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1.
Materials (Basel) ; 16(12)2023 Jun 06.
Artigo em Inglês | MEDLINE | ID: mdl-37374395

RESUMO

The properties of Pb1-xMnxTe/CdTe multilayer composite grown by molecular beam epitaxy on a GaAs substrate were studied. The study included morphological characterization by X-ray diffraction, scanning electron microscopy, secondary ion mass spectroscopy, as well as electron transport and optical spectroscopy measurements. The main focus of the study was on the sensing properties of photoresistors made of Pb1-xMnxTe/CdTe in the infrared spectral region. It was shown that the presence of Mn in the Pb1-xMnxTe conductive layers shifted the cut-off wavelength toward blue and weakened the spectral sensitivity of the photoresistors. The first effect was due to an increase in the energy gap of Pb1-xMnxTe with an increase in Mn concentration, and the second was due to a pronounced deterioration in the crystal quality of the multilayers owing to the presence of Mn atoms, as shown by the morphological analysis.

2.
Nanoscale ; 15(8): 4143-4151, 2023 Feb 23.
Artigo em Inglês | MEDLINE | ID: mdl-36745383

RESUMO

Quantum dots consisting of an axial Zn0.97Mg0.03Te insertion inside a large-bandgap Zn0.9Mg0.1Te nanowire core are fabricated in a molecular-beam epitaxy system by employing the vapor-liquid-solid growth mechanism. In addition, this structure is coated with a thin ZnSe radial shell that forms a type-II interface with the dot semiconductor. The resulting radial electron-hole separation is evidenced by several distinct effects that occur in the presence of the ZnSe shell, including the optical emission redshift of about 250 meV, a significant decrease in emission intensity, an increase in the excitonic lifetime by one order of magnitude, and an increase in the biexciton binding energy. The type-II nanowire quantum dots where electrons and holes are radially separated constitute a promising platform for potential applications in the field of quantum information technology.

3.
Light Sci Appl ; 11(1): 315, 2022 Nov 01.
Artigo em Inglês | MEDLINE | ID: mdl-36316317

RESUMO

Achieving efficient, high-power harmonic generation in the terahertz spectral domain has technological applications, for example, in sixth generation (6G) communication networks. Massless Dirac fermions possess extremely large terahertz nonlinear susceptibilities and harmonic conversion efficiencies. However, the observed maximum generated harmonic power is limited, because of saturation effects at increasing incident powers, as shown recently for graphene. Here, we demonstrate room-temperature terahertz harmonic generation in a Bi2Se3 topological insulator and topological-insulator-grating metamaterial structures with surface-selective terahertz field enhancement. We obtain a third-harmonic power approaching the milliwatt range for an incident power of 75 mW-an improvement by two orders of magnitude compared to a benchmarked graphene sample. We establish a framework in which this exceptional performance is the result of thermodynamic harmonic generation by the massless topological surface states, benefiting from ultrafast dissipation of electronic heat via surface-bulk Coulomb interactions. These results are an important step towards on-chip terahertz (opto)electronic applications.

4.
Nanotechnology ; 32(49)2021 Sep 16.
Artigo em Inglês | MEDLINE | ID: mdl-34438391

RESUMO

ZnTe/CdSe/(Zn, Mg)Te core/double-shell nanowires are grown by molecular beam epitaxy by employing the vapor-liquid-solid growth mechanism assisted with gold catalysts. A photoluminescence study of these structures reveals the presence of an optical emission in the near infrared. We assign this emission to the spatially indirect exciton recombination at the ZnTe/CdSe type II interface. This conclusion is confirmed by the observation of a significant blue-shift of the emission energy with an increasing excitation fluence induced by the electron-hole separation at the interface. Cathodoluminescence measurements reveal that the optical emission in the near infrared originates from nanowires and not from two-dimensional residual deposits between them. Moreover, it is demonstrated that the emission energy in the near infrared depends on the average CdSe shell thickness and the average Mg concentration within the (Zn, Mg)Te shell. The main mechanism responsible for these changes is associated with the strain induced by the (Zn, Mg)Te shell in the entire core/shell nanowire heterostructure.

5.
Nano Lett ; 21(6): 2370-2375, 2021 Mar 24.
Artigo em Inglês | MEDLINE | ID: mdl-33689391

RESUMO

In a Fe/(Cd,Mg)Te/CdTe quantum well hybrid structure, short-range and long-range ferromagnetic proximity effects are found to coexist. The former is observed for conduction band electrons, while the latter is observed for holes bound to shallow acceptors in the CdTe quantum well. These effects arise from the interaction of charge carriers confined in the quantum well with different ferromagnets, where electrons interact with the Fe film and holes with an interfacial ferromagnet at the Fe/(Cd,Mg)Te interface. The two proximity effects originate from fundamentally different physical mechanisms. The short-range proximity effect for electrons is determined by the overlap of their wave functions with d-electrons of the Fe film. On the contrary, the long-range effect for holes bound to acceptors is not associated with overlapping wave functions and can be mediated by elliptically polarized phonons. The coexistence of the two ferromagnetic proximity effects reveals the presence of a nontrivial spin texture within the same heterostructure.

6.
Materials (Basel) ; 13(8)2020 Apr 11.
Artigo em Inglês | MEDLINE | ID: mdl-32290498

RESUMO

Grating metamaterials were fabricated with electron beam lithography on CdTe/CdMgTe modulation doped structures with two non-interacting quantum wells. Two types of samples were studied: with etched gratings and with gratings formed by deposition of Au stripes. The polarization properties at THz frequencies of the gratings were determined at room temperature. It was shown that Au gratings formed a linear polarizer, while etched gratings did not polarize THz radiation. Transmission of circularly polarized THz radiation at low temperatures through a sample with no grating showed a strongly circularly polarized cyclotron resonance transition. Transmission of this radiation through a sample with an etched grating showed a magnetoplasmon transition that was almost perfectly linearly polarized. We concluded that magnetoplasmons in metamaterials with etched gratings are linearly polarized excitations, possibly with a small contribution of a circular component. This work opens the possibility of the detailed study of the polarization of magnetoplasmons, which has not been explored in the past.

7.
Nanotechnology ; 31(21): 215710, 2020 May 22.
Artigo em Inglês | MEDLINE | ID: mdl-32050170

RESUMO

Wurtzite CdTe and (Cd,Mn)Te nanowires embedded in (Cd,Mg)Te shells are grown by employing vapour-liquid-solid growth mechanism in a system for molecular beam epitaxy. A combined study involving cathodoluminescence, transmission electron microscopy and micro-photoluminescence is used to correlate optical and structural properties in these structures. Typical features of excitonic emission from individual wurtzite nanowires are highlighted including the emission energy of 1.65 eV, polarization properties and the appearance B-exciton related emission at high excitation densities. Angle dependent magneto-optical study performed on individual (Cd,Mn)Te nanowires reveals heavy-hole-like character of A-excitons typical for wurtzite structure and allows to determine the crystal field splitting, ΔCR. The impact of the strain originating from the lattice mismatched shell is discussed and supported by theoretical calculations.

8.
Nanotechnology ; 29(20): 205205, 2018 May 18.
Artigo em Inglês | MEDLINE | ID: mdl-29488898

RESUMO

A detailed magneto-photoluminescence study of individual (Cd, Mn)Te/(Cd, Mg)Te core/shell nanowires grown by molecular beam epitaxy is performed. First of all, an enhancement of the Zeeman splitting due to sp-d exchange interaction between band carriers and Mn-spins is evidenced in these nanostructures. Then, it is found that the value of this splitting depends strongly on the magnetic field direction with respect to the nanowire axis. The largest splitting is observed when the magnetic field is applied perpendicular and the smallest when it is applied parallel to the nanowire axis. This effect is explained in terms of magnetic field induced valence band mixing and evidences the light hole character of the excitonic emission. The values of the light and heavy hole splitting are determined for several individual nanowires based on the comparison of experimental results to theoretical calculations.

9.
Phys Rev Lett ; 119(4): 046803, 2017 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-29341779

RESUMO

In this work, we use electrostatic control of quantum Hall ferromagnetic transitions in CdMnTe quantum wells to study electron transport through individual domain walls (DWs) induced at a specific location. These DWs are formed due to the hybridization of two counterpropagating edge states with opposite spin polarization. Conduction through DWs is found to be symmetric under magnetic field direction reversal, consistent with the helical nature of these DWs. We observe that long domain walls are in the insulating regime with a localization length of 4-6 µm. In shorter DWs, the resistance saturates to a nonzero value at low temperatures. Mesoscopic resistance fluctuations in a magnetic field are investigated. The theoretical model of transport through impurity states within the gap induced by spin-orbit interactions agrees well with the experimental data. Helical DWs have the required symmetry for the formation of synthetic p-wave superconductors. The achieved electrostatic control of a single helical domain wall is a milestone on the path to their reconfigurable network and ultimately to a demonstration of the braiding of non-Abelian excitations.

10.
Nano Lett ; 15(3): 1972-8, 2015 Mar 11.
Artigo em Inglês | MEDLINE | ID: mdl-25710186

RESUMO

We study the impact of the nanowire shape anisotropy on the spin splitting of excitonic photoluminescence. The experiments are performed on individual ZnMnTe/ZnMgTe core/shell nanowires as well as on ZnTe/ZnMgTe core/shell nanowires containing optically active magnetic CdMnTe insertions. When the magnetic field is oriented parallel to the nanowire axis, the spin splitting is several times larger than for the perpendicular field. We interpret this pronounced anisotropy as an effect of mixing of valence band states arising from the strain present in the core/shell geometry. This interpretation is further supported by theoretical calculations which allow to reproduce experimental results.

11.
Phys Rev Lett ; 112(5): 057601, 2014 Feb 07.
Artigo em Inglês | MEDLINE | ID: mdl-24580629

RESUMO

By means of spin- and angle-resolved photoelectron spectroscopy we studied the spin structure of thin films of the topological insulator Bi2Se3 grown on InP(111). For thicknesses below six quintuple layers the spin-polarized metallic topological surface states interact with each other via quantum tunneling and a gap opens. Our measurements show that the resulting surface states can be described by massive Dirac cones which are split in a Rashba-like manner due to the substrate induced inversion asymmetry. The inner and the outer Rashba branches have distinct localization in the top and the bottom part of the film, whereas the band apices are delocalized throughout the entire film. Supported by calculations, our observations help in the understanding of the evolution of the surface states at the topological phase transition and provide the groundwork for the realization of two-dimensional spintronic devices based on topological semiconductors.

12.
Nano Lett ; 12(7): 3404-9, 2012 Jul 11.
Artigo em Inglês | MEDLINE | ID: mdl-22732058

RESUMO

An enhancement of the Zeeman splitting as a result of the incorporation of paramagnetic Mn ions in ZnMnTe/ZnMgTe core/shell nanowires is reported. The studied structures are grown by gold-catalyst assisted molecular beam epitaxy. The near band edge emission of these structures, conspicuously absent in the case of uncoated ZnMnTe nanowires, is activated by the presence of ZnMgTe coating. Giant Zeeman splitting of this emission is studied in ensembles of nanowires with various average Mn concentrations of the order of a few percent, as well as in individual nanowires. Thus, we show convincingly that a strong spin sp-d coupling is indeed present in these structures.

13.
Przegl Epidemiol ; 65(3): 451-4, 2011.
Artigo em Polonês | MEDLINE | ID: mdl-22184947

RESUMO

Congenital toxoplasmosis results from the primary infection with Toxoplasma gondii during the pregnancy. The more advanced pregnancy the higher risk of foetus infection, however the symptoms might be mild or the infection can be asymptomatic. However, undiagnosed infection in a new born baby results in further development of the disease in early childhood reflecting in sight and hearing impairment, neurological symptoms or mental retardation. Systematic and frequent serologic tests performed during the pregnancy can lead to the early diagnosis of primary infection and help to implement the treatment which slows down the disease progression in children with intrauterine infection. It also reduces the costs of long-term medical care required for the significantly disabled patients.


Assuntos
Complicações Parasitárias na Gravidez/diagnóstico , Complicações Parasitárias na Gravidez/prevenção & controle , Toxoplasma/isolamento & purificação , Toxoplasmose Congênita/diagnóstico , Toxoplasmose Congênita/prevenção & controle , Anticorpos Antiprotozoários/sangue , Diagnóstico Diferencial , Diagnóstico Precoce , Feminino , Humanos , Lactente , Gravidez , Complicações Parasitárias na Gravidez/imunologia , Gravidez de Alto Risco , Diagnóstico Pré-Natal/métodos , Fatores de Risco , Toxoplasmose Congênita/imunologia
14.
Nano Lett ; 8(11): 4061-5, 2008 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-18842031

RESUMO

It is shown that the growth of II-VI diluted magnetic semiconductor nanowires is possible by the catalytically enhanced molecular beam epitaxy (MBE). Zn(1-x)MnxTe NWs with manganese content up to x=0.60 were produced by this method. X-ray diffraction, Raman spectroscopy, and temperature dependent photoluminescence measurements confirm the incorporation of Mn(2+) ions in the cation substitutional sites of the ZnTe matrix of the NWs.

15.
Phys Rev Lett ; 97(24): 247601, 2006 Dec 15.
Artigo em Inglês | MEDLINE | ID: mdl-17280323

RESUMO

Field effect transistors with ferroelectric gates would make ideal rewritable nonvolatile memories were it not for the severe problems in integrating the ferroelectric oxide directly on the semiconductor channel. We propose a powerful way to avoid these problems using a gate material that is ferroelectric and semiconducting simultaneously. First, ferroelectricity in semiconductor (Cd,Zn)Te films is proven and studied using modified piezoforce scanning probe microscopy. Then, a rewritable field effect device is demonstrated by local poling of the (Cd,Zn)Te layer of a (Cd,Zn)Te/CdTe quantum well, provoking a reversible, nonvolatile change in the resistance of the 2D electron gas. The results point to a potential new family of nanoscale one-transistor memories.

16.
Przegl Epidemiol ; 59(4): 873-9, 2005.
Artigo em Polonês | MEDLINE | ID: mdl-16729429

RESUMO

OBJECTIVE: Evaluation of multiplex PCR utility for diagnosis of central nervous system disorders in HIV-infected patients. METHODS: Multiplex PCR assay for simultaneous detection of HSV-1, HSV-2, VZV, HHV-6, CMV, EBV, JCV, T. gondii DNA in 27 CSF samples from HIV-infected patients was used. PCR results were compared with clinical diagnosis and histopathological examination of brain obtained at autopsy. MAIN OBSERVATIONS: Five of seven positive results were corresponding with clinical diagnosis. In two cases also with autopsy. RESULTS: DNA of one or more pathogens was found in 6 out of 27 (22%) samples: CMV DNA in four patients, JCV DNA and T. gondii DNA in one patients each. In one case co-infections of CMV and EBV was found. CONCLUSIONS: Multiplex PCR is a useful diagnostic method. LIPA-CNS test has high specificity. Lack of nesting step of the reaction and PCR positive control verification could cause a relatively low sensitivity of the test.


Assuntos
Infecções Oportunistas Relacionadas com a AIDS/líquido cefalorraquidiano , Infecções Oportunistas Relacionadas com a AIDS/diagnóstico , Viroses do Sistema Nervoso Central/líquido cefalorraquidiano , Viroses do Sistema Nervoso Central/diagnóstico , Infecções por Herpesviridae/líquido cefalorraquidiano , Herpesviridae/isolamento & purificação , Reação em Cadeia da Polimerase/métodos , Infecções Oportunistas Relacionadas com a AIDS/virologia , Adulto , Autopsia , Viroses do Sistema Nervoso Central/virologia , DNA Viral/líquido cefalorraquidiano , Feminino , Humanos , Masculino , Pessoa de Meia-Idade , Reprodutibilidade dos Testes , Estudos Retrospectivos
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