass movement from Haryana, Punjab and Pakistan. Thus, pollutants emitted reach Delhi via air masses, deteriorating its air quality. Meteorological conditions influence pollutant concentrations during both seasons. Frequent dust storms in rabi, and Dusshera and Diwali firework celebrations in kharif season exacerbate air pollution. In rabi, PM10 and PM2.5 have a significant negative association with (relative humidity) RH and positive association with (air temperature) AT. High AT during pre-monsoon, accompanied by low RH, loosens up soil particles and they can easily disperse. Stronger winds in rabi season promote NO2 and SO2 dispersion. In kharif, lower AT, higher RH and slower winds exist. Both PM10 and PM2.5 have a negative association with AT and (wind speed) WS. With lower temperature and slower winds during winter, pollutants are trapped within the boundary layer and are unable to disperse. As expected, NO2 has a significant negative association with AT in Haryana. However, in case of Delhi, the association is significant but positive, and could be due to the odd-even scheme imposed by the Delhi government. More research is needed to determine the health effects of Haryana's rabi CRB activities on Delhi.

Water-insoluble carbonaceous components in rainwater over an urban background location in Northern India during pre-monsoon and monsoon seasons.

The carbonaceous content of rainwater was investigated in samples collected at an urban background site in northern India. Sampling was performed on an event basis during two seasons: pre-monsoon (PM) and monsoon (MN) season covering May-June and July-August, respectively, in 2016. The concentrations of different fractions of water-insoluble organic carbon (WIOC) and elemental carbon (EC) were precisely determined, and the sources of WIOC and EC were also analysed. The result revealed that the average WIOC and EC concentration in rainwater ranged from 0.4 to 52 mgC/L and from 0.1 to 15.3 mgC/L, respectively. The concentrations of WIOC and EC were found to be ~ 9 times and ~ 12 times higher, respectively, in the PM season than MN season. The WIOC/EC ratio indicated higher variation in PM season as compared to that of the MN season, suggesting divergent emission sources during the PM season. The formation of water-insoluble secondary organic carbon (WISOC) has also been identified as one of the causes for the extensive difference in the WIOC/EC ratio in different seasons. Results showed that the WIOC and its fractions were efficiently scavenged through rain. While EC and its fractions were less significantly scavenged, due to its hydrophobicity and fine size. The atmospheric scavenging coefficients of selected carbonaceous components were found significantly correlated with rain intensity (RI) during both the seasons. Higher rain intensity caused greater rates of carbonaceous component wash-out and decreasing concentrations of carbonaceous components in the rain.

Investigation of Forest Fire Activity Changes Over the Central India Domain Using Satellite Observations During 2001-2020.

Recurrent and large forest fires negatively impact ecosystem, air quality, and human health. Moderate Resolution Imaging Spectroradiometer fire product is used to identify forest fires over central India domain, an extremely fire prone region. The study finds that from 2001 to 2020, ∼70% of yearly forest fires over the region occurred during March (1,857.5 counts/month) and April (922.8 counts/month). Some years such as 2009, 2012, and 2017 show anomalously high forest fires. The role of persistent warmer temperatures and multiple climate extremes in increasing forest fire activity over central India is comprehensively investigated. Warmer period from 2006 to 2020 showed doubling and tripling of forest fire activity during forest fire (February-June; FMAMJ) and non-fire (July-January; JASONDJ) seasons, respectively. From 2015 JASONDJ to 2018 FMAMJ, central India experienced a severe heatwave, a rare drought and an extremely strong El Niño, the combined effect of which is linked to increased forest fires. Further, the study assesses quinquennial spatiotemporal changes in forest fire characteristics such as fire count density and average fire intensity. Deciduous forests of Jagdalpur-Gadchiroli Range and Indravati National Park in Chhattisgarh state are particularly fire prone (>61 fire counts/grid) during FMAMJ and many forest fires are of high intensity (>45 MW). Statistical associations link high near surface air temperature and low precipitation during FMAMJ to significantly high soil temperature, low soil moisture content, low evapotranspiration and low normalized difference vegetation index. This creates a significantly drier environment, conducive for high forest fire activity in the region.