Importance of local non-fossil sources to carbonaceous aerosols at the eastern fringe of the Tibetan Plateau, China: Δ14C and δ13C evidences.
Environ Pollut
; 311: 119858, 2022 Oct 15.
Article
in En
| MEDLINE
| ID: mdl-35964790
ABSTRACT
Carbonaceous particles are an important radiative forcing agent in the atmosphere, with large temporal and spatial variations in their concentrations and compositions, especially in remote regions. This study reported the Δ14C and δ13C of total carbon (TC) and water-insoluble particulate carbon (IPC) of the total suspended particles (TSP) and PM2.5 at a remote site of the eastern Tibetan Plateau (TP), a region that is influenced by heavy air pollution from Southwest China. The average organic carbon and elemental carbon concentrations of TSP samples in this study were 3.20 ± 2.38 µg m-3 and 0.68 ± 0.67 µg m-3, respectively, with low and high values in summer and winter, respectively. The fossil fuel contributions of TC in TSP and PM2.5 samples were 18.91 ± 7.22% and 23.13 ± 12.52%, respectively, both of which were far lower than that in Southwest China, indicating the importance of non-fossil contributions from local sources. The δ13C of TC in TSP samples of the study site was -27.06 ± 0.96, which is between the values of long-range transported sources (e.g., Southwest China) and local biomass combustion emissions. Therefore, despite the contribution from the long-range transport of particles, aerosols emitted from local biomass combustion also have an important influence on carbonaceous particles at the study site. The findings of this work can be applied to other remote sites on the eastern TP and should be considered in related research in the future.
Key words
Full text:
1
Collection:
01-internacional
Health context:
2_ODS3
Database:
MEDLINE
Main subject:
Air Pollutants
/
Particulate Matter
Country/Region as subject:
Asia
Language:
En
Journal:
Environ Pollut
Year:
2022
Document type:
Article