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1.
Adv Mater ; 36(1): e2306441, 2024 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-37712832

RESUMO

The spontaneous formation and topological transitions of vortex-antivortex pairs have implications for a broad range of emergent phenomena, for example, from superconductivity to quantum computing. Unlike magnets exhibiting collinear spin textures, helimagnets with noncollinear spin textures provide unique opportunities to manipulate topological forms such as (anti)merons and (anti)skyrmions. However, it is challenging to achieve multiple topological states and their interconversion in a single helimagnet due to the topological protection for each state. Here, the on-demand creation of multiple topological states in a helimagnet Fe0.5 Co0.5 Ge, including a spontaneous vortex pair of meron with topological charge N = -1/2 and antimeron with N = 1/2, and a vortex-antivortex bundle, that is, a bimeron (meron pair) with N = -1 is reported. The mutual transformation between skyrmions and bimerons with respect to the competitive effects of magnetic field and magnetic shape anisotropy is demonstrated. It is shown that electric currents drive the individual bimerons to form their connecting assembly and then into a skyrmion lattice. These findings signify the feasibility of designing topological states and offer new insights into the manipulation of noncollinear spin textures for potential applications in various fields.

2.
Adv Mater ; 35(20): e2210646, 2023 May.
Artigo em Inglês | MEDLINE | ID: mdl-36871172

RESUMO

3D topological spin textures-hopfions-are predicted in helimagnetic systems but are not experimentally confirmed thus far. By utilizing an external magnetic field and electric current in the present study, 3D topological spin textures are realized, including fractional hopfions with nonzero topological index, in a skyrmion-hosting helimagnet FeGe. Microsecond current pulses are employed to control the dynamics of the expansion and contraction of a bundle composed of a skyrmion and a fractional hopfion, as well as its current-driven Hall motion. This research approach has demonstrated the novel electromagnetic properties of fractional hopfions and their ensembles in helimagnetic systems.

3.
Nano Lett ; 22(23): 9358-9364, 2022 12 14.
Artigo em Inglês | MEDLINE | ID: mdl-36383503

RESUMO

Nanometric topological spin textures, such as skyrmions (Sks) and antiskyrmions (antiSks), have attracted much attention recently. However, most studies have focused on two-dimensional spin textures in films with inherent or synthetic antisymmetric spin-exchange interaction, termed Dzyaloshinskii-Moriya interaction, although three-dimensional (3D) topological spin textures, such as antiSks composed of alternating Bloch- and Néel-type spin spirals, chiral bobbers carrying emergent magnetic monopoles, and deformed Sk strings, are ubiquitous. To elucidate these textures, we have developed a 3D nanometric magnetic imaging technique, tomographic Lorentz transmission electron microscopy (TEM). The approach enables the visualization of the 3D shape of magnetic objects and their 3D vector field mapping. Here we report 3D vector field maps of deformed Sk-strings and antiSk using the technique. This research approach will lead to discoveries and understanding of fertile 3D magnetic structures in a broad class of magnets, providing insight into 3D topological magnetism.


Assuntos
Imageamento Tridimensional , Imãs , Microscopia Eletrônica de Transmissão
4.
Adv Sci (Weinh) ; 9(28): e2202950, 2022 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-35978271

RESUMO

Magnetic skyrmions and antiskyrmions have attracted much interest owing to their topological features and spintronic functionalities. In contrast to skyrmions, the generation of antiskyrmions relies on tunning both the magnitude and direction of the external magnetic field. Here, it is reported that antiskyrmions can be efficiently created via quenching and robustly persist at zero field in the Fe1.9 Ni0.9 Pd0.2 P magnet with the S4 -symmetry. It is demonstrated that well-ordered antiskyrmions form in a square lattice in a confining micrometer-scale square geometry, while the antiskyrmion lattice distorts in triangular, circular, or rotated-square geometry; the distortion depends on the relative configuration between sample edges and the two q-vectors arising from the anisotropic Dzyaloshinskii-Moriya interaction, in good agreement with micromagnetic simulations. It is also characterized transformations from antiskyrmions to skyrmions and nontopological bubbles at different directions and values of external field. These results demonstrate a roadmap for generating and controlling antiskyrmions in a confining geometry.

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