Entanglement with tweezed molecules.

Controlled molecular connection will advance quantum technologies.

Hierarchies of Frequentist Bounds for Quantum Metrology: From Cramér-Rao to Barankin.

We derive lower bounds on the variance of estimators in quantum metrology by choosing test observables that define constraints on the unbiasedness of the estimator. The quantum bounds are obtained by analytical optimization over all possible quantum measurements and estimators that satisfy the given constraints. We obtain hierarchies of increasingly tight bounds that include the quantum Cramér-Rao bound at the lowest order. In the opposite limit, the quantum Barankin bound is the variance of the locally best unbiased estimator in quantum metrology. Our results reveal generalizations of the quantum Fisher information that are able to avoid regularity conditions and identify threshold behavior in quantum measurements with mixed states, caused by finite data.

Tomography of a Number-Resolving Detector by Reconstruction of an Atomic Many-Body Quantum State.

The high-fidelity analysis of many-body quantum states of indistinguishable atoms requires the accurate counting of atoms. Here we report the tomographic reconstruction of an atom-number-resolving detector. The tomography is performed with an ultracold rubidium ensemble that is prepared in a coherent spin state by driving a Rabi coupling between the two hyperfine clock levels. The coupling is followed by counting the occupation number in one level. We characterize the fidelity of our detector and show that a negative-valued Wigner function is associated with it. Our results offer an exciting perspective for the high-fidelity reconstruction of entangled states and can be applied for a future demonstration of Heisenberg-limited atom interferometry.

Delta-Kick Squeezing.

We explore the possibility to overcome the standard quantum limit (SQL) in a free-fall atom interferometer using a Bose-Einstein condensate (BEC) in either of the two relevant cases of Bragg or Raman scattering light pulses. The generation of entanglement in the BEC is dramatically enhanced by amplifying the atom-atom interactions via the rapid action of an external trap, focusing the matter waves to significantly increase the atomic densities during a preparation stage-a technique we refer to as delta-kick squeezing (DKS). The action of a second DKS operation at the end of the interferometry sequence allows one to implement a nonlinear readout scheme, making the sub-SQL sensitivity highly robust against imperfect atom counting detection. We predict more than 30 dB of sensitivity gain beyond the SQL for the variance, assuming realistic parameters and 10^{6} atoms.

Genuine Multipartite Nonlocality with Causal-Diagram Postselection.

The generation and verification of genuine multipartite nonlocality (GMN) is of central interest for both fundamental research and quantum technological applications, such as quantum privacy. To demonstrate GMN in measurement data, the statistics are commonly postselected by neglecting undesired data. Until now, valid postselection strategies have been restricted to local postselection. A general postselection that is decided after communication between parties can mimic nonlocality, even though the complete data are local. Here, we establish conditions under which GMN is demonstrable even if observations are postselected collectively. Intriguingly, certain postselection strategies that require communication among several parties still offer a demonstration of GMN shared between all parties. The results are derived using the causal structure of the experiment and the no-signaling condition imposed by relativity. Finally, we apply our results to show that genuine three-partite nonlocality can be created with independent particle sources.

Interferometric Order Parameter for Excited-State Quantum Phase Transitions in Bose-Einstein Condensates.

Excited-state quantum phase transitions extend the notion of quantum phase transitions beyond the ground state. They are characterized by closing energy gaps amid the spectrum. Identifying order parameters for excited-state quantum phase transitions poses, however, a major challenge. We introduce a topological order parameter that distinguishes excited-state phases in a large class of mean-field models and can be accessed by interferometry in current experiments with spinor Bose-Einstein condensates. Our work opens a way for the experimental characterization of excited-state quantum phases in atomic many-body systems.

Metrological Detection of Multipartite Entanglement from Young Diagrams.

We characterize metrologically useful multipartite entanglement by representing partitions with Young diagrams. We derive entanglement witnesses that are sensitive to the shape of Young diagrams and show that Dyson's rank acts as a resource for quantum metrology. Common quantifiers, such as the entanglement depth and k-separability are contained in this approach as the diagram's width and height. Our methods are experimentally accessible in a wide range of atomic systems, as we illustrate by analyzing published data on the quantum Fisher information and spin-squeezing coefficients.

Quantifying computational advantage of Grover's algorithm with the trace speed.

Despite intensive research, the physical origin of the speed-up offered by quantum algorithms remains mysterious. No general physical quantity, like, for instance, entanglement, can be singled out as the essential useful resource. Here we report a close connection between the trace speed and the quantum speed-up in Grover's search algorithm implemented with pure and pseudo-pure states. For a noiseless algorithm, we find a one-to-one correspondence between the quantum speed-up and the polarization of the pseudo-pure state, which can be connected to a wide class of quantum statistical speeds. For time-dependent partial depolarization and for interrupted Grover searches, the speed-up is specifically bounded by the maximal trace speed that occurs during the algorithm operations. Our results quantify the quantum speed-up with a physical resource that is experimentally measurable and related to multipartite entanglement and quantum coherence.

Heisenberg-Limited Noisy Atomic Clock Using a Hybrid Coherent and Squeezed State Protocol.

We propose a hybrid quantum-classical atomic clock where the interrogation of atoms prepared in a spin-coherent (or weakly squeezed) state is used to feed back one or more highly spin-squeezed atomic states toward their optimal phase-sensitivity point. The hybrid clock overcomes the stability of a single Ramsey clock using coherent or optimal spin-squeezed states and reaches a Heisenberg-limited stability while avoiding nondestructive measurements. When optimized with respect to the total number of particles, the protocol surpasses the state-of-the-art proposals that use Greenberger-Horne-Zeilinger or NOON states. We compare analytical predictions with numerical simulations of clock operations, including correlated 1/f local oscillator noise.

Multiparameter squeezing for optimal quantum enhancements in sensor networks.

Squeezing currently represents the leading strategy for quantum enhanced precision measurements of a single parameter in a variety of continuous- and discrete-variable settings and technological applications. However, many important physical problems including imaging and field sensing require the simultaneous measurement of multiple unknown parameters. The development of multiparameter quantum metrology is yet hindered by the intrinsic difficulty in finding saturable sensitivity bounds and feasible estimation strategies. Here, we derive the general operational concept of multiparameter squeezing, identifying metrologically useful states and optimal estimation strategies. When applied to spin- or continuous-variable systems, our results generalize widely-used spin- or quadrature-squeezing parameters. Multiparameter squeezing provides a practical and versatile concept that paves the way to the development of quantum-enhanced estimation of multiple phases, gradients, and fields, and for the efficient characterization of multimode quantum states in atomic and optical sensor networks.

Motional Fock states for quantum-enhanced amplitude and phase measurements with trapped ions.

The quantum noise of the vacuum limits the achievable sensitivity of quantum sensors. In non-classical measurement schemes the noise can be reduced to overcome this limitation. However, schemes based on squeezed or Schrödinger cat states require alignment of the relative phase between the measured interaction and the non-classical quantum state. Here we present two measurement schemes on a trapped ion prepared in a motional Fock state for displacement and frequency metrology that are insensitive to this phase. The achieved statistical uncertainty is below the standard quantum limit set by quantum vacuum fluctuations, enabling applications in spectroscopy and mass measurements.

Metrological Nonlinear Squeezing Parameter.

The well-known metrological linear squeezing parameters (such as quadrature or spin squeezing) efficiently quantify the sensitivity of Gaussian states. Yet, these parameters are insufficient to characterize the much wider class of highly sensitive non-Gaussian states. Here, we introduce a class of metrological nonlinear squeezing parameters obtained by analytical optimization of measurement observables among a given set of accessible (possibly nonlinear) operators. This allows for the metrological characterization of non-Gaussian quantum states of discrete and continuous variables. Our results lead to optimized and experimentally feasible recipes for a high-precision moment-based estimation of a phase parameter and can be used to systematically construct multipartite entanglement and nonclassicality witnesses for complex quantum states.

Sensitivity Bounds for Multiparameter Quantum Metrology.

We identify precision limits for the simultaneous estimation of multiple parameters in multimode interferometers. Quantum strategies to enhance the multiparameter sensitivity are based on entanglement among particles, modes, or combining both. The maximum attainable sensitivity of particle-separable states defines the multiparameter shot-noise limit, which can be surpassed without mode entanglement. Further enhancements up to the multiparameter Heisenberg limit are possible by adding mode entanglement. Optimal strategies that saturate the precision bounds are provided.

Multipartite Entanglement at Finite Temperature.

The interplay of quantum and thermal fluctuations in the vicinity of a quantum critical point characterizes the physics of strongly correlated systems. Here we investigate this interplay from a quantum information perspective presenting the universal phase diagram of the quantum Fisher information at a quantum phase transition. Different regions in the diagram are identified by characteristic scaling laws of the quantum Fisher information with respect to temperature. This feature has immediate consequences on the thermal robustness of quantum coherence and multipartite entanglement. We support the theoretical predictions with the analysis of paradigmatic spin systems showing symmetry-breaking quantum phase transitions and free-fermion models characterized by topological phases. In particular we show that topological systems are characterized by the survival of large multipartite entanglement, reaching the Heisenberg limit at finite temperature.

Hyper- and hybrid nonlocality.

The controlled generation and identification of quantum correlations, usually encoded in either qubits or continuous degrees of freedom, builds the foundation of quantum information science. Recently, more sophisticated approaches, involving a combination of two distinct degrees of freedom, have been proposed to improve on the traditional strategies. Hyperentanglement describes simultaneous entanglement in more than one distinct degree of freedom, whereas hybrid entanglement refers to entanglement shared between a discrete and a continuous degree of freedom. In this work we propose a scheme that allows us to combine the two approaches, and to extend them to the strongest form of quantum correlations. Specifically, we show how two identical, initially separated particles can be manipulated to produce Bell nonlocality among their spins, among their momenta, as well as across their spins and momenta. We discuss possible experimental realizations with atomic and photonic systems.

Role of Particle Entanglement in the Violation of Bell Inequalities.

Entanglement between two separate systems is a necessary resource to violate a Bell inequality in a test of local realism. We demonstrate that to overcome the Bell bound, this correlation must be accompanied by the entanglement between the constituent particles. This happens whenever a super-selection rule prohibits coherences between states with different total number of particles and thus imposes a constraint on feasible local operations in each sub-system. We show that the necessary entanglement between the particles might solely result from their indistinguishability. We also give an example of both mode and particle-entangled pure state, which does not violate any Bell inequality. Our result reveals a fundamental relation between the non-locality and the particle entanglement.

Frequentist and Bayesian Quantum Phase Estimation.

Frequentist and Bayesian phase estimation strategies lead to conceptually different results on the state of knowledge about the true value of an unknown parameter. We compare the two frameworks and their sensitivity bounds to the estimation of an interferometric phase shift limited by quantum noise, considering both the cases of a fixed and a fluctuating parameter. We point out that frequentist precision bounds, such as the Cramér-Rao bound, for instance, do not apply to Bayesian strategies and vice versa. In particular, we show that the Bayesian variance can overcome the frequentist Cramér-Rao bound, which appears to be a paradoxical result if the conceptual difference between the two approaches are overlooked. Similarly, bounds for fluctuating parameters make no statement about the estimation of a fixed parameter.

Multipartite Entanglement in Topological Quantum Phases.

We witness multipartite entanglement in the ground state of the Kitaev chain-a benchmark model of a one dimensional topological superconductor-also with variable-range pairing, using the quantum Fisher information. Phases having a finite winding number, for both short- and long-range pairing, are characterized by a power-law diverging finite-size scaling of multipartite entanglement. Moreover, the occurring quantum phase transitions are sharply marked by the divergence of the derivative of the quantum Fisher information, even in the absence of a closing energy gap.

Optimal Measurements for Simultaneous Quantum Estimation of Multiple Phases.

A quantum theory of multiphase estimation is crucial for quantum-enhanced sensing and imaging and may link quantum metrology to more complex quantum computation and communication protocols. In this Letter, we tackle one of the key difficulties of multiphase estimation: obtaining a measurement which saturates the fundamental sensitivity bounds. We derive necessary and sufficient conditions for projective measurements acting on pure states to saturate the ultimate theoretical bound on precision given by the quantum Fisher information matrix. We apply our theory to the specific example of interferometric phase estimation using photon number measurements, a convenient choice in the laboratory. Our results thus introduce concepts and methods relevant to the future theoretical and experimental development of multiparameter estimation.

Witnessing entanglement without entanglement witness operators.

Quantum mechanics predicts the existence of correlations between composite systems that, although puzzling to our physical intuition, enable technologies not accessible in a classical world. Notwithstanding, there is still no efficient general method to theoretically quantify and experimentally detect entanglement of many qubits. Here we propose to detect entanglement by measuring the statistical response of a quantum system to an arbitrary nonlocal parametric evolution. We witness entanglement without relying on the tomographic reconstruction of the quantum state, or the realization of witness operators. The protocol requires two collective settings for any number of parties and is robust against noise and decoherence occurring after the implementation of the parametric transformation. To illustrate its user friendliness we demonstrate multipartite entanglement in different experiments with ions and photons by analyzing published data on fidelity visibilities and variances of collective observables.