Ultrafast electro-optic time-frequency fractional Fourier imaging at the single-photon level.

The Fractional Fourier Transform (FRT) corresponds to an arbitrary-angle rotation in the phase space, e.g., the time-frequency (TF) space, and generalizes the fundamentally important Fourier Transform. FRT applications range from classical signal processing (e.g., time-correlated noise optimal filtering) to emerging quantum technologies (e.g., super-resolution TF sensing) which rely on or benefit from coherent low-noise TF operations. Here a versatile low-noise single-photon-compatible implementation of the FRT is presented. Optical TF FRT can be synthesized as a series of a spectral disperser, a time-lens, and another spectral disperser. Relying on the state-of-the-art electro-optic modulators (EOM) for the time-lens, our method avoids added noise inherent to the alternatives based on non-linear optical interactions (such as wave-mixing, cross-phase modulation, or parametric processes). Precise control of the EOM-driving radio-frequency signal enables fast all-electronic control of the FRT angle. In the experiment, we demonstrate FRT angles of up to 1.63 rad for pairs of coherent temporally separated 11.5 ps-wide pulses in the near-infrared (800 nm). We observe a good agreement between the simulated and measured output spectra in the bright-light and single-photon-level regimes, and for a range of pulse separations (20 ps to 26.7 ps). Furthermore, a tradeoff is established between the maximal FRT angle and optical bandwidth, with the current setup accommodating up to 248 GHz of bandwidth. With the ongoing progress in EOM on-chip integration, we envisage excellent scalability and vast applications in all-optical TF processing both in the classical and quantum regimes.

Beating the spectroscopic Rayleigh limit via post-processed heterodyne detection.

Quantum-inspired superresolution methods surpass the Rayleigh limit in imaging, or the analogous Fourier limit in spectroscopy. This is achieved by carefully extracting the information carried in the emitted optical field by engineered measurements. An alternative to complex experimental setups is to use simple homodyne detection and customized data analysis. We experimentally investigate this method in the time-frequency domain and demonstrate the spectroscopic superresolution for two distinct types of light sources: thermal and phase-averaged coherent states. The experimental results are backed by theoretical predictions based on estimation theory.

Variable electro-optic shearing interferometry for ultrafast single-photon-level pulse characterization.

Despite the multitude of available methods, the characterization of ultrafast pulses remains a challenging endeavor, especially at the single-photon level. We introduce a pulse characterization scheme that maps the magnitude of its short-time Fourier transform. Contrary to many well-known solutions it does not require nonlinear effects and is therefore suitable for single-photon-level measurements. Our method is based on introducing a series of controlled time and frequency shifts, where the latter is performed via an electro-optic modulator allowing a fully-electronic experimental control. We characterized the full spectral and temporal width of a classical and single-photon-level pulse and successfully tested the applicability of the reconstruction algorithm of the spectral phase and amplitude. The method can be extended by implementing a phase-sensitive measurement and is naturally well-suited to partially-incoherent light.

Quantum Asymmetry and Noisy Multimode Interferometry.

Quantum asymmetry is a physical resource that coincides with the amount of coherence between the eigenspaces of a generator responsible for phase encoding in interferometric experiments. We highlight an apparently counterintuitive behavior that the asymmetry may increase as a result of a decrease of coherence inside a degenerate subspace. We intuitively explain and illustrate the phenomena by performing a three-mode single-photon interferometric experiment, where one arm carries the signal and two noisy reference arms have fluctuating phases. We show that the source of the observed sensitivity improvement is the reduction of correlations between these fluctuations and comment on the impact of the effect when moving from the single-photon quantum level to the classical regime. Finally, we also establish the analogy of the effect in the case of entanglement resource theory.

Single-Photon Hologram of a Zero-Area Pulse.

Single photons exhibit inherently quantum and unintuitive properties such as the Hong-Ou-Mandel effect, demonstrating their bosonic and quantized nature, yet at the same time may correspond to single excitations of spatial or temporal modes with a very complex structure. Those two features are rarely seen together. Here we experimentally demonstrate how the Hong-Ou-Mandel effect can be spectrally resolved and harnessed to characterize a complex temporal mode of a single-photon-a zero-area pulse-obtained via a resonant interaction of a terahertz-bandwidth photon with a narrow gigahertz-wide atomic transition of atomic vapor. The combination of bosonic quantum behavior with bandwidth-mismatched light-atom interaction is of fundamental importance for deeper understanding of both phenomena, as well as their engineering offering applications in characterization of ultrafast transient processes.

Fast imaging of multimode transverse-spectral correlations for twin photons.

Hyperentangled photonic states-exhibiting nonclassical correlations in several degrees of freedom-offer improved performance of quantum optical communication and computation schemes. Experimentally, a hyperentanglement of transverse-wave-vector and spectral modes can be obtained in a straightforward way with multimode parametric single-photon sources. Nevertheless, experimental characterization of such states remains challenging. Not only single-photon detection with high spatial resolution-a single-photon camera-is required, but also a suitable mode converter to observe the spectral-temporal degree of freedom. We experimentally demonstrate a measurement of full four-dimensional transverse-wave-vector-spectral correlations between pairs of photons produced in noncollinear spontaneous parametric downconversion. Utilization of a custom ultrafast single-photon camera provides high resolution and a short measurement time.

Quantum Optics of Spin Waves through ac Stark Modulation.

We bring the set of linear quantum operations, important for many fundamental studies in photonic systems, to the material domain of collective excitations known as spin waves. Using the ac Stark effect we realize quantum operations on single excitations and demonstrate a spin-wave analog of the Hong-Ou-Mandel effect, realized via a beam splitter implemented in the spin-wave domain. Our scheme equips atomic-ensemble-based quantum repeaters with quantum information processing capability and can be readily brought to other physical systems, such as doped crystals or room-temperature atomic ensembles.

Visibility-Based Hypothesis Testing Using Higher-Order Optical Interference.

Many quantum information protocols rely on optical interference to compare data sets with efficiency or security unattainable by classical means. Standard implementations exploit first-order coherence between signals whose preparation requires a shared phase reference. Here, we analyze and experimentally demonstrate the binary discrimination of visibility hypotheses based on higher-order interference for optical signals with a random relative phase. This provides a robust protocol implementation primitive when a phase lock is unavailable or impractical. With the primitive cost quantified by the total detected optical energy, optimal operation is typically reached in the few-photon regime.

Spatially resolved control of fictitious magnetic fields in a cold atomic ensemble.

Effective and unrestricted engineering of atom-photon interactions requires precise spatially resolved control of light beams. The significant potential of such manipulations lies in a set of disciplines ranging from solid-state to atomic physics. Here we use a Zeeman-like ac-Stark shift caused by a shaped laser beam to perform rotations of spins with spatial resolution in a large ensemble of cold rubidium atoms. We show that inhomogeneities of light intensity are the main source of dephasing and, thus, decoherence; yet, with proper beam shaping, this deleterious effect is strongly mitigated allowing rotations of 15 rad within one spin-precession lifetime. Finally, as a particular example of a complex manipulation enabled by our scheme, we demonstrate a range of collapse-and-revival behaviors of a free-induction decay signal by imprinting comb-like patterns on the atomic ensemble.

Wavevector multiplexed atomic quantum memory via spatially-resolved single-photon detection.

Parallelized quantum information processing requires tailored quantum memories to simultaneously handle multiple photons. The spatial degree of freedom is a promising candidate to facilitate such photonic multiplexing. Using a single-photon resolving camera, we demonstrate a wavevector multiplexed quantum memory based on a cold atomic ensemble. Observation of nonclassical correlations between Raman scattered photons is confirmed by an average value of the second-order correlation function [Formula: see text] in 665 separated modes simultaneously. The proposed protocol utilizing the multimode memory along with the camera will facilitate generation of multi-photon states, which are a necessity in quantum-enhanced sensing technologies and as an input to photonic quantum circuits.

Quantum fingerprinting using two-photon interference.

We present a quantum fingerprinting protocol relying on two-photon interference which does not require a shared phase reference between the parties preparing optical signals carrying data fingerprints. We show that the scaling of the protocol, in terms of transmittable classical information, is analogous to the recently proposed and demonstrated scheme based on coherent pulses and first-order interference, offering comparable advantage over classical fingerprinting protocols without access to shared prior randomness. We analyze the protocol taking into account non-Poissonian photon statistics of optical signals and a variety of imperfections, such as transmission losses, dark counts, and residual distinguishability. The impact of these effects on the protocol performance is quantified with the help of Chernoff information.