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1.
Data Brief ; 32: 106202, 2020 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-32953952

RESUMO

This work describes the data collection of new lipophilic esters and amides herbicides, analogues to 2,4-dichlorophenoxyacetic acid (2,4-D) and Propanil. The data include 1H and 13C NMR spectra and UV-VIS spectroscopic experiments, from the work "Novel lipophilic analogues from 2,4-D and Propanil herbicides: Biological activity and kinetic studies". The UV-VIS and 1H NMR spectra were employed to kinetic degradation design, and could be used to access new herbicides derivatives with better environmental properties.

2.
Chem Phys Lipids ; 231: 104947, 2020 09.
Artigo em Inglês | MEDLINE | ID: mdl-32622838

RESUMO

This work describes the synthesis of new lipophilic amides and esters analogues of classical organochlorides herbicides by incorporation of long-chains from fatty acids and derivatives. The new fatty esters and amides were synthesized in 96-99% and 80-89% yields, respectively. In general, all compounds tested showed superior in vitro activity than commercial herbicides against growth L. sativa and A. cepa, in ranges 86-100% of germinative inhibition. The target compounds showed, significantly more susceptible towards acid hydrolysis than 2,4-dichlorophenoxyacetic acid (2,4-D). The kinetic and NMR studies showed that the incorporation of lipophilic chains resulted in a decrease in half-life time of new herbicides compounds (1.5 h) than 2,4-D (3 h). These findings suggest the synthesis of new lipophilic herbicides as potential alternative to traditional formulations, by incorporation of long fatty alkyl chains in the molecular structure of 2,4-D, resulting in superior in vitro herbicidal activity, best degradation behavior and more hydrophobic derivatives.


Assuntos
Ácido 2,4-Diclorofenoxiacético/farmacologia , Amidas/farmacologia , Ésteres/farmacologia , Herbicidas/farmacologia , Propanil/farmacologia , Ácido 2,4-Diclorofenoxiacético/química , Amidas/síntese química , Amidas/química , Ésteres/síntese química , Ésteres/química , Herbicidas/química , Interações Hidrofóbicas e Hidrofílicas , Cinética , Estrutura Molecular , Cebolas/efeitos dos fármacos , Cebolas/crescimento & desenvolvimento , Oryza/efeitos dos fármacos , Oryza/crescimento & desenvolvimento , Propanil/química
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