Strong Terahertz Third-Harmonic Generation by Kinetic Heavy Quasiparticles in CaRuO_{3}.
Phys Rev Lett
; 132(19): 196501, 2024 May 10.
Article
en En
| MEDLINE
| ID: mdl-38804953
ABSTRACT
We report on time-resolved nonlinear terahertz spectroscopy of a strongly correlated ruthenate, CaRuO_{3}, as a function of temperature, frequency, and terahertz field strength. Third-harmonic radiation for frequencies up to 2.1 THz is observed evidently at low temperatures below 80 K, where the low-frequency linear dynamical response deviates from the Drude model and a coherent heavy quasiparticle band emerges by strong correlations associated with the Hund's coupling. Phenomenologically, by taking an experimentally observed frequency-dependent scattering rate, the deviation of the field driven kinetics from the Drude behavior is reconciled in a time-dependent Boltzmann description, which allows an attribution of the observed third-harmonic generation to the terahertz field driven nonlinear kinetics of the heavy quasiparticles.
Texto completo:
1
Colección:
01-internacional
Base de datos:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Año:
2024
Tipo del documento:
Article
País de afiliación:
Alemania