Thermal and Coherent Spin Pumping by Noncollinear Antiferromagnets.

Antiferromagnets attract much interest because of their potential for spintronic applications and open fundamental physics questions, but especially noncollinear antiferromagnets remain relatively unexplored. Here, we formulate the thermal and coherent pumping of spins in noncollinear antiferromagnets|normal metal bilayers. We find that the spin current polarization is a vector with components along both the Néel vector and net magnetic moment. The spin mixing conductance for the coherent spin pumping is a tensor with elements depending on the degree of noncollinearity and interface spin configuration. We explain the controversial sign problem of the antiferromagnetic spin Seebeck effect by interface effects and suggest that interface engineering may enhance the spin pumping efficiency.

Sliding Phase Transition in Ferroelectric van der Waals Bilayers.

We address the sliding thermodynamics of van der Waals-bonded bilayers by continuum electromechanics. We attribute the robustness of the ferroelectricity recently observed in h-BN and WTe_{2} bilayers to large in-plane stiffness of the monolayers. We compute the electric susceptibility and specific heat in a mean-field self-consistent phonon approximation. We compare critical temperatures and electric switching fields with the observed values.

Electric field-dependent phonon spectrum and heat conduction in ferroelectrics.

This article shows experimentally that an external electric field affects the velocity of the longitudinal acoustic phonons (vLA), thermal conductivity (κ), and diffusivity (D) in a bulk lead zirconium titanate-based ferroelectric. Phonon conduction dominates κ, and the observations are due to changes in the phonon dispersion, not in the phonon scattering. This gives insight into the nature of the thermal fluctuations in ferroelectrics, namely, phonons labeled ferrons that carry heat and polarization. It also opens the way for phonon-based electrically driven all-solid-state heat switches, an enabling technology for solid-state heat engines. A quantitative theoretical model combining piezoelectric strain and phonon anharmonicity explains the field dependence of vLA, κ, and D without any adjustable parameters, thus connecting thermodynamic equilibrium properties with transport properties. The effect is four times larger than previously reported effects, which were ascribed to field-dependent scattering of phonons.

Nonlinear Magnon Polaritons.

We experimentally and theoretically demonstrate that nonlinear spin-wave interactions suppress the hybrid magnon-photon quasiparticle or "magnon polariton" in microwave spectra of a yttrium iron garnet film detected by an on-chip split-ring resonator. We observe a strong coupling between the Kittel and microwave cavity modes in terms of an avoided crossing as a function of magnetic fields at low microwave input powers, but a complete closing of the gap at high powers. The experimental results are well explained by a theoretical model including the three-magnon decay of the Kittel magnon into spin waves. The gap closure originates from the saturation of the ferromagnetic resonance above the Suhl instability threshold by a coherent backreaction from the spin waves.

Nonlocal Detection of Interlayer Three-Magnon Coupling.

A leading nonlinear effect in magnonics is the interaction that splits a high-frequency magnon into two low-frequency magnons with conserved linear momentum. Here, we report experimental observation of nonlocal three-magnon scattering between spatially separated magnetic systems, viz. a CoFeB nanowire and a yttrium iron garnet (YIG) thin film. Above a certain threshold power of an applied microwave field, a CoFeB Kittel magnon splits into a pair of counterpropagating YIG magnons that induce voltage signals in Pt electrodes on each side, in excellent agreement with model calculations based on the interlayer dipolar interaction. The excited YIG magnon pairs reside mainly in the first excited (n=1) perpendicular standing spin-wave mode. With increasing power, the n=1 magnons successively scatter into nodeless (n=0) magnons through a four-magnon process. Our results demonstrate nonlocal detection of two separately propagating magnons emerging from one common source that may enable quantum entanglement between distant magnons for quantum information applications.

Broadband microwave detection using electron spins in a hybrid diamond-magnet sensor chip.

Quantum sensing has developed into a main branch of quantum science and technology. It aims at measuring physical quantities with high resolution, sensitivity, and dynamic range. Electron spins in diamond are powerful magnetic field sensors, but their sensitivity in the microwave regime is limited to a narrow band around their resonance frequency. Here, we realize broadband microwave detection using spins in diamond interfaced with a thin-film magnet. A pump field locally converts target microwave signals to the sensor-spin frequency via the non-linear spin-wave dynamics of the magnet. Two complementary conversion protocols enable sensing and high-fidelity spin control over a gigahertz bandwidth, allowing characterization of the spin-wave band at multiple gigahertz above the sensor-spin frequency. The pump-tunable, hybrid diamond-magnet sensor chip opens the way for spin-based gigahertz material characterizations at small magnetic bias fields.

Efficient Gating of Magnons by Proximity Superconductors.

Electrostatic gating confines and controls the transport of electrons in integrated circuits. Magnons, the quanta of spin waves of the magnetic order, are promising alternative information carriers, but difficult to gate. Here we report that superconducting strips on top of thin magnetic films can totally reflect magnons by their diamagnetic response to the magnon stray fields. The induced large frequency shifts unidirectionally block the magnons propagating normal to the magnetization. Two superconducting gates parallel to the magnetization create a magnonic cavity. The option to gate coherent magnons adds functionalities to magnonic devices, such as reprogrammable logical devices and increased couplings to other degrees of freedom.

Analog Quantum Control of Magnonic Cat States on a Chip by a Superconducting Qubit.

We propose to directly and quantum-coherently couple a superconducting transmon qubit to magnons-the quanta of the collective spin excitations, in a nearby magnetic particle. The magnet's stray field couples to the qubit via a superconducting quantum interference device. We predict a resonant magnon-qubit exchange and a nonlinear radiation-pressure interaction that are both stronger than dissipation rates and tunable by an external flux bias. We additionally demonstrate a quantum control scheme that generates magnon-qubit entanglement and magnonic Schrödinger cat states with high fidelity.

Thermoelectric Polarization Transport in Ferroelectric Ballistic Point Contacts.

We formulate a scattering theory of polarization and heat transport through a ballistic ferroelectric point contact. We predict a polarization current under either an electric field or a temperature difference that depends strongly on the direction of the ferroelectric order and can be detected by its magnetic stray field and associated thermovoltage and Peltier effect.

Seebeck effect in nanomagnets.

We present a theory of the Seebeck effect in nanomagnets with dimensions smaller than the spin diffusion length, showing that the spin accumulation generated by a temperature gradient strongly affects the thermopower. We also identify a correction arising from the transverse temperature gradient induced by the anomalous Ettingshausen effect and an induced spin-heat accumulation gradient. The relevance of these effects for nanoscale magnets is illustrated byab initiocalculations on dilute magnetic alloys.

Theory of Transport in Ferroelectric Capacitors.

The spontaneous order of electric and magnetic dipoles in ferroelectrics and ferromagnets even at high temperatures is both fascinating and useful. Transport of magnetism in the form of spin currents is vigorously studied in spintronics, but the polarization current of the ferroelectric order has escaped attention. We therefore present a time-dependent diffusion theory for heat and polarization transport in a planar ferroelectric capacitor with parameters derived from a one-dimensional phonon model. We predict steady-state Seebeck and transient Peltier effects that await experimental discovery.

Spin-Wave Doppler Shift by Magnon Drag in Magnetic Insulators.

The Doppler shift of the quasiparticle dispersion by charge currents is responsible for the critical supercurrents in superconductors and instabilities of the magnetic ground state of metallic ferromagnets. Here we predict an analogous effect in thin films of magnetic insulators in which microwaves emitted by a proximity stripline generate coherent chiral spin currents that cause a Doppler shift in the magnon dispersion. The spin-wave instability is suppressed by magnon-magnon interactions that limit spin currents to values close to but below the threshold for the instability. The spin current limitations by the backaction of magnon currents on the magnetic order should be considered as design parameters in magnonic devices.

Magnetic resonance imaging of spin-wave transport and interference in a magnetic insulator.

Spin waves-the elementary excitations of magnetic materials-are prime candidate signal carriers for low-dissipation information processing. Being able to image coherent spin-wave transport is crucial for developing interference-based spin-wave devices. We introduce magnetic resonance imaging of the microwave magnetic stray fields that are generated by spin waves as a new approach for imaging coherent spin-wave transport. We realize this approach using a dense layer of electronic sensor spins in a diamond chip, which combines the ability to detect small magnetic fields with a sensitivity to their polarization. Focusing on a thin-film magnetic insulator, we quantify spin-wave amplitudes, visualize spin-wave dispersion and interference, and demonstrate time-domain measurements of spin-wave packets. We theoretically explain the observed anisotropic spin-wave patterns in terms of chiral spin-wave excitation and stray-field coupling to the sensor spins. Our results pave the way for probing spin waves in atomically thin magnets, even when embedded between opaque materials.

Unidirectional Pumping of Phonons by Magnetization Dynamics.

We propose a method to control surface phonon transport by weak magnetic fields based on the pumping of surface acoustic waves (SAWs) by magnetostriction. We predict that the magnetization dynamics of a nanowire on top of a dielectric films injects SAWs with opposite angular momenta into opposite directions. Two parallel nanowires form a phononic cavity that at magnetic resonances pump a unidirectional SAW current into half of the substrate.

Noncontact Spin Pumping by Microwave Evanescent Fields.

The angular momentum of evanescent light fields has been studied in nano-optics and plasmonics but not in the microwave regime. Here we predict noncontact pumping of electron spin currents in conductors by the evanescent stray fields of excited magnetic nanostructures. The coherent transfer of the photon to the electron spin is proportional to the g factor, which is large in narrow gap semiconductors and surface states of topological insulators. The spin pumping current is chiral when the spin susceptibility displays singularities that indicate collective states. However, 1D systems with linear dispersion at the Fermi energy, such as metallic carbon nanotubes, are an exception since spin pumping is chiral even without interactions.

Voltage- and temperature-dependent rare-earth dopant contribution to the interfacial magnetic anisotropy.

The control of magnetic materials and devices by voltages without electric currents holds the promise of power-saving nano-scale devices. Here we study the temperature-dependent voltage control of the magnetic anisotropy caused by rare-earth (RE) local moments at an interface between a magnetic metal and a non-magnetic insulator, such as Co|(RE)|MgO. Based on a Stevens operator representation of crystal and applied field effects, we find large dominantly quadrupolar intrinsic and field-induced interface anisotropies at room temperature. We suggest improved functionalities of transition metal tunnel junctions by dusting their interfaces with rare earths.

Magnon Accumulation in Chirally Coupled Magnets.

We report strong chiral coupling between magnons and photons in microwave waveguides that contain chains of small magnets on special lines. Large magnon accumulations at one edge of the chain emerge when exciting the magnets by a phased antenna array. This mechanism holds the promise of new functionalities in nonlinear and quantum magnonics.

Spin transport in insulators without exchange stiffness.

The discovery of new materials that efficiently transmit spin currents has been important for spintronics and material science. The electric insulator Gd3Ga5O12 (GGG), a standard substrate for growing magnetic films, can be a spin current generator, but has never been considered as a superior conduit for spin currents. Here we report spin current propagation in paramagnetic GGG over several microns. Surprisingly, spin transport persists up to temperatures of 100 K [Formula: see text] Tg = 180 mK, the magnetic glass-like transition temperature of GGG. At 5 K and 3.5 T, we find a spin diffusion length λGGG = 1.8 ± 0.2 µm and a spin conductivity σGGG = (7.3 ± 0.3) × 104 Sm-1 that is larger than that of the record quality magnet Y3Fe5O12 (YIG). We conclude that exchange stiffness is not required for efficient spin transport, which challenges conventional models and provides new material-design strategies for spintronic devices.

Chiral Pumping of Spin Waves.

We report a theory for the coherent and incoherent chiral pumping of spin waves into thin magnetic films through the dipolar coupling with a local magnetic transducer, such as a nanowire. The ferromagnetic resonance of the nanowire is broadened by the injection of unidirectional spin waves that generates a nonequilibrium magnetization in only half of the film. A temperature gradient between the local magnet and film leads to a unidirectional flow of incoherent magnons, i.e., a chiral spin Seebeck effect.

Optical Cooling of Magnons.

Inelastic scattering of light by spin waves generates an energy flow between the light and magnetization fields, a process that can be enhanced and controlled by concentrating the light in magneto-optical resonators. Here, we model the cooling of a sphere made of a magnetic insulator, such as yttrium iron garnet, using a monochromatic laser source. When the magnon lifetimes are much larger than the optical ones, we can treat the latter as a Markovian bath for magnons. The steady-state magnons are canonically distributed with a temperature that is controlled by the light intensity. We predict that such a cooling process can significantly reduce the temperature of the magnetic order within current technology.