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1.
J Air Waste Manag Assoc ; 71(10): 1251-1264, 2021 10.
Artigo em Inglês | MEDLINE | ID: mdl-34406104

RESUMO

The potential effects of 21st century climate change on ozone (O3) concentrations in the United States are investigated using global climate simulations to drive higher-resolution regional meteorological and chemical transport models. Community Earth System Model (CESM) and Coupled Model version 3 (CM3) simulations of the Representative Concentration Pathway 8.5 scenario are dynamically downscaled using the Weather Research and Forecasting model, and the resulting meteorological fields are used to drive the Community Multiscale Air Quality model. Air quality is modeled for five 11-year periods using both a 2011 air pollutant emission inventory and a future projection accounting for full implementation of promulgated regulatory controls. Across the U.S., CESM projects daily maximum temperatures during summer to increase 1-4°C by 2050 and 2-7°C by 2095, while CM3 projects warming of 2-7°C by 2050 and 4-11°C by 2095. The meteorological changes have geographically varying impacts on O3 concentrations. Using the 2011 emissions dataset, O3 increases 1-5 ppb in the central Great Plains and Midwest by 2050 and more than 10 ppb by 2095, but it remains unchanged or even decreases in the Gulf Coast, Maine, and parts of the Southwest. Using the projected emissions, modeled increases are attenuated while decreases are amplified, indicating that planned air pollution control measures ameliorate the ozone climate penalty. The relationships between changes in maximum temperature and changes in O3 concentrations are examined spatially and quantified to explore the potential for developing an efficient approach for estimating air quality impacts of other future climate scenarios.Implications: The effects of climate change on ozone air quality in the United States are investigated using two global climate model simulations of a high warming scenario for five decadal periods in the 21st century. Warming summer temperatures simulated under both models lead to higher ozone concentrations in some regions, with the magnitude of the change increasing with temperature over the century. The magnitude and spatial extent of the increases are attenuated under a future emissions projection that accounts for regulatory controls. Regional linear regression relationships are developed as a first step toward development of a reduced form model for efficient estimation of the health impacts attributable to changes in air quality resulting from a climate change scenario.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Ozônio , Poluentes Atmosféricos/análise , Poluição do Ar/análise , Modelos Teóricos , Ozônio/análise , Temperatura , Estados Unidos
2.
Int J Climatol ; 41(2): 1305-1327, 2021 Feb 17.
Artigo em Inglês | MEDLINE | ID: mdl-34017157

RESUMO

The Weather Research and Forecasting (WRF) model and a combination of the Regional Spectral Model (RSM) and the Japanese Meteorological Agency Non-Hydrostatic Model (NHM) were used to dynamically downscale selected CMIP5 global climate models to provide 2-km projections with hourly model output for Puerto Rico and the U.S. Virgin Islands. Two 20-year time slices were downscaled for historical (1986-2005) and future (2041-2060) periods following RCP8.5. Projected changes to mean and extreme temperature and precipitation were quantified for Holdridge life zones within Puerto Rico and for the U.S. Virgin Islands. The evaluation reveals a persistent cold bias for all islands in the U.S. Caribbean, a dry bias across Puerto Rico, and a wet bias on the windward side of mountains within the U.S. Virgin Islands. Despite these biases, model simulations show a robust drying pattern for all islands that is generally larger for Puerto Rico (25% annual rainfall reduction for some life zones) than the U.S. Virgin Islands (12% island average). The largest precipitation reductions are found during the more convectively active afternoon and evening hours. Within Puerto Rico, the model uncertainty increases for the wetter life zones, especially for precipitation. Across the life zones, both models project unprecedented maximum and minimum temperatures that may exceed 200 days annually above the historical baseline with only small changes to the frequency of extreme rainfall. By contrast, in the U.S. Virgin Islands, there is no consensus on the location of the largest drying relative to the windward and leeward side of the islands. However, the models project the largest increases in maximum temperature on the southern side of St. Croix and in higher elevations of St. Thomas and St. John.

3.
Nat Clim Chang ; 4(23): 1-8, 2021 Mar 25.
Artigo em Inglês | MEDLINE | ID: mdl-34017361

RESUMO

In the past quarter-century, Eastern North Carolina (ENC) experienced several devastating tropical cyclones that led to widespread flooding and damage. Historical climate records reflect an increasing trend in the frequency and intensity of extreme rainfall events across the eastern U.S., which is projected to continue to increase throughout the twenty-first century. Potential changes to extreme rainfall across ENC are explored and quantified for 2025-2100 for three tropical cyclones using an approach based on relative changes in future extreme rainfall frequencies (return periods) from dynamically downscaled projections. Maximum rainfall intensities at '2100' could increase locally by 168%, with widespread regional increases in total rainfall up to 44%. Although these magnitudes exceed the consensus in the literature, the values here are comparable to the most extreme rainfall events observed in the U.S. during the early twenty-first century, which suggests that the intensity of projected future events is already a present-day reality.

4.
Atmos Chem Phys ; 18(20): 15471-15489, 2018.
Artigo em Inglês | MEDLINE | ID: mdl-30972111

RESUMO

The potential impacts of climate change on regional ozone (O3) and fine particulate (PM2.5) air quality in the United States are investigated by linking global climate simulations with regional scale meteorological and chemical transport models. Regional climate at 2000 and at 2030 under three Representative Concentration Pathways (RCPs) is simulated by using the Weather Research and Forecasting (WRF) model to downscale 11-year time slices from the Community Earth System Model (CESM). The downscaled meteorology is then used with the Community Multiscale Air Quality (CMAQ) model to simulate air quality during each of these 11-year periods. The analysis isolates the future air quality differences arising from climate-driven changes in meteorological parameters and specific natural emissions sources that are strongly influenced by meteorology. Other factors that will affect future air quality, such as anthropogenic air pollutant emissions and chemical boundary conditions, are unchanged across the simulations. The regional climate fields represent historical daily maximum and daily minimum temperatures well, with mean biases less than 2 K for most regions of the U.S. and most seasons of the year and good representation of variability. Precipitation in the central and eastern U.S. is well simulated for the historical period, with seasonal and annual biases generally less than 25%, with positive biases exceeding 25% in the western U.S. throughout the year and in part of the eastern U.S. during summer. Maximum daily 8-h ozone (MDA8 O3) is projected to increase during summer and autumn in the central and eastern U.S. The increase in summer mean MDA8 O3 is largest under RCP8.5, exceeding 4 ppb in some locations, with smaller seasonal mean increases of up to 2 ppb simulated during autumn and changes during spring generally less than 1 ppb. Increases are magnified at the upper end of the O3 distribution, particularly where projected increases in temperature are greater. Annual average PM2.5 concentration changes range from -1.0 to 1.0 µg m-3. Organic PM2.5 concentrations increase during summer and autumn due to increased biogenic emissions. Aerosol nitrate decreases during winter, accompanied by lesser decreases in ammonium and sulfate, due to warmer temperatures causing increased partitioning to the gas phase. Among meteorological factors examined to account for modeled changes in pollution, temperature and isoprene emissions are found to have the largest changes and the greatest impact on O3 concentrations.

5.
J Appl Meteorol Climatol ; 57(8): 1883-1906, 2018.
Artigo em Inglês | MEDLINE | ID: mdl-33623485

RESUMO

The use of nudging in the Weather Research and Forecasting (WRF) Model to constrain regional climate downscaling simulations is gaining in popularity because it can reduce error and improve consistency with the driving data. While some attention has been paid to whether nudging is beneficial for downscaling, very little research has been performed to determine best practices. In fact, many published papers use the default nudging configuration (which was designed for numerical weather prediction), follow practices used by colleagues, or adapt methods developed for other regional climate models. Here, a suite of 45 three-year simulations is conducted with WRF over the continental United States to systematically and comprehensively examine a variety of nudging strategies. The simulations here use a longer test period than did previously published works to better evaluate the robustness of each strategy through all four seasons, through multiple years, and across nine regions of the United States. The analysis focuses on the evaluation of 2-m temperature and precipitation, which are two of the most commonly required downscaled output fields for air quality, health, and ecosystems applications. Several specific recommendations are provided to effectively use nudging in WRF for regional climate applications. In particular, spectral nudging is preferred over analysis nudging. Spectral nudging performs best in WRF when it is used toward wind above the planetary boundary layer (through the stratosphere) and temperature and moisture only within the free troposphere. Furthermore, the nudging toward moisture is very sensitive to the nudging coefficient, and the default nudging coefficient in WRF is too high to be used effectively for moisture.

6.
Environ Res Lett ; 12(11)2017 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-33204303

RESUMO

Reductions in greenhouse gas (GHG) emissions can bring ancillary benefits of improved air quality and reduced premature mortality, in addition to slowing climate change. Here we study the co-benefits of global and domestic GHG mitigation on US air quality and human health in 2050 at fine resolution using dynamical downscaling of meteorology and air quality from global simulations to the continental US, and quantify for the first time the co-benefits from foreign GHG mitigation. Relative to the reference scenario from which RCP4.5 was created, global GHG reductions in RCP4.5 avoid 16000 PM2.5-related all-cause deaths yr-1 (90% confidence interval, 11700-20300), and 8000 (3600-12400) O3-related respiratory deaths yr-1 in the US in 2050. Foreign GHG mitigation avoids 15% and 62% of PM2.5- and O3-related total avoided deaths, highlighting the importance of foreign mitigation for US health. GHG mitigation in the US residential sector brings the largest co-benefits for PM2.5-related deaths (21% of total domestic co-benefits), and industry for O3 (17%). Monetized benefits for avoided deaths from ozone and PM2.5 are $137 ($87-187) per ton CO2 at high valuation and $45 ($29-62) at low valuation, of which 31% are from foreign GHG reductions. These benefits likely exceed the marginal cost of GHG reductions in 2050. The US gains significantly greater air quality and health co-benefits when its GHG emission reductions are concurrent with reductions in other nations. Similarly, previous studies estimating co-benefits locally or regionally may greatly underestimate the full co-benefits of coordinated global actions.

7.
Atmos Chem Phys ; 16(15): 9533-9548, 2016.
Artigo em Inglês | MEDLINE | ID: mdl-30245703

RESUMO

Policies to mitigate greenhouse gas (GHG) emissions will not only slow climate change, but can also have ancillary benefits of improved air quality. Here we examine the co-benefits of both global and regional GHG mitigation on U.S. air quality in 2050 at fine resolution, using dynamical downscaling methods, building on a previous global co-benefits study (West et al., 2013). The co-benefits for U.S. air quality are quantified via two mechanisms: through reductions in co-emitted air pollutants from the same sources, and by slowing climate change and its influence on air quality, following West et al. (2013). Additionally, we separate the total co-benefits into contributions from domestic GHG mitigation versus mitigation in foreign countries. We use the WRF model to dynamically downscale future global climate to the regional scale, the SMOKE program to directly process global anthropogenic emissions into the regional domain, and we provide dynamical boundary conditions from global simulations to the regional CMAQ model. The total co-benefits of global GHG mitigation from the RCP4.5 scenario compared with its reference are estimated to be higher in the eastern U.S. (ranging from 0.6-1.0 µg m-3) than the west (0-0.4 µg m-3) for PM2.5, with an average of 0.47 µg m-3 over U.S.; for O3, the total co-benefits are more uniform at 2-5 ppb with U.S. average of 3.55 ppb. Comparing the two mechanisms of co-benefits, we find that reductions of co-emitted air pollutants have a much greater influence on both PM2.5 (96% of the total co-benefits) and O3 (89% of the total) than the second co-benefits mechanism via slowing climate change, consistent with West et al. (2013). GHG mitigation from foreign countries contributes more to the U.S. O3 reduction (76% of the total) than that from domestic GHG mitigation only (24%), highlighting the importance of global methane reductions and the intercontinental transport of air pollutants. For PM2.5, the benefits of domestic GHG control are greater (74% of total). Since foreign contributions to co-benefits can be substantial, with foreign O3 benefits much larger than those from domestic reductions, previous studies that focus on local or regional co-benefits may greatly underestimate the total co-benefits of global GHG reductions. We conclude that the U.S. can gain significantly greater domestic air quality co-benefits by engaging with other nations to control GHGs.

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