Bosonic excitation spectra of superconductingBi2Sr2CaCu2O8+δandYBa2Cu3O6+xextracted from scanning tunneling spectra.

A detailed interpretation of scanning tunneling spectra obtained on unconventional superconductors enables one to gain information on the pairing boson. Decisive for this approach are inelastic tunneling events. Due to the lack of momentum conservation in tunneling from or to the sharp tip, those are enhanced in the geometry of a scanning tunneling microscope compared to planar tunnel junctions. This work extends the method of obtaining the bosonic excitation spectrum by deconvolution from tunneling spectra to nodald-wave superconductors. In particular, scanning tunneling spectra of slightly underdopedBi2Sr2CaCu2O8+δwith aTcof 82 K and optimally dopedYBa2Cu3O6+xwith aTcof 92 K reveal a resonance mode in their bosonic excitation spectrum atΩres≈63 meVandΩres≈61 meVrespectively. In both cases, the overall shape of the bosonic excitation spectrum is indicative of predominant spin scattering with a resonant mode atΩres<2Δand overdamped spin fluctuations for energies larger than 2Δ. To perform the deconvolution of the experimental data, we implemented an efficient iterative algorithm that significantly enhances the reliability of our analysis.

Progress on the Fabrication of Superconducting Wires and Tapes via Hot Isostatic Pressing.

Fabrication of high-performance superconducting wires and tapes is essential for large-scale applications of superconducting materials. The powder-in-tube (PIT) method involves a series of cold processes and heat treatments and has been widely used for fabricating BSCCO, MgB2, and iron-based superconducting wires. The densification of the superconducting core is limited by traditional heat treatment under atmospheric pressure. The low density of the superconducting core and a large number of pores and cracks are the main factors limiting the current-carrying performance of PIT wires. Therefore, to improve the transport critical current density of the wires, it is essential to densify the superconducting core and eliminate pores and cracks to enhance grain connectivity. Hot isostatic pressing (HIP) sintering was employed to improve the mass density of superconducting wires and tapes. In this paper, we review the development and application of the HIP process in the manufacturing of BSCCO, MgB2, and iron-based superconducting wires and tapes. The development of HIP parameters and the performance of different wires and tapes are reviewed. Finally, we discuss the advantages and prospects of the HIP process for the fabrication of superconducting wires and tapes.

Nanowire bolometer using a 2D high-temperature superconductor.

Superconducting nanowires are very important due to their applications ranging from quantum technology to astronomy. In this work, we implement a non-invasive process to fabricate nanowires of high-Tcsuperconductor Bi2Sr2CaCu2O8+δ. We demonstrate that our nanowires can be used as bolometers in the visible range with very high responsivity of 9.7 × 103V W-1. Interestingly, in a long (30µm) nanowire of 9 nm thickness and 700 nm width, we observe bias current-dependent localized spots of maximum photovoltage. Moreover, the scalability of the bolometer responsivity with the normal state resistance of the nanowire could allow further performance improvement by increasing the nanowire length in a meander geometry. We observe phase slip events in nanowires with small cross-sections (12 nm thick, 300 nm wide, and 3µm long) at low temperatures. Our study presents a scalable method for realizing sensitive bolometers working near the liquid-nitrogen temperature.

Superconducting Vortex-Charge Measurement Using Cavity Electromechanics.

As the magnetic field penetrates the surface of a superconductor, it results in the formation of flux vortices. It has been predicted that the flux vortices will have a charged vortex core and create a dipolelike electric field. Such a charge trapping in vortices is particularly enhanced in high-Tc superconductors (HTS). Here, we integrate a mechanical resonator made of a thin flake of HTS Bi2Sr2CaCu2O8+δ into a microwave circuit to realize a cavity-electromechanical device. Due to the exquisite sensitivity of cavity-based devices to the external forces, we directly detect the charges in the flux vortices by measuring the electromechanical response of the mechanical resonator. Our measurements reveal the strength of surface electric dipole moment due to a single vortex core to be approximately 30 |e|aB, equivalent to a vortex charge per CuO2 layer of 3.7 × 10-2|e|, where aB is the Bohr radius and e is the electronic charge.

Two-Dimensional Bi2Sr2CaCu2O8+δ Nanosheets for Ultrafast Photonics and Optoelectronics.

Two-dimensional (2D) Bi2Sr2CaCu2O8+δ (BSCCO) is a emerming class of 2D materials with high-temperature superconductivity for which their electronic transport properties have been intensively studied. However, the optical properties, especially nonlinear optical response and the photonic and optoelectronic applications of normal state 2D Bi2Sr2CaCu2O8+δ (Bi-2212), have been largely unexplored. Here, the linear and nonlinear optical properties of mechanically exfoliated Bi-2212 thin flakes are systematically investigated. 2D Bi-2212 shows a profound plasmon absorption in near-infrared wavelength range with ultrafast carrier dynamics as well as tunable nonlinear absorption depending on the thickness. We demonstrated that 2D Bi-2212 can be applied not only as an effective mode-locker for ultrashort pulse generation but also as an active medium for infrared light detection due to its plasmon absorption. Our results may trigger follow up studies on the optical properties of 2D BSCCO and demonstrate potential opportunities for photonic and optoelectronic applications.

Electronic and vibrational properties of the highTcsuperconductor Bi2Sr2CaCu2O8: anab initiostudy.

In this work,ab initiocalculations were performed in order to study the vibrational spectra of the Bi2Sr2CaCu2O8(Bi2212) compound. A structural modulation correction on some atomic positions, producing a distorted structure with lower symmetry, is used for the calculation. We argue that this correction allows to account for an average effect of the incommensurate superstructure, generating a more accurate representation of the real unit cell observed in this compound. A complete and conclusive vibrational assignment is performed, discussing the correspondences with previous experimental and theoretical reports. A brief analysis of the electronic density of states and band structure comparing the tetragonal and distorted unit cell is also included.

Higher superconducting transition temperature by breaking the universal pressure relation.

By investigating the bulk superconducting state via dc magnetization measurements, we have discovered a common resurgence of the superconducting transition temperatures (Tcs) of the monolayer Bi2Sr2CuO6+δ (Bi2201) and bilayer Bi2Sr2CaCu2O8+δ (Bi2212) to beyond the maximum Tcs (Tc-maxs) predicted by the universal relation between Tc and doping (p) or pressure (P) at higher pressures. The Tc of underdoped Bi2201 initially increases from 9.6 K at ambient to a peak at 23 K at 26 GPa and then drops as expected from the universal Tc-P relation. However, at pressures above 40 GPa, Tc rises rapidly without any sign of saturation up to 30 K at 51 GPa. Similarly, the Tc for the slightly overdoped Bi2212 increases after passing a broad valley between 20 and 36 GPa and reaches 90 K without any sign of saturation at 56 GPa. We have, therefore, attributed this Tc resurgence to a possible pressure-induced electronic transition in the cuprate compounds due to a charge transfer between the Cu 3[Formula: see text] and the O 2p bands projected from a hybrid bonding state, leading to an increase of the density of states at the Fermi level, in agreement with our density functional theory calculations. Similar Tc-P behavior has also been reported in the trilayer Br2Sr2Ca2Cu3O10+δ (Bi2223). These observations suggest that higher Tcs than those previously reported for the layered cuprate high-temperature superconductors can be achieved by breaking away from the universal Tc-P relation through the application of higher pressures.