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Synergetic effect of H+ adsorption and ethylene functional groups of covalent organic frameworks on the CO2 photoreduction in aqueous solution.
Zhou, Jie; Cui, Jin-Xian; Dong, Man; Sun, Chun-Yi; You, Si-Qi; Wang, Xin-Long; Zhou, Zi-Yan; Su, Zhong-Min.
Afiliación
  • Zhou J; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn.
  • Cui JX; School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo, Shandong 255049, China. zyzhou@sdut.edu.cn.
  • Dong M; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn.
  • Sun CY; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn.
  • You SQ; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn.
  • Wang XL; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn.
  • Zhou ZY; School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo, Shandong 255049, China. zyzhou@sdut.edu.cn.
  • Su ZM; National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education Department of Chemistry, Northeast Normal University Changchun, Jilin, 130024, P. R. China. suncy009@nenu.edu.cn wangxl824@nenu.edu.cn and Jilin Provincial Scien
Chem Commun (Camb) ; 56(53): 7261-7264, 2020 Jul 02.
Article en En | MEDLINE | ID: mdl-32469023
We prepare a novel COF for CO2 photoreduction with 99.9% CO selectivity in aqueous solution without a cocatalyst. DFT shows that the preferential adsorption of H+ on the COF results in increased CO2 adsorption energy providing an anchoring site of CO2, and with the cooperation of an ethylene group, CO2 reduction is triggered.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2020 Tipo del documento: Article
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2020 Tipo del documento: Article