ABSTRACT
The present work reports an analysis of the production yield of residues from the 6Li ï¼ 181Ta reaction in a low-energy regime. The experimental yield of 183gOs, 183mOs, 182Os, 183Re, 183Ta, 182m2Ta, and 180Ta have been measured in the 27-43 MeV energy window and compared with equilibrium and pre-equilibrium model calculations under the framework of the nuclear reaction model code, EMPIRE-3.2.2. The maximum yield measured for 183gOs is 80.5 ± 14.9 MBq/C at 40.2 MeV energy in a 2.3 mg/cm2 thick Ta target corresponding to a cross-section of 360.1 ± 34.4 mb from the 181Ta(6Li,4n)183Os reaction and that for 183Re is 1.36 ± 0.4 MBq/C at 42.75 MeV in a 2.4 mg/cm2 thick target. The model estimations agree well with the experimental yields of 183gOs and 183Re. The possible production of stable residues has been estimated using the model-predicted cross-section in the studied energy range. A comparison of production yields of 183m,gOs from 6Li- and 7Li-induced reaction on Ta demonstrates the 6Li reaction as a better candidate. Thick target yields have been evaluated for Os and Re isotopes.
ABSTRACT
Excitation functions of the Tnati(p,x)S43,47c, V48 and Cnatu(p,x)64Cu, Z62,65n reactions were measured in the energy range of 8.8-18.4 MeV by using the stacked-foil activation technique and off-line gamma spectroscopy. The irradiation was carried out at the superconducting linac of the Institute of Modern Physics, Chinese Academy of Sciences. Besides, the reliability and effectiveness of theoretical data from the TALYS code, recommended data of the International Atomic Energy Agency (IAEA) and evaluated nuclear data of the ENDF/B-VIII.0, JENDL-4.0/HE and PADF-2007 libraries were evaluated and verified by comparing with experimental data. Our experimental results agree with most of the available literature data. TALYS-1.95 code could not reproduce, in most cases, the experimental data. Evaluated nuclear data from the ENDF/B-VIII.0, JENDL-4.0/HE and PADF-2007 libraries are able to reproduce, in most cases, the experimental data trend. Recommended data of the IAEA are in good consistent with our work and most of the available literature data.