Geometrical Bounds on Irreversibility in Squeezed Thermal Bath.

Irreversible entropy production (IEP) plays an important role in quantum thermodynamic processes. Here, we investigate the geometrical bounds of IEP in nonequilibrium thermodynamics by exemplifying a system coupled to a squeezed thermal bath subject to dissipation and dephasing, respectively. We find that the geometrical bounds of the IEP always shift in a contrary way under dissipation and dephasing, where the lower and upper bounds turning to be tighter occur in the situation of dephasing and dissipation, respectively. However, either under dissipation or under dephasing, we may reduce both the critical time of the IEP itself and the critical time of the bounds for reaching an equilibrium by harvesting the benefits of squeezing effects in which the values of the IEP, quantifying the degree of thermodynamic irreversibility, also become smaller. Therefore, due to the nonequilibrium nature of the squeezed thermal bath, the system-bath interaction energy has a prominent impact on the IEP, leading to tightness of its bounds. Our results are not contradictory with the second law of thermodynamics by involving squeezing of the bath as an available resource, which can improve the performance of quantum thermodynamic devices.

Cavity spectral-hole-burning to boost coherence in plasmon-emitter strong coupling systems.

Significant decoherence of the plasmon-emitter (i.e., plexcitonic) strong coupling systems hinders the progress towards their applications in quantum technology due to the unavoidable lossy nature of the plasmons. Inspired by the concept of spectral-hole-burning (SHB) for frequency-selective bleaching of the emitter ensemble, we propose 'cavity SHB' by introducing cavity modes with moderate quality factors to the plexcitonic system to boost its coherence. We show that the detuning of the introduced cavity mode with respect to the original plexcitonic system, which defines the location of the cavity SHB, is the most critical parameter. Simultaneously introducing two cavity modes of opposite detunings, the excited-state population of the emitter can be enhanced by 4.5 orders of magnitude within 300 fs, and the attenuation of the emitter's population can be slowed down by about 56 times. This theoretical proposal provides a new approach of cavity engineering to enhance the plasmon-emitter strong coupling systems' coherence, which is important for realistic hybrid-cavity design for applications in quantum technology.

Steering Room-Temperature Plexcitonic Strong Coupling: A Diexcitonic Perspective.

Plexcitonic strong coupling between a plasmon-polariton and a quantum emitter empowers ultrafast quantum manipulations in the nanoscale under ambient conditions. The main body of previous studies deals with homogeneous quantum emitters. To enable multiqubit states for future quantum computing and network, the strong coupling involving two excitons of the same material but different resonant energies has been investigated and observed primarily at very low temperature. Here, we report a room-temperature diexcitonic strong coupling (DiSC) nanosystem in which the excitons of a transition metal dichalcogenide monolayer and dye molecules are both strongly coupled to a single Au nanocube. Coherent information exchange in this DiSC nanosystem could be observed even when exciton energy detuning is about five times larger than the respective line widths. The strong coupling behaviors in such a DiSC nanosystem can be manipulated by tuning the plasmon resonant energies and the coupling strengths, opening up a paradigm of controlling plasmon-assisted coherent energy transfer.

Reconfigurable Photon Sources Based on Quantum Plexcitonic Systems.

A single photon in a strongly nonlinear cavity is able to block the transmission of a second photon, thereby converting incident coherent light into antibunched light, which is known as the photon blockade effect. Photon antipairing, where only the entry of two photons is blocked and the emission of bunches of three or more photons is allowed, is based on an unconventional photon blockade mechanism due to destructive interference of two distinct excitation pathways. We propose quantum plexcitonic systems with moderate nonlinearity to generate both antibunched and antipaired photons. The proposed plexcitonic systems benefit from subwavelength field localizations that make quantum emitters spatially distinguishable, thus enabling a reconfigurable photon source between antibunched and antipaired states via tailoring the energy bands. For a realistic nanoprism plexcitonic system, chemical and optical schemes of reconfiguration are demonstrated. These results pave the way to realize reconfigurable nonclassical photon sources in a simple quantum plexcitonic platform.

Optical signatures of Mott-superfluid transition in nitrogen-vacancy centers coupled to photonic crystal cavities: publisher's note.

This publisher's note contains corrections to Opt. Lett.44, 2081 (2019)OPLEDP0146-959210.1364/OL.44.002081.

Quantum Plasmonic Immunoassay Sensing.

Plasmon-polaritons are among the most promising candidates for next-generation optical sensors due to their ability to support extremely confined electromagnetic fields and empower strong coupling of light and matter. Here we propose quantum plasmonic immunoassay sensing as an innovative scheme, which embeds immunoassay sensing with recently demonstrated room-temperature strong coupling in nanoplasmonic cavities. In our protocol, the antibody-antigen-antibody complex is chemically linked with a quantum emitter label. Placing the quantum-emitter-enhanced antibody-antigen-antibody complexes inside or close to a nanoplasmonic (hemisphere dimer) cavity facilitates strong coupling between the plasmon-polaritons and the emitter label resulting in signature Rabi splitting. Through rigorous statistical analysis of multiple analytes randomly distributed on the substrate in extensive realistic computational experiments, we demonstrate a drastic enhancement of the sensitivity up to nearly 1500% compared to conventional shifting-type plasmonic sensors. Most importantly and in stark contrast to classical sensing, we achieve in the strong-coupling (quantum) sensing regime an enhanced sensitivity that is no longer dependent on the concentration of antibody-antigen-antibody complexes down to the single-analyte limit. The quantum plasmonic immunoassay scheme thus not only leads to the development of plasmonic biosensing for single molecules but also opens up new pathways toward room-temperature quantum sensing enabled by biomolecular inspired protocols linked with quantum nanoplasmonics.

Optical signatures of Mott-superfluid transition in nitrogen-vacancy centers coupled to photonic crystal cavities.

Detecting optical signatures of quantum phase transitions (QPT) in driven-dissipative systems constitutes a new frontier for many-body physics. Here we propose a practical idea to characterize the extensively studied phenomenon of photonic QPT, based on a many-body system composed of nitrogen-vacancy centers embedded individually in photonic crystal cavities, by detecting the critical behaviors of mean photon number, photon fluctuation, photon correlation, and emitted spectrum. Our results bridge these observables to the distinct optical signatures in different quantum phases and serve as good indicators and invaluable tools for studying dynamical properties of dissipative QPT.

Generation of multiqubit steady-state quantum correlation by squeezed-reservoir engineering.

Stationary quantum correlation among two-level systems (TLSs) in steady state is one of unique resources for applications in quantum information processing. Here we propose a scheme to generate such quantum correlation among the TLSs inside a lossy cavity. It is found that, by applying a broadband squeezed laser acting as a squeezed-vacuum reservoir to the cavity, a stable quantum correlation of the TLSs can be generated. By adiabatically eliminating the cavity field, we derive a reduced master equation of the TLSs in the bad-cavity limit. We show that the generated quantum correlation is essentially determined by the squeezing features transferred from the squeezed-vacuum reservoir via the cavity field as a quantum bus. We study the effect of the system parameters, such as the squeezing, the detuning, the coupling strength, and the decay rate of the TLSs, on the performance of the scheme. The feasibility of our proposal is supported by the application of currently available experimental techniques.

Characterizing real-space topology in Rice-Mele model by thermodynamics.

The thermodynamic quantities which are related to energy-level statistics are used to characterize the real-space topology of the Rice-Mele model. Through studying the energy spectrum of the model under different boundary conditions, we found that the non-normalizable wave function for the infinite domain is reduced to the edge state adhered to the boundary. For the finite domain with symmetric boundary condition, the critical point for the topological phase transition is equal to the inverse of the domain length. In contrast, the critical point is zero for the semi-infinite domain. Additionally, the symmetry of the energy spectrum is found to be sensitive to the boundary conditions of the Rice-Mele model, and the emergence of the edge states as well as the topological phase transition can be reflected in the thermodynamic properties. A potentially practical scheme is proposed for simulating the Rice-Mele model and detecting the relevant thermodynamic quantities in the context of Bose-Einstein condensate.

Majorana transport in superconducting nanowire with Rashba and Dresselhaus spin-orbit couplings.

The tunneling experiment is a key technique for detecting Majorana fermion (MF) in solid state systems. We use Keldysh non-equilibrium Green function method to study two-lead tunneling in superconducting nanowire with Rashba and Dresselhaus spin-orbit couplings. A zero-bias dc conductance peak appears in our setup which signifies the existence of MF and is in accordance with previous experimental results on InSb nanowire. Interestingly, due to the exotic property of MF, there exists a hole transmission channel which makes the currents asymmetric at the left and right leads. The ac current response mediated by MF is also studied here. To discuss the impacts of Coulomb interaction and disorder on the transport property of Majorana nanowire, we use the renormalization group method to study the phase diagram of the wire. It is found that there is a topological phase transition under the interplay of superconductivity and disorder. We find that the Majorana transport is preserved in the superconducting-dominated topological phase and destroyed in the disorder-dominated non-topological insulator phase.