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1.
Water Res ; 265: 122293, 2024 Aug 17.
Artigo em Inglês | MEDLINE | ID: mdl-39167972

RESUMO

Sorption-based atmospheric water harvesting holds promise for alleviating water scarcity, but current prototypes have not shown significant increases in practical yields despite efforts in the enlarged engineering scale. This is due to weakened heat and mass transfer with a packed sorbent bed. In this work, the desiccant-coated adsorbers were employed to fabricate the water harvesting device that incorporates internal fluid for cooling and heating during sorption and desorption. Featured with an internal cooling effect, practical water productivity could be improved by 1.75-9.96 times with a low desorption temperature (45-62 °C). The continuous water harvesting system could produce 0.77-3.98 Lwater/kgsorbent/day with a thermal energy consumption of 7.7-30.4 MJ/kg in wide climates from 20 % to 80 % RH, providing a reference for device design in the engineering view. The demonstration revealed that using natural cooling in the sorption stage has great benefits in improving water harvesting performance, which can be integrated into the building sectors or a wider range of scenarios.

2.
Nano Lett ; 20(5): 3791-3797, 2020 05 13.
Artigo em Inglês | MEDLINE | ID: mdl-32319296

RESUMO

Efficient heat removal and recovery are two conflicting processes that are difficult to achieve simultaneously. Here, in this work, we pave a new way to achieve this through the use of a smart thermogalvanic hydrogel film, in which the ions and water undergo two separate thermodynamic cycles: thermogalvanic reaction and water-to-vapor phase transition. When the hydrogel is attached to a heat source, it can achieve efficient evaporative cooling while simultaneously converting a portion of the waste heat into electricity. Moreover, the hydrogel can absorb water from the surrounding air to regenerate its water content later on. This reversibility can be finely designed. As an applicative demonstration, the hydrogel film with a thickness of 2 mm was attached to a cell phone battery while operating. It successfully decreased the temperature of the battery by 20 °C and retrieved electricity of 5 µW at the discharging rate of 2.2 C.

3.
Adv Mater ; 32(17): e1907307, 2020 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-32048339

RESUMO

High temperature brings adverse impacts on the energy efficiency, and even destroys a semiconductor device. Here, a novel and cost-effective strategy is proposed to boost the energy efficiency of semiconductor devices by using the self-adaptive evaporative cooling of a lithium- and bromine-enriched polyacrylamide hydrogel. Water inside the hydrogel can quickly evaporate to dissipate the waste heat generated by the nugatory carrier transport in the P-N junction. In dormancy, the hydrogel harvests water molecules from the surrounding air to regenerate itself. The hydrogel is demonstrated to low down the operating temperature of a commercial polycrystalline silicon solar cell by 17 °C under one sun condition and enhances its efficiency from 14.5% to 15.5%. It is also capable of increasing the maximum power of a simulated chip by 45% at a fixed operating temperature. The hydrogel is expected to be widely adopted in current semiconductor industry to improve its energy efficiency.

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