RESUMO
This investigation quantifies the activity concentrations of natural radionuclides (226Ra, 232Th, and 40K) in the soils and certain rocks of the Koytash-Ugam Range, Uzbekistan, and assesses their radiological risks. Gamma-spectrometric analysis of soil and rock samples revealed activity concentrations ranging from 456.2 ± 56.0 to 813.9 ± 76.0 Bq kg-1 for 40K, 18.2 ± 6.3 to 70.0 ± 12.0 Bq kg-1 for 226Ra, and 30.1 ± 2.9 to 57.9 ± 10 Bq kg-1 for 232Th. This data indicates a heterogeneous distribution of radionuclides, informing radiation safety and health risk assessments on a global scale. The calculation of radiological hazard indices, including the alpha-index (ranging from 0.09 to 0.35), gamma-index (ranging from 0.40 to 0.73), and both internal (ranging from 0.40 to 0.54) and external (ranging from 0.36 to 0.54) hazard indices, was undertaken to ascertain potential health risks. The radium equivalent activity ranged from 108.4 to 199.3 Bq kg-1, and the absorbed dose rates were 51.0-93.3 nGy h-1 indoors and 96.6-178.2 nGy h-1 outdoors. These metrics underlie the estimated annual effective dose of 536.5-988.5 × 10-3 mSv y-1, highlighting the variability in radiation exposure. Additionally, the potential lifetime cancer risk was projected at 1770.4 to 3262.0 per million, with an annual gonadal dose equivalent of 361.9 to 655.5 µSv y-1, reflecting natural background radiation influence. The results underscore the importance of safe material use in construction and the necessity for routine natural radioactivity monitoring. Radon flux density (RFD) values within acceptable construction limits (26-176 mBq m-2 s-1) suggest the area's suitability for development, considering recommended safety guidelines. This study not only aids local environmental and public health frameworks but also enriches the international knowledge base, facilitating comparative studies for the advancement of global radiation protection standards. Through a detailed examination of radionuclide distribution in an under-researched area, our research highlights the critical need for integrated international approaches to natural radiological hazard assessment.
Assuntos
Monitoramento de Radiação , Rádio (Elemento) , Poluentes Radioativos do Solo , Tório , Poluentes Radioativos do Solo/análise , Uzbequistão , Rádio (Elemento)/análise , Tório/análise , Solo/química , Medição de Risco , Radioisótopos de Potássio/análise , Radiação de FundoRESUMO
This study investigates soil radioactivity at the Pomuk gas field in Uzbekistan, a region with history of underground nuclear activity. Using a NaI (Tl) scintillation gamma spectrometer, soil samples were analyzed for concentrations of 232Th, 226Ra, 40K, and 137Cs. Concentrations were found to be in the range of 19.0-31.0 Bq/kg for 232Th, 12.0-32.0 Bq/kg for 226Ra, 450.0-634.0 Bq/kg for 40K, and 2.4-11.0 Bq/kg for 137Cs. Surface radon flux density was measured using a coal sorbent-based passive method, with values ranging from 26.1 to 79.0 mBq/m2s. Mean activity values for radium equivalent (Raeq) and gamma representative level index (Iγ) were calculated to be 75.2-96.5 Bq/kg and 0.3-0.4 Bq/kg, respectively. The absorbed airborne gamma dose rates (GDR) varied between 41.0 and 52.0 nGy/h, while annual effective dose rates (AEDR) were 0.3-0.4 µSv/year. The radiological risk assessment indicates the area is within safe limits for the population and environment, providing a foundation for future radiological monitoring programs.
Assuntos
Monitoramento de Radiação , Radioatividade , Rádio (Elemento) , Poluentes Radioativos do Solo , Solo , Uzbequistão , Explosões , Campos de Petróleo e Gás , Monitoramento Ambiental , Poluentes Radioativos do Solo/análise , Monitoramento de Radiação/métodos , Radioisótopos de Potássio/análise , Rádio (Elemento)/análise , Tório/análise , Espectrometria gamaRESUMO
Natural radioactivity is a public health issue that affects people all around the world. Environmental radioactivity accounts for approximately 87% of the radiation dose received by human beings. The primary external source of irradiation to the human body is gamma radiation emitted by naturally occurring radioisotopes such as 40K and radionuclides from the 232Th and 238U families, as well as their decay products, which exist at trace amounts in all ground formations. The establishment of baseline data for environmental radiological studies is of great importance for the assessment of environmental radiological levels in Uzbekistan and related studies on human health risks. The current study aimed to describe the research state of the art on natural radioactivity in Uzbekistan with emphasis on results obtained during the last 20 years. NaI (Tl) and High Purity Germanium HPGe detectors were employed in most conducted studies. The results showed that data for natural radionuclide activity were below international standards in all but a few areas. The research results of this paper can play a good guidance and reference role in the planning of such research in the future.