RESUMO
In this study, we analyzed the hourly concentration data of PM10 and PM2.5 in major cities in Jinzhong basin from 2017 to 2019. The main distribution characteristics of aerosols in Jinzhong and Taiyuan were determined, and PM2.5 hourly concentration data and HYSPLIT in Jinzhong basin in winter were discussed. The results showed that the overall level of particulate matter concentration in Taiyuan was higher than that in Jinzhong, and the monthly and seasonal variation characteristics were similar. All showed high concentrations in winter and low concentrations in summer, and the highest concentration value appeared in January. The aerosol pollution caused by the static and stable weather in Jinzhong was more common than that caused by the sand and dust weather in Taiyuan. The distribution of particulate matter showed the characteristics of more intermediate values in Jinzhong and more high and fewer low values in Taiyuan, and winter was the highest incidence season of PM2.5 pollution in Jinzhong basin. PM2.5 transmission passageways in the main cities of Jinzhong basin in winter could be divided into four categories:class 1 was transmitted along the transverse valley of Taihang Mountain, and class 2 was the southeast transmission channel. Class 1 and class 2 were the short-range transmission passageways; air masses carried more moisture, and PM2.5 transmitted along such passageways allowed moisture to be absorbed more easily, increasing levels and aggravating local pollution. Class 3 was the northwest passageway, corresponding to the most serious pollution period of PM2.5 in Jinzhong basin before the arrival of cold air, which also corresponded to the dust transmission passageway. Class 4 was the Fenwei Plain passageway, corresponding to high-concentration PM2.5 pollution. Areas with dense pollution tracks (more than 100 pollution tracks) and areas with slow air flow movement (RTA pollution track end points greater than 50) easily became potential source areas of target cities (PSCF contribution greater than 0.7). The main potential source areas of PM2.5 in winter in Jinzhong (PSCF contributing more than 0.7) were mainly distributed in Linfen, Jincheng, and other places in Shanxi province, as well as in the north of Henan province, the south of Hebei province, and central and south Shaanxi province. The distribution range of main potential source areas of PM2.5 in Taiyuan in winter was wider than that in Jinzhong, including the south of Lvliang, Yangquan, Linfen, and Yuncheng and the south of Jinzhong in Shanxi, as well as most areas in southern Shaanxi, northern Henan province, and southern Hebei province. In addition, the PSCF distribution of high-value centers above 0.9 was wider than that of Jinzhong. When pollution occurs in cities that PSCF contributed more than 0.9, special attention should be paid to the influence of mutual transmission between them and cities in Jinzhong basin. Jinzhong and Taiyuan showed different distribution characteristics corresponding to the surface wind direction when light and higher pollution occur, when the wind direction near the ground in Jinzhong was E, the frequency of light and higher pollution was 8.1%; it was the highest in all wind directions. When the wind direction near the ground in Taiyuan was SSW, the frequency of light to higher polluted weather was the highest in all wind directions (5.1%). In the case of calm wind, the frequency of light to higher pollution in Taiyuan (3.4%) was higher than that in Jinzhong (0.5%).
Assuntos
Poluentes Atmosféricos , Poluição do Ar , Aerossóis/análise , Poluentes Atmosféricos/análise , Poluição do Ar/análise , Cidades , Poeira/análise , Monitoramento Ambiental/métodos , Material Particulado/análise , Estações do AnoRESUMO
In order to systematically study the transmission characteristics of seasonal and typical pollutants in Shijiazhuang, hourly data of ground-level pollutants(PM2.5, PM10, O3, NO2, SO2, and CO) from 46 state-and provincial-controlled stations, and meteorological(temperature, humidity, and wind speed) data from 17 counties in Shijiazhuang City from December 2018 to November 2019 was analyzed. The interpolation(IDW) and correlation analysis were applied to seasonal and temporal spatial patterns of pollutant concentration. The backward trajectories analysis was performed to explore the seasonal transmission pattern and potential source areas of pollution in Shijiazhuang by combining with the global data assimilation system(GDAS). The results indicate that the different seasons have characteristic pollutants, as follows:spring(PM10, 48.91%), summer(O3, 81.97%), autumn(PM10 and PM2.5, 47.54% and 32.79%), and winter(PM2.5, 74.44%), which are related to the variation of meteorological conditions. Furthermore, the PM10(spring) concentration correlated negatively with the wind speed, presenting a high distribution in the northwest and low in the southeast, with a southerly transmission direction(53.32%). Central and southern Hebei, central and northern Henan, and central Shanxi are the potential sources of pollution(WPCWTij ≥ 160 µg·m-3), impacting western Shandong and northwest Shanxi(WPSCFij ≥ 0.3) with PM10. Moreover, the O3(summer) concentration correlated positively with temperature, and negatively with humidity. The southeast-south(54.24%) is the source direction of the transmission, and the potential source of O3 pollution is an arc area with Shijiazhuang in the center and Cangzhou and Heze as the double wings. Lastly, the PM2.5(autumn and winter) concentration correlated positively with humidity, and the winter concentration shows an increasing gradient from west to east. The trajectories of PM2.5 clustered the source directions:autumn(northeast-southeast, 74.75%), winter(northwest, 55.47%); central and southern Hebei, central and western Shanxi and northern Henan are the concentrated sources of potential pollution(WPCWTij ≥ 180 µg·m-3).
Assuntos
Poluentes Atmosféricos , Poluição do Ar , Poluentes Atmosféricos/análise , China , Monitoramento Ambiental , Poluição Ambiental , Material Particulado/análise , Estações do AnoRESUMO
During the dry season, from November to April, agricultural biomass burning and forest fires especially from March to late April in mainland Southeast Asian countries of Myanmar, Thailand, Laos and Vietnam frequently cause severe particulate pollution not only in the local areas but also across the whole region and beyond due to the prevailing meteorological conditions. Recently, the BASE-ASIA (Biomass-burning Aerosols in South East Asia: Smoke Impact Assessment) and 7-SEAS (7-South-East Asian Studies) studies have provided detailed analysis and important understandings of the transport of pollutants, in particular, the aerosols and their characteristics across the region due to biomass burning in Southeast Asia (SEA). Following these studies, in this paper, we study the transport of particulate air pollution across the peninsular region of SEA and beyond during the March 2014 burning period using meteorological modelling approach and available ground-based and satellite measurements to ascertain the extent of the aerosol pollution and transport in the region of this particular event. The results show that the air pollutants from SEA biomass burning in March 2014 were transported at high altitude to southern China, Hong Kong, Taiwan and beyond as has been highlighted in the BASE-ASIA and 7-SEAS studies. There are strong evidences that the biomass burning in SEA especially in mid-March 2014 has not only caused widespread high particle pollution in Thailand (especially the northern region where most of the fires occurred) but also impacted on the air quality in Hong Kong as measured at the ground-based stations and in LulinC (Taiwan) where a remote background monitoring station is located.