First order phase transition in the frustrated triangular antiferromagnet CsNiCl3.

ABSTRACT

By means of high-resolution ultrasonic velocity measurements, as a function of temperature and magnetic field, the nature of the different low temperatures magnetic phase transitions observed for the quasi-one-dimensional compound CsNiCl3 is established. Special attention has been devoted to the field-induced 120 degrees phase transition above the multicritical point in the H-T phase diagram where the elastic constant C44 reveals a steplike variation and hysteresis effects. These results represent the first experimental evidence that the 120 degrees phase transition is weakly first order and contradict the popular notion of new universality classes for chiral systems.