Effects of the uncertainty contributions on the methods used for measurement uncertainty evaluation.

Adequate measurement uncertainty evaluation is crucial for supporting basic measurement purposes. However, the most prevalent approach, the uncertainty propagation, may not be validly applicable under certain conditions which require the use of less restricted alternative method (MCM-based propagation of distributions). We demonstrate the effects of major conditions, e.g. non-linear measurement model, non-Gaussian input quantities, on the reliability of uncertainty evaluation methods, highlighting the importance of the less frequently examined impact of uncertainty component contributions to the standard uncertainty of measurand.

Evaluation of Hungarian monitoring results and source localization of the 106Ru release in the fall of 2017.

Anthropogenic 106Ru has been detected in the environment from late September to early October 2017 by several European environmental radiological monitoring networks. The paper presents the comprehensive evaluation of Hungarian monitoring results related to the occurrence of 106Ru in various environmental compartments (airborne particulates, deposition, plants, and terrestrial indicators), which was implemented to determine the temporal and spatial variation of the contaminant on a national scale and also to verify the findings based on the data arising from environmental monitoring at a local scale in Budapest. Difficulties in direct comparison of the diverse reported data were also considered; results arising from varied sampling periods were corrected with account taken of the relation between the sampling duration and 4-day-long plume residence (estimation based on the daily monitoring of air and backward trajectory analysis). Integrated analysis of air and deposition measurements and meteorological data was also performed; the deposition processes were investigated by establishing the correlations of activity concentrations measured in the atmosphere and in the deposition samples. In order to study the temporal distribution and spatial localization of the 106Ru contamination and to interpret the measurements at ground level, backward trajectory analysis was performed with HYSPLIT model. The backward trajectory simulations suggested that the release had probably occurred during the last week of September 2017 from the geographical area between Volga and the Urals. In addition, assessment of the doses due to the 106Ru release was implemented considering external exposure from cloudshine and groundshine and internal exposure via inhalation.

Methods, results and dose consequences of 106Ru detection in the environment in Budapest, Hungary.

From late September to early October of 2017, the majority of European networks involved in environmental radiological monitoring - including the environmental monitoring system of the KFKI Campus in Budapest - detected 106Ru isotope of artificial origin in the atmosphere. The reported values higher than the minimum detectable activity (MDA) concentrations were in the range of 0.8 µBq/m3 - 145 mBq/m3. Based on the results of environmental measurements and the available meteorological data, assessments were made to analyze concentration levels of 106Ru activity and to help understand the behavior of radioruthenium in various environmental media. Evaluation of the daily variation of activity levels indicated a maximum of 4 day-long residence time of 106Ru contamination presence in ground level air in Budapest. An average 106Ru activity concentration of 25.6 ±â€¯1.4 mBq/m3 have been observed for the estimated residence time of 106Ru in the air. Deposition of 106Ru was dominantly influenced by rainfall, the major contributor wet deposition which led to an average of 11.3 ±â€¯1.3 Bq/m2 deposition on the ground surface prior to plume passage.