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1.
Environ Pollut ; 346: 123623, 2024 Apr 01.
Artigo em Inglês | MEDLINE | ID: mdl-38387545

RESUMO

Microplastics (MPs), pollutants detected at high frequency in the environment, can be served as carriers of many kinds of pollutants and have typical characteristics of environmental persistence and bioaccumulation. The potential risks of MPs ecological environment and health have been widely concerned by scholars and engineering practitioners. Previous reviews mostly focused on the pollution characteristics and ecological toxicity of MPs, but there were few reviews on MPs analysis methods, aging mechanisms and removal strategies. To address this issue, this review first summarizes the contamination characteristics of MPs in different environmental media, and then focuses on analyzing the detection methods and analyzing the aging mechanisms of MPs, which include physical aging and chemical aging. Further, the ecotoxicity of MPs to different organisms and the associated enhanced removal strategies are outlined. Finally, some unresolved research questions related to MPs are prospected. This review focuses on the ageing and ecotoxic behaviour of MPs and provides some theoretical references for the potential environmental risks of MPs and their deep control.


Assuntos
Poluentes Ambientais , Poluentes Químicos da Água , Microplásticos/toxicidade , Microplásticos/análise , Plásticos/toxicidade , Monitoramento Ambiental/métodos , Poluentes Químicos da Água/toxicidade , Poluentes Químicos da Água/análise , Poluentes Ambientais/toxicidade , Poluentes Ambientais/análise
2.
Sci Total Environ ; 912: 168822, 2024 Feb 20.
Artigo em Inglês | MEDLINE | ID: mdl-38043821

RESUMO

The preparation of biochar from digestate is one of the effective ways to achieve the safe disposal and resource utilization of digestate. Nevertheless, up to now, a comprehensive review encompassing the factors influencing anaerobic digestate-derived biochar production and its applications is scarce in the literature. Therefore, to fill this gap, the present work first outlined the research hotspots of digestate in the last decade using bibliometric statistical analysis with the help of VOSviewer. Then, the characteristics of the different sources of digestate were summarized. Furthermore, the influencing factors of biochar preparation from digestate and the modification methods of digestate-derived biochar and associated mechanisms were analyzed. Notably, a comprehensive synthesis of anaerobic digestate-derived biochar applications is provided, encompassing enhanced anaerobic digestion, heavy metal remediation, aerobic composting, antibiotic/antibiotic resistance gene removal, and phosphorus recovery from digestate liquor. The economic and environmental impacts of digestate-derived biochar were also analyzed. Finally, the development prospect and challenges of using biochar from digestate to combat environmental pollution are foreseen. The aim is to not only address digestate management challenges at the source but also offer a novel path for the resourceful utilization of digestate.


Assuntos
Carvão Vegetal , Recuperação e Remediação Ambiental , Meio Ambiente , Poluição Ambiental , Anaerobiose
3.
Artigo em Inglês | MEDLINE | ID: mdl-38158486

RESUMO

The issue of environmental pollution caused by the widespread presence of microplastics (MPs) in environmental media has garnered significant attention. However, research on MPs pollution has mainly focused on aquatic ecosystems in recent years. The sources and pollution characteristics of MPs in the environment, especially in solid waste, have not been well-described. Additionally, there are few reports on the ecotoxicity of MPs, which highlights the need to fill this gap. This review first summarizes the occurrence characteristics of MPs in water, soil, and marine environments, and then provides an overview of their toxic effects on organisms and the relevant mechanisms. This paper also provides an outlook on the hotspots of research on pollution characterization and ecotoxicity of MPs. Finally, this review aims to provide insights for future ecotoxicity control of MPs. Overall, this paper expands our understanding of the pollution characteristics and ecological toxicity of MPs in current environmental media, providing forward-looking guidance for future research.

4.
Bioresour Technol ; 387: 129647, 2023 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-37567350

RESUMO

In light of the characteristics of excessive acidification and low biogas yield during kitchen waste (KW) dry digestion, the impact of the calcium oxide (CaO) on KW mesophilic dry digestion was investigated, and the enhanced mechanism was revealed through metagenomic approach. The results showed that CaO increased the biogas production, when the CaO dosage was 0.07 g/g (based on total solid), the biogas production reached 656.84 mL/g suspended solids (VS), approximately 8.38 times of that in the control. CaO promoted the leaching and hydrolysis of key organic matter in KW. CaO effectively promoted the conversion of volatile fatty acid (VFA) and mitigated over-acidification. Macrogenome analysis revealed that CaO increased the microbial diversity in KW dry digestion and upregulated the abundance of genes related to amino acid and carbohydrates metabolism. This study provides an effective strategy with potential economic benefits to improve the bioconversion efficiency of organic matter in KW.


Assuntos
Biocombustíveis , Ácidos Graxos Voláteis , Anaerobiose , Ácidos Graxos Voláteis/metabolismo , Compostos de Cálcio , Metano/metabolismo , Reatores Biológicos
5.
Bioresour Technol ; 370: 128534, 2023 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-36574889

RESUMO

This work investigated the effect of calcium hypochlorite (CH) coupled aged refuse (AR) treatment on the enhanced hydrogen generation from sludge anaerobic dark fermentation (SADF). The enhanced mechanism was systematically revealed through sludge disintegration, organic matter biotransformation, and microbial community characteristics, etc. The experimental data showed that CH coupled AR increased the hydrogen yield to 18.1 mL/g, significantly higher than that in the AR or CH group alone. Mechanistic analysis showed that CH-coupled AR significantly promoted sludge disintegration and hydrolysis processes, providing sufficient material for hydrogen-producing bacteria. Microbiological analysis showed that CH-coupled AR increased the relative abundance of responsible hydrogen-producing microorganisms. In addition, CH-coupled AR was very effective in reducing phosphate content in the fermentation liquid and fecal coliforms in the digestate, thus facilitating the subsequent treatment of fermentation broth and digestate. CH coupled AR is an alternative strategy to increase hydrogen production from sludge.


Assuntos
Hidrogênio , Esgotos , Fermentação , Anaerobiose , Esgotos/microbiologia , Hidrogênio/metabolismo , Concentração de Íons de Hidrogênio , Ácidos Graxos Voláteis/metabolismo
6.
Bioresour Technol ; 368: 128358, 2023 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-36414141

RESUMO

Polybrominated diphenyl ethers (PBDEs), derived from electronics, furniture, etc., are detected with high level in excess sludge (ES). In this work, the influence of PBDEs on ES dark fermentation (ESDF) hydrogen production and the related key mechanisms were explored. The result shows PBDEs exposure reduced hydrogen production, and hydrogen accumulation decreased from 17.6 mL/g in blank to 12.3 mL/g with 12.0 mg/Kg PBDEs. PBDEs induced the reactive oxygen species production, which directly led to cell inactivation and reduced hydrogen production. Furthermore, PBDEs decreased ES disintegration, hydrolysis, acidification and homoacetogenic processes and inhibited the activities of enzymes related to hydrogen production. PBDEs also affected the diversity and richness of microbial communities in dark fermentation systems, especially high doses of PBDEs reduced the relative abundance of microorganisms associated with hydrogen production. In conclusion, PBDEs reduce hydrogen generation from ES.


Assuntos
Poluentes Ambientais , Éteres Difenil Halogenados , Esgotos , Fermentação , Hidrogênio
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