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1.
Nat Commun ; 14(1): 3365, 2023 Jun 08.
Artigo em Inglês | MEDLINE | ID: mdl-37291127

RESUMO

Spin Seebeck effect (SSE) refers to the generation of an electric voltage transverse to a temperature gradient via a magnon current. SSE offers the potential for efficient thermoelectric devices because the transverse geometry of SSE enables to utilize waste heat from a large-area source by greatly simplifying the device structure. However, SSE suffers from a low thermoelectric conversion efficiency that must be improved for widespread application. Here we show that the SSE substantially enhances by oxidizing a ferromagnet in normal metal/ferromagnet/oxide structures. In W/CoFeB/AlOx structures, voltage-induced interfacial oxidation of CoFeB modifies the SSE, resulting in the enhancement of thermoelectric signal by an order of magnitude. We describe a mechanism for the enhancement that results from a reduced exchange interaction of the oxidized region of ferromagnet, which in turn increases a temperature difference between magnons in the ferromagnet and electrons in the normal metal and/or a gradient of magnon chemical potential in the ferromagnet. Our result will invigorate research for thermoelectric conversion by suggesting a promising way of improving the SSE efficiency.


Assuntos
Eletricidade , Elétrons , Animais , Estro , Temperatura Alta , Óxidos , Oxigênio
2.
Phys Rev Lett ; 125(2): 027205, 2020 Jul 10.
Artigo em Inglês | MEDLINE | ID: mdl-32701310

RESUMO

We theoretically show that the coupling between magnons in an antiferromagnetically coupled ferrimagnet and microwave photons in a cavity is largely enhanced at the angular momentum compensation point (T_{A}) when T_{A} is distinct from the magnetization compensation point. The origin of the enhanced magnon-photon coupling at T_{A} is identified as the antiferromagnetic spin dynamics combined with a finite magnetization. Moreover, we show that strong magnon-photon coupling can be achieved at high excitation frequency in a ferrimagnet, which is challenging to achieve for a ferromagnet due to low magnon frequency and for an antiferromagnet due to weak magnon-photon coupling. Our results will invigorate research on magnon-photon coupling by proposing ferrimagnets as a versatile platform that offers advantages of both ferromagnets and antiferromagnets.

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