Supercapacitance and superinductance of TiN and NbTiN films in the vicinity of superconductor-to-insulator transition.

We investigate the low-temperature complex impedance of disordered insulating thin TiN and NbTiN films in the frequency region 400 Hz-1 MHz in close proximity to the superconductor-insulator transition (SIT). The frequency, temperature, and magnetic field dependencies of the real and imaginary parts of the impedance indicate that in full accord with the theoretical predictions and earlier observations, the films acquire self-induced electronic granularity and become effectively random arrays of superconducting granules coupled via Josephson links. Accordingly, the inductive component of the response is due to superconducting droplets, while the capacitive component results from the effective Josephson junctions capacitances. The impedance crosses over from capacitive to inductive behavior as films go across the transition.

Imaging quantum fluctuations near criticality.

A quantum phase transition (QPT) occurs between two competing phases of matter at zero temperature, driven by quantum fluctuations. Though the presence of these fluctuations is well established, they have not been locally imaged in space and their local dynamics has not been studied so far. We use a scanning superconducting quantum interference device to image quantum fluctuations in the vicinity of the QPT from a superconductor to an insulator. We find fluctuations of the diamagnetic response in both space and time that survive well below the transition temperature, demonstrating their quantum nature. The fluctuations appear as telegraph-like noise with a range of characteristic times and a non-monotonic temperature dependence, revealing unexpected quantum granularity. The lateral dimension of these fluctuations grows towards criticality, offering a new measurable length scale. Our results provide physical insight about the reorganization of phases across a QPT, with implications for any theoretical description. This paves a new route for future quantum information applications.

Quantum contributions to the magnetoconductivity of critically disordered superconducting TiN films.

The onset of superconductivity in the presence of disorder is a fundamental problem of condensed matter physics. Here we investigate the magnetoconductance of disordered ([Formula: see text]) superconducting TiN films above the critical temperature T c. We show that the magnetoconductivity of moderately disordered films with [Formula: see text] is in full agreement with the perturbative theory of quantum contributions to conductivity. We demonstrate that the magnetoconductivity of films with [Formula: see text] is also in agreement with the perturbative theory down to temperatures [Formula: see text]. The quantitative discrepancy between experiment and theory develops only below temperatures [Formula: see text] for films with [Formula: see text]. This discrepancy can be eliminated if we assume steeper temperature dependence of the Larkin's electron-electron attraction strength, [Formula: see text]. The obtained temperature dependence of electron phase breaking time [Formula: see text] is in agreement with theoretical predictions for all samples.

Electronic transport in two-dimensional high dielectric constant nanosystems.

There has been remarkable recent progress in engineering high-dielectric constant two dimensional (2D) materials, which are being actively pursued for applications in nanoelectronics in capacitor and memory devices, energy storage, and high-frequency modulation in communication devices. Yet many of the unique properties of these systems are poorly understood and remain unexplored. Here we report a numerical study of hopping conductivity of the lateral network of capacitors, which models two-dimensional insulators, and demonstrate that 2D long-range Coulomb interactions lead to peculiar size effects. We find that the characteristic energy governing electronic transport scales logarithmically with either system size or electrostatic screening length depending on which one is shorter. Our results are relevant well beyond their immediate context, explaining, for example, recent experimental observations of logarithmic size dependence of electric conductivity of thin superconducting films in the critical vicinity of superconductor-insulator transition where a giant dielectric constant develops. Our findings mark a radical departure from the orthodox view of conductivity in 2D systems as a local characteristic of materials and establish its macroscopic global character as a generic property of high-dielectric constant 2D nanomaterials.

Magnetic field-induced dissipation-free state in superconducting nanostructures.

A superconductor in a magnetic field acquires a finite electrical resistance caused by vortex motion. A quest to immobilize vortices and recover zero resistance at high fields made intense studies of vortex pinning one of the mainstreams of superconducting research. Yet, the decades of efforts resulted in a realization that even promising nanostructures, utilizing vortex matching, cannot withstand high vortex density at large magnetic fields. Here, we report a giant reentrance of vortex pinning induced by increasing magnetic field in a W-based nanowire and a TiN-perforated film densely populated with vortices. We find an extended range of zero resistance with vortex motion arrested by self-induced collective traps. The latter emerge due to order parameter suppression by vortices confined in narrow constrictions by surface superconductivity. Our findings show that geometric restrictions can radically change magnetic properties of superconductors and reverse detrimental effects of magnetic field.

Stimulation of the fluctuation superconductivity by PT symmetry.

We discuss fluctuations near the second-order phase transition where the free energy has an additional non-Hermitian term. The spectrum of the fluctuations changes when the odd-parity potential amplitude exceeds the critical value corresponding to the PT-symmetry breakdown in the topological structure of the Hilbert space of the effective non-Hermitian Hamiltonian. We calculate the fluctuation contribution to the differential resistance of a superconducting weak link and find the manifestation of the PT-symmetry breaking in its temperature evolution. We successfully validate our theory by carrying out measurements of far from equilibrium transport in mesoscale-patterned superconducting wires.

Out-of-equilibrium heating of electron liquid: fermionic and bosonic temperatures.

We investigate out-of-the equilibrium properties of the electron liquid in a two-dimensional disordered superconductor subject to the electric bias and temperature gradient. We calculate kinetic coefficients and Nyquist noise, and find that they are characterized by distinct effective temperatures: Te, characterizing single-particle excitations, TCp, describing the Cooper pairs, and Teh, corresponding to electron-hole or dipole excitations. Varying the ratio between the electric j and thermal jth currents and boundary conditions one can heat different kinds of excitations tuning their corresponding temperatures. We propose the experiment to determine these effective temperatures.

Hierarchical energy relaxation in mesoscopic tunnel junctions: effect of a nonequilibrium environment on low-temperature transport.

We develop a theory of far from the equilibrium transport in arrays of tunnel junctions. We find that if the rate of the electron-electron interactions exceeds the rate of the electron-phonon energy exchange, the energy relaxation ensuring the charge transfer may occur sequentially. In particular, cotunneling transport in arrays of junctions is dominated by the relaxation via the intermediate bosonic environment, the electron-hole excitations, rather than by the electron-phonon mechanism. The current-voltage characteristics are highly sensitive to the spectrum of the environmental modes and to the applied bias, which sets the lower bound for the effective temperature. We demonstrate that the energy gap in the electron-hole spectrum which opens below some critical temperature T* due to long-range Coulomb interactions gives rise to the suppression of the tunneling current.

Disorder-induced inhomogeneities of the superconducting state close to the superconductor-insulator transition.

Scanning tunneling spectroscopy at very low temperatures on homogeneously disordered superconducting titanium nitride thin films reveals strong spatial inhomogeneities of the superconducting gap Delta in the density of states. Upon increasing disorder, we observe suppression of the superconducting critical temperature Tc towards zero, enhancement of spatial fluctuations in Delta, and growth of the Delta/Tc ratio. These findings suggest that local superconductivity survives across the disorder-driven superconductor-insulator transition.

Collective Cooper-pair transport in the insulating state of Josephson-junction arrays.

We investigate collective Cooper-pair transport of one- and two-dimensional Josephson-junction arrays. We derive an analytical expression for the current-voltage characteristic revealing thermally activated conductivity at small voltages and threshold voltage depinning. The activation energy and the related depinning voltage represent a dynamic Coulomb barrier for collective charge transfer over the whole system and scale with the system size. We show that both quantities are nonmonotonic functions of the magnetic field. We propose that formation of the dynamic Coulomb barrier and its size scaling are consequences of the mutual Josephson phase synchronization across the system. We apply the results for interpretation of experimental data in disordered films near the superconductor-insulator transition.

Quantum metallicity on the high-field side of the superconductor-insulator transition.

We investigate ultrathin superconducting TiN films, which are very close to the localization threshold. Perpendicular magnetic field drives the films from the superconducting to an insulating state, with very high resistance. Further increase of the magnetic field leads to an exponential decay of the resistance towards a finite value. In the limit of low temperatures, the saturation value can be very accurately extrapolated to the universal quantum resistance h/e2. Our analysis suggests that at high magnetic fields a new ground state, distinct from the normal metallic state occurring above the superconducting transition temperature, is formed. A comparison with other studies on different materials indicates that the quantum metallic phase following the magnetic-field-induced insulating phase is a generic property of systems close to the disorder-driven superconductor-insulator transition.

Localized superconductivity in the quantum-critical region of the disorder-driven superconductor-insulator transition in TiN thin films.

We investigate low-temperature transport properties of thin TiN superconducting films in the vicinity of the disorder-driven superconductor-insulator transition. In a zero magnetic field, we find an extremely sharp separation between superconducting and insulating phases, evidencing a direct superconductor-insulator transition without an intermediate metallic phase. At moderate temperatures, in the insulating films we reveal thermally activated conductivity with the magnetic field-dependent activation energy. At very low temperatures, we observe a zero-conductivity state, which is destroyed at some depinning threshold voltage V{T}. These findings indicate the formation of a distinct collective state of the localized Cooper pairs in the critical region at both sides of the transition.