Observation of Acoustically Induced Dressed States of Rare-Earth Ions.

Acoustically induced dressed states of long-lived erbium ions in a crystal are demonstrated. These states are formed by rapid modulation of two-level systems via strain induced by surface acoustic waves whose frequencies exceed the optical linewidth of the ion ensemble. Multiple sidebands and the reduction of their intensities appearing near the surface are evidence of a strong interaction between the acoustic waves and the ions. This development allows for on-chip control of long-lived ions and paves the way to highly coherent hybrid quantum systems with telecom photons, acoustic phonons, and electrons.

Optical-referenceless optical frequency counter with twelve-digit absolute accuracy.

A simpler and more accurate measurement of absolute optical frequencies (AOFs) is very important for optical communications and navigation systems. To date, an optical reference has been needed for measuring AOFs with twelve-digit accuracy because of the difficulty in measuring them directly. Here, we focus on an electro-optics-modulation comb that can bridge the vast frequency gap between photonics and electronics. We demonstrate an unprecedented method that can directly measure AOFs to an accuracy of twelve digits with an RF frequency counter by simply delivering a frequency-unknown laser into an optical phase modulator. This could open up a new horizon for optical-referenceless optical frequency metrology. Our method can also simultaneously achieve a 100-fold phase-noise reduction in a conventional signal generator. This corresponds to an increase in the transmission speed of wireless communications of by about seven times.

Operation at 1 MHz of 1.7-cycle multiple plate compression at 35-W average output power.

We generate 1.7-cycle and 35-µJ pulses at a 1-MHz repetition rate by using two-stage multiple plate continuum compression of Yb-laser pulses with 80-W average input power. By adjusting the plate positions with careful consideration of the thermal lensing effect due to the high average power, we compress the output pulse with a 184-fs initial duration to 5.7 fs by using only group-delay-dispersion compensation. This pulse achieves a sufficient beam quality (M2 < 1.5) reaching a focused intensity over 1014 W/cm2 and a high spatial-spectral homogeneity (98%). Our study holds promise for a MHz-isolated-attosecond-pulse source for advanced attosecond spectroscopic and imaging technologies with unprecedentedly high signal-to-noise ratios.

Spatially resolved multimode excitation for smooth supercontinuum generation in a SiN waveguide.

We propose a method of supercontinuum light generation enhanced by multimode excitation in a precisely dispersion-engineered deuterated SiN (SiN:D) waveguide. Although a regularly designed SiN-based nonlinear optical waveguide exhibits anomalous dispersion with the fundamental and first-order multimode operation, the center-symmetric light pumping at the input edge has so far inhibited the full potential of the nonlinearity of SiN-based materials. On the basis of numerical analysis and simulation for the SiN:D waveguide, we intentionally applied spatial position offsets to excite the fundamental and higher-order modes to realize bandwidth broadening with flatness. Using this method, we achieved an SNR improvement of up to 18 dB at a wavelength of 0.6 µm with an offset of about 1 µm in the Y-axis direction and found that the contribution was related to the presence of dispersive waves due to the excitation of TE10, and TE01 modes.

Direct f-3f self-referencing using an integrated silicon-nitride waveguide.

We have achieved the simultaneous generation of a 2.6-octave-wide supercontinuum (SC) spectrum over 400-2500 nm and third-harmonic light solely by a dispersion-controlled silicon-nitride waveguide (SiNW). To increase the visible intensity of the SC light component, we fabricated low-loss 5-mm-long deuterated SiNWs with spot-size converters by low-temperature deposition. We succeeded in measuring the carrier-envelope-offset (CEO) signal with a 34-dB signal-to-noise ratio because this short deuterated SiNW provides a large temporal overlap between the f and 3f components. In addition, we have demonstrated this method of CEO locking at telecommunications wavelengths with f-3f self-referencing generated solely by the SiNW without the use of highly nonlinear fiber and an additional nonlinear crystal. Compared with the method of CEO locking with a highly nonlinear fiber and a standard f-2f self-referencing interferometer, this method is not only simple and compact but also stable.

Low-noise optical measurement of sound using midfringe locked interferometer with differential detection.

A midfringe locked interferometer with differential detection is proposed for non-contact optical sound measurement, and the equivalent noise level of approximately 0 dB SPL/Hz is achieved. The noise level of the proposed method is 30 dB lower than that of a very recent laser Doppler vibrometer and close to that of a quarter-inch measurement microphone. The midfringe locking stabilizes the optical interferometer against slow environmental fluctuations and enables detection of the acoustic signal directly from optical intensity. The differential detection method eliminates laser intensity noise, which is a dominant noise source in optical interferometers. The noise level of the constructed system was approximately 10 dB above the optical shot-noise (the classical detection limit attributed to the quantum nature of light) at frequencies higher than 2 kHz. Further noise reduction by several available methods could lead to optical measurements that are more sensitive than measurements by microphones. In addition, the constructed interferometer is used to reconstruct sound fields generated by a half-inch laboratory standard microphone used as a transmitter. The proposed method will be a powerful tool for measuring small-amplitude sound fields where it has been challenging to use existing methods.

Spatially resolved spectral phase interferometry with an isolated attosecond pulse.

We demonstrate spatially resolved supercontinuum spectral phase interferometry with an isolated attosecond pulse (IAP). The measured spatial-spectral interferogram over the broadband region indicates a high degree of IAP coherence in both spatial and spectral domains. In addition, the spectral-delay interferogram shows periodic temporal oscillations over the full IAP continuous spectrum, which indicates high temporal coherence. The supercontinuum spectral phase interferometry with broadband IAP will contribute to exploring spatiotemporal dispersive electronic dynamics through phase-based spectroscopy in the future.

Optical frequency distribution using laser repeater stations with planar lightwave circuits.

We report a cascaded optical fiber link which connects laboratories in RIKEN, the University of Tokyo, and NTT within a 100-km region using a transfer light at 1397 nm, a subharmonic of the Sr clock frequency. The multiple cascaded link employing several laser repeater stations benefits from a wide feedback bandwidth for fiber noise compensation, which allows constructing optical lattice clock networks based on the master-slave configuration. We developed the laser repeater stations based on planar lightwave circuits to significantly reduce the interferometer noise for improved link stability. We implemented a 240-km-long cascaded link in a UTokyo-NTT-UTokyo loop using light sent from RIKEN via a 30-km-long link. In environments with large fiber noise, the link instability is 3 × 10-16 at an averaging time of 1 s and reaches 1 × 10-18 at 2,600 s.

Highly sensitive transient reflection measurement in extreme ultraviolet region for tracking carrier and coherent phonon dynamics.

A highly sensitive method for detecting transient reflection in the extreme ultraviolet (XUV) region was developed on the basis of high-order harmonics for tracking carrier and coherent phonon dynamics. The use of lock-in detection and boxcar integration enables us to observe optical modulation (ΔR/R) as high as 1 × 10-4, and the data acquisition takes only four minutes. XUV transient reflections of bismuth exhibited exponential decay originating from excited carriers and periodic oscillation originating from A1g optical phonons. The linear power dependence of the electronic and phonon amplitudes indicated that one-photon excitation occurred under the experimental conditions. The cosine of the initial phase of the phonon oscillation revealed that a displacive excitation mechanism contributed to phonon generation. The phonon parameters obtained by the XUV and NIR probes were consistent even though their penetration depths were different. The result indicated that the XUV and NIR pulses probe the same excited region, which should be near the surface due to the short penetration depth of the NIR pump pulses. The present highly sensitive means of detecting XUV transient reflections in solid-state materials could be utilized for detecting attosecond dynamics in the future.

Multi-petahertz electron interference in Cr:Al2O3 solid-state material.

Lightwave-field-induced ultrafast electric dipole oscillation is promising for realizing petahertz (1015 Hz: PHz) signal processing in the future. In building the ultrahigh-clock-rate logic operation system, one of the major challenges will be petahertz electron manipulation accompanied with multiple frequencies. Here we study multi-petahertz interference with electronic dipole oscillations in alumina with chromium dopant (Cr:Al2O3). An intense near-infrared lightwave-field induces multiple electric inter-band polarizations, which are characterized by Fourier transform extreme ultraviolet attosecond spectroscopy. The interference results from the superposition state of periodic dipole oscillations of 667 to 383 attosecond (frequency of 1.5 to 2.6 PHz) measured by direct time-dependent spectroscopy and consists of various modulations on attosecond time scale through individual electron dephasing times of the Cr donor-like and Al2O3 conduction band states. The results indicate the possible manipulation of petahertz interference signal with multiple dipole oscillations using material band engineering and such a control will contribute to the study of ultrahigh-speed signal operation.

Characterizing inner-shell with spectral phase interferometry for direct electric-field reconstruction.

In many atomic, molecular and solid systems, Lorentzian and Fano profiles are commonly observed in a broad research fields throughout a variety of spectroscopies. As the profile structure is related to the phase of the time-dependent dipole moment, it plays an important role in the study of quantum properties. Here we determine the dipole phase in the inner-shell transition using spectral phase interferometry for direct electric-field reconstruction (SPIDER) with isolated attosecond pulses (IAPs). In addition, we propose a scheme for pulse generation and compression by manipulating the inner-shell transition. The electromagnetic radiation generated by the transition is temporally compressed to a few femtoseconds in the extreme ultraviolet (XUV) region. The proposed pulse-compression scheme may provide an alternative route to producing attosecond pulses of light.

Dynamical study of femtosecond-laser-ablated liquid-aluminum nanoparticles using spatiotemporally resolved x-ray-absorption fine-structure spectroscopy.

We study the temperature evolution of aluminum nanoparticles generated by femtosecond laser ablation with spatiotemporally resolved x-ray-absorption fine-structure spectroscopy. We successfully identify the nanoparticles based on the L-edge absorption fine structure of the ablation plume in combination with the dependence of the edge structure on the irradiation intensity and the expansion velocity of the plume. In particular, we show that the lattice temperature of the nanoparticles is estimated from the L-edge slope, and that its spatial dependence reflects the cooling of the nanoparticles during plume expansion. The results reveal that the emitted nanoparticles travel in a vacuum as a condensed liquid phase with a lattice temperature of about 2500 to 4200 K in the early stage of plume expansion.

Sampling measurement of soft-x-ray-pulse shapes by femtosecond sequential ionization of Kr+ in an intense laser field.

We propose a sampling technique for measuring the shape of ultrashort soft-x-ray pulses. The technique uses the transient state of Kr+ ions that is produced by the femtosecond sequential evolution of Kr ions during optical-field-induced ionization as an ultrafast x-ray-absorption sampling gate. We demonstrate the technique by measuring the pulse shape of the 51st harmonic (15.6 nm) generated by a 100-fs titanium:sapphire laser pulse. The measured pulse duration is 220 fs. Our experimental result confirms that the sequential evolution of Kr+ ions from neutral Kr to Kr2+ is the dominant contribution to the ionization process from the aspect of time-domain measurement.