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Nat Commun ; 9(1): 1446, 2018 04 13.
Artigo em Inglês | MEDLINE | ID: mdl-29654315

RESUMO

DNA nanotechnology has enabled complex nanodevices, but the ability to directly manipulate systems with fast response times remains a key challenge. Current methods of actuation are relatively slow and only direct devices into one or two target configurations. Here we report an approach to control DNA origami assemblies via externally applied magnetic fields using a low-cost platform that enables actuation into many distinct configurations with sub-second response times. The nanodevices in these assemblies are manipulated via mechanically stiff micron-scale lever arms, which rigidly couple movement of a micron size magnetic bead to reconfiguration of the nanodevice while also enabling direct visualization of the conformation. We demonstrate control of three assemblies-a rod, rotor, and hinge-at frequencies up to several Hz and the ability to actuate into many conformations. This level of spatiotemporal control over DNA devices can serve as a foundation for real-time manipulation of molecular and atomic systems.


Assuntos
DNA de Cadeia Simples/química , Nanoestruturas , Nanotecnologia/métodos , Magnetismo , Microscopia de Força Atômica , Microscopia Eletrônica de Transmissão , Conformação de Ácido Nucleico , Oscilometria , Propriedades de Superfície , Gravação em Vídeo
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