Time Crystal in a Single-Mode Nonlinear Cavity.

Time crystal is a class of nonequilibrium phases with broken time-translational symmetry. Here, we demonstrate the time crystal in a single-mode nonlinear cavity. The time crystal originates from the self-oscillation induced by a linear gain and is stabilized by a nonlinear damping. We show in the time crystal phase there are sharp dissipative gap closing and pure imaginary eigenvalues of the Liouvillian spectrum in the thermodynamic limit. Dynamically, we observe a metastable regime with the emergence of quantum oscillation, followed by a dissipative evolution with a timescale much longer than the oscillating period. Moreover, we show there is a dissipative phase transition at the Hopf bifurcation, which can be characterized by the photon number fluctuation in the steady state. These results pave a new promising way for further experiments and deepen our understanding of time crystals.

Fast Generation of GHZ-like States Using Collective-Spin XYZ Model.

The Greenberger-Horne-Zeilinger (GHZ) state is a key resource for quantum information processing and quantum metrology. The atomic GHZ state can be generated by one-axis twisting (OAT) interaction H_{OAT}=χJ_{z}^{2} with χ the interaction strength, but it requires a long evolution time χt=π/2 and is thus seriously influenced by decoherence and losses. Here we propose a three-body collective-spin XYZ model which creates a GHZ-like state in a very short timescale χt∼lnN/N for N particles. We show that this model can be effectively produced by applying Floquet driving to an original OAT Hamiltonian. Compared with the ideal GHZ state, the GHZ-like state generated using our model can maintain similar metrological properties reaching the Heisenberg-limited scaling, and it shows better robustness to decoherence and particle losses. This Letter opens the avenue for generating GHZ-like states with a large particle number, which holds great potential for the study of macroscopic quantum effects and for applications in quantum metrology and quantum information.

[Influence of Ammonium Sulfate and Ammonium Nitrate on the Properties of Ambient PM2.5 in Zhenjiang].

Recently, the contribution of inorganic salts (nitrates in particular) to the mass concentration of particulate matter with an aerodynamic diameter of less than 2.5 µm (PM2.5) has been increasing across China. However, it is urgent to understand how the increased inorganic salts affect the crucial properties of PM2.5. Here, we conducted continuous field observations at Zhenjiang Ecology and Environment Protection Bureau from January 1 to December 31, 2021. The mass concentrations of ammonium sulfate[(NH4)2SO4] and ammonium nitrate (NH4NO3) were calculated using different methods. The contributions of (NH4)2SO4 and NH4NO3 to the extinction coefficient, hygroscopic growth, and acidity of PM2.5 were discussed in detail. Our results demonstrated that the mean mass concentrations of (NH4)2SO4 and NH4NO3 during the study period were (6.5±4.5) and (15.0±13.3) µg·m-3, which contributed (20.5±18.2)% and (34.5±18.4)% to the mass concentration of PM2.5, respectively. The total extinction coefficient of PM2.5 was (224.5±194.2) Mm-1, in which NH4NO3 was the largest contributor[(40.1±20.9)%] followed by (NH4)2SO4[(19.1±10.8)%]. (NH4)2SO4 and NH4NO3 were also the dominant contributors to the hygroscopic growth of PM2.5. In particular, NH4NO3contributed from (53.8±13.4)% to (61.6±14.6)% to the aerosol water content of PM2.5 under pollution conditions. Thus, NH4NO3 was a key air pollutant to be targeted for further improving the visibility and air quality in Zhenjiang in the future. However, the reduction in the precursors of NH4NO3 would lead to an increase in aerosol acidity, particularly in the spring and winter seasons. Our results help us understand the evolution of air quality and the related impacts and also provide important information on air quality improvement in Zhenjiang in the future.

Observation of Exceptional Points in Thermal Atomic Ensembles.

Exceptional points (EPs) in non-Hermitian systems have recently attracted wide interest and spawned intriguing prospects for enhanced sensing. However, EPs have not yet been realized in thermal atomic ensembles, which is one of the most important platforms for quantum sensing. Here we experimentally observe EPs in multilevel thermal atomic ensembles and realize enhanced sensing of the magnetic field for 1 order of magnitude. We take advantage of the rich energy levels of atoms and construct effective decays for selected energy levels by employing laser coupling with the excited state, yielding unbalanced decay rates for different energy levels, which finally results in the existence of EPs. Furthermore, we propose the optical polarization rotation measurement scheme to detect the splitting of the resonance peaks, which makes use of both the absorption and dispersion properties and shows an advantage with enhanced splitting compared with the conventional transmission measurement scheme. Additionally, in our system both the effective coupling strength and decay rates are flexibly adjustable, and thus the position of the EPs are tunable, which expands the measurement range. Our Letter not only provides a new controllable platform for studying EPs and non-Hermitian physics, but also provide new ideas for the design of EP-enhanced sensors and opens up realistic opportunities for practical applications in the high-precision sensing of magnetic field and other physical quantities.

PT-Symmetric Feedback Induced Linewidth Narrowing.

Narrow linewidth is a long-pursued goal in precision measurement and sensing. We propose a parity-time symmetric (PT-symmetric) feedback method to narrow the linewidths of resonance systems. By using a quadrature measurement-feedback loop, we transform a dissipative resonance system into a PT-symmetric system. Unlike the conventional PT-symmetric systems that typically require two or more modes, here the PT-symmetric feedback system contains only a single resonance mode, which greatly extends the scope of applications. The method enables remarkable linewidth narrowing and enhancement of measurement sensitivity. We illustrate the concept in a thermal ensemble of atoms, achieving a 48-fold narrowing of the magnetic resonance linewidth. By applying the method in magnetometry, we realize a 22-times improvement of the measurement sensitivity. This work opens the avenue for studying non-Hermitian physics and high-precision measurements in resonance systems with feedback.

Constraints on Spin-Spin Velocity-Dependent Interactions.

The existence of exotic spin-dependent forces may shine light on new physics beyond the standard model. We utilize two iron shielded SmCo_{5} electron-spin sources and two optically pumped magnetometers to search for exotic long-range spin-spin velocity-dependent force. The orientations of spin sources and magnetometers are optimized such that the exotic force is enhanced and common-mode noise is effectively subtracted. We set direct limit on proton-electron interaction in the force range from 1 cm to 1 km. Our experiment represents more than 10 orders of magnitude improvement than previous works.

[Research Progress of SOA Formation from Anthropogenic VOCs Under Complex Pollution Condition].

Although the air quality in China has been greatly improved in recent years, the air pollution remains severe. The annual mean PM2.5 concentrations have not met the second grade of the National Ambient Air Quality Standards in China and are still much higher than the guideline value of the World Health Organization. Thus, the PM2.5 concentration needs to be further reduced. Secondary organic aerosol (SOA) is an important component of PM2.5 and has an important impact on air quality, global climate change, and human health. Therefore, understanding the formation mechanism of SOA is an important basis to control SOA and further reduce PM2.5. As an important precursor of SOA, volatile organic compounds (VOCs) can be oxidized by oxidants such as ·OH, NO3[KG-*2/3]·, Cl·, and O3 to generate low volatile organic compounds and further to form SOA through gas-particle partitioning, homogeneous nucleation, aqueous phase reaction, and heterogeneous reaction processes. The formation of SOA can be affected by many factors, such as the types and initial concentrations of VOCs, VOCs/NOx ratios, relative humidity (RH), temperature (T), seed aerosols, oxidants, aqueous phase process, and photochemical process. The observed SOA concentration is always underestimated by air quality models because a comprehensive understanding of the complexity of SOA chemical composition and formation mechanisms is still lacking, especially that under the highly complex air pollution conditions in China. Therefore, the formation mechanism and influencing factors of SOA under highly complex air pollution conditions have become an important concern in the field of atmospheric sciences. Recently, much laboratory work has focused on the formation of SOA under complex conditions. The research progress of SOA formation from different anthropogenic VOCs are reviewed here, and the methods used and the impact of different influencing factors on SOA formation are introduced. Finally, the key scientific issues that exist in the research of the SOA mechanism at present are put forward, and the future research direction is projected.

Gain-Loss-Induced Hybrid Skin-Topological Effect.

Non-Hermitian topological effects are of crucial importance both in fundamental physics and applications. Here we discover the gain-loss-induced hybrid second-order skin-topological effect and the PT phase transition in skin-topological modes. By studying a non-Hermitian Haldane model, we find that the topological edge modes are localized on a special type of corner, while the bulk modes remain extended. Such an effect originates from the interplay between gain, loss, and the chiral edge currents induced by the nonlocal flux, which can be characterized by considering the properties of the edge sites as a one-dimensional chain. We establish a relation between the skin-topological effect and the PT symmetries belonging to different edges. Moreover, we discover the PT phase transition with the emergence of exceptional points between pairs of skin-topological modes. Our results pave the way for the investigation of non-Hermitian topological physics and PT phase transition in higher-dimensional systems.

On-chip nanophotonic topological rainbow.

The era of Big Data requires nanophotonic chips to have large information processing capacity. Multiple frequency on-chip nanophotonic devices are highly desirable for density integration, but such devices are more susceptible to structural imperfection because of their nano-scale. Topological photonics provides a robust platform for next-generation nanophotonic chips. Here we give an experimental report of an on-chip nanophotonic topological rainbow realized by employing a translational deformation freedom as a synthetic dimension. The topological rainbow can separate, slow, and trap topological photonic states of different frequencies into different positions. A homemade scattering scanning near-field optical microscope with high resolution is introduced to directly measure the topological rainbow effect of the silicon-based photonic chip. The topological rainbow based on synthetic dimension have no restrictions for optical lattice types, symmetries, materials, wavelength band, and is easy for on-chip integration. This work builds a bridge between silicon chip technologies and topological photonics.

Loss-induced nonreciprocity.

Nonreciprocity is important in both optical information processing and topological photonics studies. Conventional principles for realizing nonreciprocity rely on magnetic fields, spatiotemporal modulation, or nonlinearity. Here we propose a generic principle for generating nonreciprocity by taking advantage of energy loss, which is usually regarded as harmful. The loss in a resonance mode induces a phase lag, which is independent of the energy transmission direction. When multichannel lossy resonance modes are combined, the resulting interference gives rise to nonreciprocity, with different coupling strengths for the forward and backward directions, and unidirectional energy transmission. This study opens a new avenue for the design of nonreciprocal devices without stringent requirements.

Atom-Photon Spin-Exchange Collisions Mediated by Rydberg Dressing.

We show that a single photon propagating through a Rydberg-dressed atomic ensemble can exchange its spin state with a single atom. Such a spin-exchange collision exhibits both dissipative and coherent features, depending on the interaction strength. For strong interaction, the collision dissipatively drives the system into an entangled dark state of the photon with an atom. In the weak interaction regime, the scattering coherently flips the spin of a single photon in the multiphoton input pulse, demonstrating a generic single-photon subtracting process. An analytical treatment of this process reveals a universal trade-off between efficiency and purity of the extracted photon, which applies to a wide class of single-photon subtractors. We show that such a trade-off can be optimized by adjusting the scattering rate under a novel phase-matching condition.

Collision-Induced Broadband Optical Nonreciprocity.

Optical nonreciprocity is an essential property for a wide range of applications, such as building nonreciprocal optical devices that include isolators and circulators. The realization of optical nonreciprocity relies on breaking the symmetry associated with Lorentz reciprocity, which typically requires stringent conditions such as introducing a strong magnetic field or a high-finesse cavity with nonreciprocal coupling geometry. Here we discover that the collision effect of thermal atoms, which is undesirable for most studies, can induce broadband optical nonreciprocity. By exploiting the thermal atomic collision, we experimentally observe magnet-free and cavity-free optical nonreciprocity, which possesses a high isolation ratio, ultrabroad bandwidth, and low insertion loss simultaneously. The maximum isolation ratio is close to 40 dB, while the insertion loss is less than 1 dB. The bandwidth for an isolation ratio exceeding 20 dB is over 1.2 GHz, which is 2 orders of magnitude broader than typical resonance-enhanced optical isolators. Our work paves the way for the realization of high-performance optical nonreciprocal devices and provides opportunities for applications in integrated optics and quantum networks.

Hybrid photonic-plasmonic nano-cavity with ultra-high Q/V.

Optical cavities with high figure of merit Q/V is essential to enhance the interaction of light and matter. Here, a hybrid photonic-plasmonic nano-cavity, consisting of an L3 photonic crystal nano-cavity and plasmonic bowtie nano-antennas, is proposed to have an ultrahigh figure of merit Q/V of 8.4×106(λ/n)-3, which is the highest value ever demonstrated for all previous works about L3-type photonic crystal nano-cavities. The value of Q/V is enhanced by more than 25 times compared to that in a bare L3 photonic crystal nano-cavity and is 60 times greater than plasmonic bowtie nano-antennas. As a result, the single-atom cooperativity parameter is improved by 26 times with respect to a bare L3 photonic crystal nano-cavity, and strong coupling between light and a single emitter is achieved. The proposed structure provides a new platform to achieve strong coupling between light and a single emitter, which holds great potential for applications in quantum optics, quantum information, and nonlinear optics.

Optical Forces: From Fundamental to Biological Applications.

Optical forces, generally arising from changes of field gradients or linear momentum carried by photons, form the basis for optical trapping and manipulation. Advances in optical forces help to reveal the nature of light-matter interactions, giving answers to a wide range of questions and solving problems across various disciplines, and are still yielding new insights in many exciting sciences, particularly in the fields of biological technology, material applications, and quantum sciences. This review focuses on recent advances in optical forces, ranging from fundamentals to applications for biological exploration. First, the basics of different types of optical forces with new light-matter interaction mechanisms and near-field techniques for optical force generation beyond the diffraction limit with nanometer accuracy are described. Optical forces for biological applications from in vitro to in vivo are then reviewed. Applications from individual manipulation to multiple assembly into functional biophotonic probes and soft-matter superstructures are discussed. At the end future directions for application of optical forces for biological exploration are provided.

The role of carbon dioxide in acute brain injury.

Carbon dioxide is a common gas in the air which has been widely used in medical treatment. A carbon dioxide molecule consists of two oxygen atoms and one carbon atom through a covalent bond. In the body, carbon dioxide reacts with water to produce carbonic acid. In healthy people, carbon dioxide is maintained within a narrow range (35-45 mmHg) by physiological mechanisms. The role of hypocapnia (partial pressure of carbon dioxide < 35 mmHg) and hypercapnia (partial pressure of carbon dioxide > 45 mmHg) in the nervous system is intricate. Past researches mainly focus on the effect of hypocapnia to nerve protection. Nevertheless, Hypercapnia seems to play an important role in neuroprotection. The mechanisms of hypocapnia and hypercapnia in the nervous system deserve our attention. The purpose of this review is to summarize the effect of hypocapnia and hypercapnia in stroke and traumatic brain injury.

Chaotic synchronization of two optical cavity modes in optomechanical systems.

The synchronization of the motion of microresonators has attracted considerable attention. In previous studies, the microresonators for synchronization were studied mostly in the linear regime. While the important problem of synchronizing nonlinear microresonators was rarely explored. Here we present theoretical methods to synchronize the motions of chaotic optical cavity modes in an optomechanical system, where one of the optical modes is strongly driven into chaotic motion and transfers chaos to other weakly driven optical modes via a common mechanical resonator. This mechanical mode works as a common force acting on each optical mode, which, thus, enables the synchronization of states. We find that complete synchronization can be achieved in two identical chaotic cavity modes. For two arbitrary nonidentical chaotic cavity modes, phase synchronization can also be achieved in the strong-coupling small-detuning regime.

Ultrasmall broadband wavelength and polarization router based on hybrid waveguide of monolithic-LiNbO3.

The nanoscale wavelength and polarization router, which can simultaneously separate wavelength and polarization modes, is an essential component of on-chip nanophotonic devices. Here, an on-chip wavelength and polarization router is realized experimentally based on a three-layer hybrid waveguide of Au-SiO2-LiNbO3 etched with asymmetric nano-cavities. The central area size of the device is only 1.60×1.96 µm2. A broad operation band covers from 500 nm to 1150 nm with low cross talk of under 10 dB. The monolithic-LiNbO3is introduced for the first time, to the best of our knowledge, to on-chip multichannel wavelength and polarization routers. This work plays a key role for dense chip integration, visible light displays, and communications, and can inspire LiNbO3-based nanophotonic devices.

Binding Performance of Human Intravenous Immunoglobulin and 20(S)-7-Ethylcamptothecin.

A previous study showed that intravenous immunoglobulin (IVIG) could preserve higher levels of biologically active lactone moieties of topotecan, 7-ethyl-10-hydroxycamptothecin (SN-38) and 10-hydroxycamptothecin at physiological pH 7.40. As one of camptothecin analogues (CPTs), the interaction of 7-ethylcamptothecin and IVIG was studied in vitro in this study. It was shown that the main binding mode of IVIG to 7-ethylcamptothecin was hydrophobic interaction and hydrogen bonding, which is a non-specific and spontaneous interaction. The hydrophobic antigen-binding cavity of IgG would enwrap the drug into a host-guest inclusion complex and prevent hydrolysis of the encapsulated drug, while the drug is adjacent to the chromophores of IgG and may exchange energy with chromophores and quench the fluorescence of the protein. Also, the typical ß-sheet structure of IVIG unfolded partially after binding to 7-ethylcamptothecin. Additionally, the binding properties of IVIG and six CPTs with different substituents at A-ring and/or B-ring including camptothecin, topotecan, irinotecan, 10-hydroxycamptothecin, 7-ethylcamptothecin and SN-38 were collected together and compared each other. Synergizing with anti-cancer drugs, IVIG could be used as a transporter protein for 7-ethylcamptothecin and other CPTs, allowing clinicians to devise new treatment protocols for patients.

The unexpected diversity of microbial communities associated with black corals revealed by high-throughput Illumina sequencing.

The microbes associated with black corals remain poorly studied. The present study is the first attempt to investigate microbial community structure in the black corals Antipathes ceylonensis and A. dichotoma from the South China Sea by using high-throughput Illumina sequencing. A total of 52 bacterial and 3 archaeal phyla were recovered in this study, suggesting the black corals harboured highly diverse microbial communities. Among the 55 microbial phyla, Proteobacteria, Firmicutes, Bacteroidetes, Chloroflexi, Acidobacteria and Actinobacteria dominated in the two black corals from the South China Sea. Although most of the microbial phyla recovered from the two black corals have been reported in previous studies on coral-associated microbes, eight bacterial phyla including Synergistetes, Thermi, AncK6, GNO2, NKB19, NC10, WWE1 and GAL15, and the archaeal phylum Parvarchaeota are reported for the first time from corals in this study, which expands our knowledge about the diversity of coral-associated microbes. The comparison of microbial communities in the different black coral species indicated that A. ceylonensis harboured few abundant bacterial genera such as Citrobacter and Pseudomonas, whereas a high diversity of rare bacterial genera (<1% abundance), such as Winogradskyella and Rubricoccus, was detected only in A. dichotoma. These results suggested that the microbial community in black corals exhibited species-specific variation.