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D-A-Type Molecules with Free Rotors for Highly Efficient Interfacial Solar-Driven Steam Generation and Thermoelectric Performance.
Wang, Danfeng; Qi, Shuo; Dong, Jingwen; Wang, Xin; Zhang, Yan; Zhou, Shiyuan; Gu, Peiyang; Jia, Tao; Zhang, Qichun.
Afiliación
  • Wang D; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Qi S; Key Laboratory of Forest Plant Ecology, Ministry of Education, Engineering Research Center of Forest Bio-preparation, Heilongjiang Province Key Laboratory of Ecology Utilization of Forestry Based Active Substances, College of Chemistry, Chemical Engineering and Resource Utilization, Northeast Forest
  • Dong J; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Wang X; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Zhang Y; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Zhou S; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Gu P; Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China.
  • Jia T; Key Laboratory of Forest Plant Ecology, Ministry of Education, Engineering Research Center of Forest Bio-preparation, Heilongjiang Province Key Laboratory of Ecology Utilization of Forestry Based Active Substances, College of Chemistry, Chemical Engineering and Resource Utilization, Northeast Forest
  • Zhang Q; Department of Materials Science and Engineering, Department of Chemistry, and Center Of Super-Diamond and Advanced Films (COSDAF), City University of Hong Kong, 83 Tat Chee Avenue, Hong Kong, SAR 999077, P. R. China.
Org Lett ; 25(31): 5730-5734, 2023 Aug 11.
Article en En | MEDLINE | ID: mdl-37470402
ABSTRACT
Three "π"-shaped D-A-type thiodiazoloquinoxaline derivatives with different electronic structures and rotations have been prepared. Their particular structures allow these molecules to possess a broad absorption range and sufficient intramolecular motions, dissipating energy through a thermal deactivation pathway. Among the three materials, TPA-TQN showed the best steam generation efficiency (84.52%) and water-electricity cogeneration efficiency (63.95%). This study suggests that D-A structures with different electronic configurations, free rotors, and hydrophilicities make great contributions to the overall solar energy conversion performances.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Org Lett Asunto de la revista: BIOQUIMICA Año: 2023 Tipo del documento: Article País de afiliación: China
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Org Lett Asunto de la revista: BIOQUIMICA Año: 2023 Tipo del documento: Article País de afiliación: China