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1.
Nat Commun ; 15(1): 7442, 2024 Aug 28.
Artigo em Inglês | MEDLINE | ID: mdl-39198418

RESUMO

Quantum materials have a fascinating tendency to manifest novel and unexpected electronic states upon proper manipulation. Ideally, such manipulation should induce strong and irreversible changes and lead to new relevant length scales. Plastic deformation introduces large numbers of dislocations into a material, which can organize into extended structures and give rise to qualitatively new physics as a result of the huge localized strains. However, this approach is largely unexplored in the context of quantum materials, which are traditionally grown to be as pristine and clean as possible. Here we show that plastic deformation induces robust magnetism in the quantum paraelectric SrTiO3, a property that is completely absent in the pristine material. We combine scanning magnetic measurements and near-field optical microscopy to find that the magnetic order is localized along dislocation walls and coexists with ferroelectric order along the walls. The magnetic signals can be switched on and off via external stress and altered by external electric fields, which demonstrates that plastically deformed SrTiO3 is a quantum multiferroic. These results establish plastic deformation as a versatile knob for the manipulation of the electronic properties of quantum materials.

2.
Proc Natl Acad Sci U S A ; 121(32): e2310195121, 2024 Aug 06.
Artigo em Inglês | MEDLINE | ID: mdl-39093945

RESUMO

The duality between deformations of elastic bodies and noninertial flows in viscous liquids has been a guiding principle in decades of research. However, this duality is broken when a spheroidal or other doubly curved liquid film is suddenly forced out of mechanical equilibrium, as occurs, e.g., when the pressure inside a liquid bubble drops rapidly due to rupture or controlled evacuation. In such cases, the film may evolve through a noninertial yet geometrically nonlinear surface dynamics, which has remained largely unexplored. We reveal the driver of such dynamics as temporal variations in the curvature of the evolving surface. Focusing on the prototypical example of a floating bubble that undergoes rapid depressurization, we show that the bubble surface evolves via a topological instability and a subsequent front propagation, whereby a small planar zone that includes a singular flow structure, analogous to a disclination in elastic systems, nucleates spontaneously and expands in the spherically shaped film. This flow pattern brings about hoop compression and triggers another, symmetry-breaking instability to the formation of radial wrinkles that invade the flattening film. Our analysis reveals the dynamics as a nonequilibrium branch of "jellium" physics, whereby a rate-of-change of surface curvature in a viscous film is akin to charge in an electrostatic medium that comprises polarizable and conducting domains. We explain key features underlying recent experiments and highlight a qualitative inconsistency between the prediction of linear stability analysis and the observed "wavelength" of surface wrinkles.

3.
Phys Rev Lett ; 129(23): 237001, 2022 Dec 02.
Artigo em Inglês | MEDLINE | ID: mdl-36563208

RESUMO

We study superconductivity in a three-dimensional zero-density Dirac semimetal in proximity to a ferroelectric quantum critical point. We find that the interplay of criticality, inversion-symmetry breaking, and Dirac dispersion gives rise to a robust superconducting state at the charge-neutrality point, where no Fermi surface is present. Using Eliashberg theory, we show that the ferroelectric quantum critical point is unstable against the formation of a ferroelectric density wave (FDW), whose fluctuations, in turn, lead to a first-order superconducting transition. Surprisingly, long-range superconducting and FDW orders are found to cooperate with each other, in contrast to the more usual scenario of phase competition. Therefore, we suggest that driving charge neutral Dirac materials, e.g., Pb_{x}Sn_{1-x}Te, through a ferroelectric quantum critical point may lead to superconductivity intertwined with FDW order.

4.
Nat Commun ; 13(1): 2655, 2022 May 12.
Artigo em Inglês | MEDLINE | ID: mdl-35551454

RESUMO

The origin of the pseudogap behavior, found in many high-Tc superconductors, remains one of the greatest puzzles in condensed matter physics. One possible mechanism is fermionic incoherence, which near a quantum critical point allows pair formation but suppresses superconductivity. Employing quantum Monte Carlo simulations of a model of itinerant fermions coupled to ferromagnetic spin fluctuations, represented by a quantum rotor, we report numerical evidence of pseudogap behavior, emerging from pairing fluctuations in a quantum-critical non-Fermi liquid. Specifically, we observe enhanced pairing fluctuations and a partial gap opening in the fermionic spectrum. However, the system remains non-superconducting until reaching a much lower temperature. In the pseudogap regime the system displays a "gap-filling" rather than "gap-closing" behavior, similar to the one observed in cuprate superconductors. Our results present direct evidence of the pseudogap state, driven by superconducting fluctuations.

5.
Phys Rev Lett ; 118(8): 085303, 2017 Feb 24.
Artigo em Inglês | MEDLINE | ID: mdl-28282165

RESUMO

We study the impact of the nonanalytic reconstruction of vortex cores on static vortex structures in weakly coupled superfluids. We show that, in rotating two-dimensional systems, the Abrikosov vortex lattice is unstable to vortex core deformation: Each zero of the wave function becomes a cut of finite length. The directors characterizing the orientations of the cuts are themselves ordered in superstructures due either to surface effects or to interaction with shear deformations of the lattice (spiral structure). Similar instability may also be observable in clean superconducting films.

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