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Dramatic improvement in the "Bulk" hyperpolarization of 131Xe via spin exchange optical pumping probed using in situ low-field NMR.
Molway, Michael J; Bales-Shaffer, Liana; Ranta, Kaili; Ball, James; Sparling, Eleanor; Prince, Mia; Cocking, Daniel; Basler, Dustin; Murphy, Megan; Kidd, Bryce E; Gafar, Abdulbasit Tobi; Porter, Justin; Albin, Kierstyn; Rosen, Matthew S; Chekmenev, Eduard Y; Michael Snow, W; Barlow, Michael J; Goodson, Boyd M.
Afiliação
  • Molway MJ; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Bales-Shaffer L; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Ranta K; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Ball J; School of Medicine, University of Nottingham, Queens Medical Centre, Nottingham, UK.
  • Sparling E; School of Medicine, University of Nottingham, Queens Medical Centre, Nottingham, UK.
  • Prince M; School of Medicine, University of Nottingham, Queens Medical Centre, Nottingham, UK.
  • Cocking D; School of Medicine, University of Nottingham, Queens Medical Centre, Nottingham, UK.
  • Basler D; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Murphy M; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Kidd BE; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Gafar AT; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Porter J; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Albin K; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA.
  • Rosen MS; A.A. Martinos Center for Biomedical Imaging, Massachusetts General Hospital and Harvard Medical School, Boston 02129, MA, USA; Department of Physics, Harvard University, Cambridge 02138, MA, USA.
  • Chekmenev EY; Department of Chemistry, Integrative Biosciences (Ibio), Karmanos Cancer Institute (KCI), Wayne State University, Detroit 48202, MI, USA; Russian Academy of Sciences, Leninskiy Prospekt 14, 119991 Moscow, Russia.
  • Michael Snow W; Department of Physics, Indiana University, Bloomington, IN, USA.
  • Barlow MJ; School of Medicine, University of Nottingham, Queens Medical Centre, Nottingham, UK.
  • Goodson BM; School of Chemical and Biomolecular Sciences, Southern Illinois University, Carbondale 62901, IL, USA. Electronic address: bgoodson@chem.siu.edu.
J Magn Reson ; 354: 107521, 2023 Sep.
Article em En | MEDLINE | ID: mdl-37487304
ABSTRACT
We report on hyperpolarization of quadrupolar (I=3/2) 131Xe via spin-exchange optical pumping. Observations of the 131Xe polarization dynamics via in situ low-field NMR show that the estimated alkali-metal/131Xe spin-exchange rates can be large enough to compete with 131Xe spin relaxation. 131Xe polarization up to 7.6±1.5% was achieved in ∼8.5×1020 spins-a ∼100-fold improvement in the total spin angular momentum-potentially enabling various applications, including measurement of spin-dependent neutron-131Xe s-wave scattering; sensitive searches for time-reversal violation in neutron-131Xe interactions beyond the Standard Model; and surface-sensitive pulmonary MRI.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: J Magn Reson Assunto da revista: DIAGNOSTICO POR IMAGEM Ano de publicação: 2023 Tipo de documento: Article País de afiliação: Estados Unidos
Texto completo
Adicionar na Minha BVS
Imprimir
XML
PubMed Links
Buscar no Google

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: J Magn Reson Assunto da revista: DIAGNOSTICO POR IMAGEM Ano de publicação: 2023 Tipo de documento: Article País de afiliação: Estados Unidos