Evidence for chiral supercurrent in quantum Hall Josephson junctions.

Hybridizing superconductivity with the quantum Hall (QH) effect has notable potential for designing circuits capable of inducing and manipulating non-Abelian states for topological quantum computation1-3. However, despite recent experimental progress towards this hybridization4-15, concrete evidence for a chiral QH Josephson junction16-the elemental building block for coherent superconducting QH circuits-is still lacking. Its expected signature is an unusual chiral supercurrent flowing in QH edge channels, which oscillates with a specific 2ϕ0 magnetic flux periodicity16-19 (ϕ0 = h/2e is the superconducting flux quantum, where h is the Planck constant and e is the electron charge). Here we show that ultra-narrow Josephson junctions defined in encapsulated graphene nanoribbons exhibit a chiral supercurrent, visible up to 8 T and carried by the spin-degenerate edge channel of the QH plateau of resistance h/2e2 ≈ 12.9 kΩ. We observe reproducible 2ϕ0-periodic oscillations of the supercurrent, which emerge at a constant filling factor when the area of the loop formed by the QH edge channel is constant, within a magnetic-length correction that we resolve in the data. Furthermore, by varying the junction geometry, we show that reducing the superconductor/normal interface length is crucial in obtaining a measurable supercurrent on QH plateaus, in agreement with theories predicting dephasing along the superconducting interface19-22. Our findings are important for the exploration of correlated and fractional QH-based superconducting devices that host non-Abelian Majorana and parafermion zero modes23-32.

Coulomb-mediated antibunching of an electron pair surfing on sound.

Electron flying qubits are envisioned as potential information links within a quantum computer, but also promise-like photonic approaches-to serve as self-standing quantum processing units. In contrast to their photonic counterparts, electron-quantum-optics implementations are subject to Coulomb interactions, which provide a direct route to entangle the orbital or spin degree of freedom. However, controlled interaction of flying electrons at the single-particle level has not yet been established experimentally. Here we report antibunching of a pair of single electrons that is synchronously shuttled through a circuit of coupled quantum rails by means of a surface acoustic wave. The in-flight partitioning process exhibits a reciprocal gating effect which allows us to ascribe the observed repulsion predominantly to Coulomb interaction. Our single-shot experiment marks an important milestone on the route to realize a controlled-phase gate for in-flight quantum manipulations.

Absence of edge reconstruction for quantum Hall edge channels in graphene devices.

Quantum Hall (QH) edge channels propagating along the periphery of two-dimensional (2D) electron gases under perpendicular magnetic field are a major paradigm in physics. However, groundbreaking experiments that could use them in graphene are hampered by the conjecture that QH edge channels undergo a reconstruction with additional nontopological upstream modes. By performing scanning tunneling spectroscopy up to the edge of a graphene flake on hexagonal boron nitride, we show that QH edge channels are confined to a few magnetic lengths at the crystal edges. This implies that they are ideal 1D chiral channels defined by boundary conditions of vanishing electronic wave functions at the crystal edges, hence free of electrostatic reconstruction. We further evidence a uniform charge carrier density at the edges, incompatible with the existence of upstream modes. This work has profound implications for electron and heat transport experiments in graphene-based systems and other 2D crystalline materials.

Imaging tunable quantum Hall broken-symmetry orders in graphene.

ABSTARCT: When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy1-5. The zeroth Landau level of graphene under a magnetic field is a particularly interesting strongly interacting flat band because interelectron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders6-11. Evidence for these states stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy12 or by dielectric screening of the Coulomb interaction13. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders14. Here we image three distinct broken-symmetry phases in graphene using scanning tunnelling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low- or high-dielectric-constant environment, and with a magnetic field. In the unscreened case, we find a Kekulé bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition15,16. Under dielectric screening, a sublattice-unpolarized ground state13 emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekulé and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions6-10. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials.

A tunable Fabry-Pérot quantum Hall interferometer in graphene.

Electron interferometry with quantum Hall (QH) edge channels in semiconductor heterostructures can probe and harness the exchange statistics of anyonic excitations. However, the charging effects present in semiconductors often obscure the Aharonov-Bohm interference in QH interferometers and make advanced charge-screening strategies necessary. Here we show that high-mobility monolayer graphene constitutes an alternative material system, not affected by charging effects, for performing Fabry-Pérot QH interferometry in the integer QH regime. In devices equipped with gate-tunable quantum point contacts acting on the edge channels of the zeroth Landau level, we observe-in agreement with theory-high-visibility Aharonov-Bohm interference widely tunable through electrostatic gating or magnetic fields. A coherence length of 10 µm at a temperature of 0.02 K allows us to further achieve coherently coupled double Fabry-Pérot interferometry. In future, QH interferometry with graphene devices may enable investigations of anyonic excitations in fractional QH states.

Helical quantum Hall phase in graphene on SrTiO3.

The ground state of charge-neutral graphene under perpendicular magnetic field was predicted to be a quantum Hall topological insulator with a ferromagnetic order and spin-filtered, helical edge channels. In most experiments, however, an insulating state is observed that is accounted for by lattice-scale interactions that promote a broken-symmetry state with gapped bulk and edge excitations. We tuned the ground state of the graphene zeroth Landau level to the topological phase through a suitable screening of the Coulomb interaction with the high dielectric constant of a strontium titanate (SrTiO3) substrate. Robust helical edge transport emerged at magnetic fields as low as 1 tesla and withstanding temperatures up to 110 kelvin over micron-long distances. This versatile graphene platform may find applications in spintronics and topological quantum computation.

Low-Magnetic-Field Regime of a Gate-Defined Constriction in High-Mobility Graphene.

We report on the evolution of the coherent electronic transport through a gate-defined constriction in a high-mobility graphene device from ballistic transport to quantum Hall regime upon increasing the magnetic field. At a low field, the conductance exhibits Fabry-Pérot resonances resulting from the npn cavities formed beneath the top-gated regions. Above a critical field B* corresponding to the cyclotron radius equal to the npn cavity length, Fabry-Pérot resonances vanish, and snake trajectories are guided through the constriction with a characteristic set of conductance oscillations. Increasing further the magnetic field allows us to probe the Landau level spectrum in the constriction and unveil distortions due to the combination of confinement and deconfinement of Landau levels in a saddle potential. These observations are confirmed by numerical calculations.

On the origins of transport inefficiencies in mesoscopic networks.

A counter-intuitive behavior analogous to the Braess paradox is encountered in a two-terminal mesoscopic network patterned in a two-dimensional electron system (2DES). Decreasing locally the electron density of one channel of the network paradoxically leads to an increased network electrical conductance. Our low temperature scanning gate microscopy experiments reveal different occurrences of such puzzling conductance variations, thanks to tip-induced localized modifications of electron flow throughout the network's channels in the ballistic and coherent regime of transport. The robustness of the puzzling behavior is inspected by varying the global 2DES density, magnetic field and the tip-surface distance. Depending on the overall 2DES density, we show that either Coulomb Blockade resonances due to disorder-induced localized states or Fabry-Perot interferences tuned by the tip-induced electrostatic perturbation are at the origin of transport inefficiencies in the network, which are lifted when gradually closing one channel of the network with the tip.

Tunable transmission of quantum Hall edge channels with full degeneracy lifting in split-gated graphene devices.

Charge carriers in the quantum Hall regime propagate via one-dimensional conducting channels that form along the edges of a two-dimensional electron gas. Controlling their transmission through a gate-tunable constriction, also called quantum point contact, is fundamental for many coherent transport experiments. However, in graphene, tailoring a constriction with electrostatic gates remains challenging due to the formation of p-n junctions below gate electrodes along which electron and hole edge channels co-propagate and mix, short circuiting the constriction. Here we show that this electron-hole mixing is drastically reduced in high-mobility graphene van der Waals heterostructures thanks to the full degeneracy lifting of the Landau levels, enabling quantum point contact operation with full channel pinch-off. We demonstrate gate-tunable selective transmission of integer and fractional quantum Hall edge channels through the quantum point contact. This gate control of edge channels opens the door to quantum Hall interferometry and electron quantum optics experiments in the integer and fractional quantum Hall regimes of graphene.

A new transport phenomenon in nanostructures: a mesoscopic analog of the Braess paradox encountered in road networks.

The Braess paradox, known for traffic and other classical networks, lies in the fact that adding a new route to a congested network in an attempt to relieve congestion can degrade counterintuitively the overall network performance. Recently, we have extended the concept of the Braess paradox to semiconductor mesoscopic networks, whose transport properties are governed by quantum physics. In this paper, we demonstrate theoretically that, alike in classical systems, congestion plays a key role in the occurrence of a Braess paradox in mesoscopic networks.

Half-integer Shapiro steps at the 0-pi crossover of a ferromagnetic Josephson junction.

We investigate the current-phase relation of S/F/S junctions near the crossover between the 0 and the pi ground states. We use Nb/CuNi/Nb junctions where this crossover is driven both by thickness and temperature. For a certain thickness a nonzero minimum of critical current is observed at the crossover temperature. We analyze this residual supercurrent by applying a high frequency excitation and observe the formation of half-integer Shapiro steps. We attribute these fractional steps to a doubling of the Josephson frequency due to a sin((2phi) current-phase relation. This phase dependence is explained by the splitting of the energy levels in the ferromagnetic exchange field.