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Complex anisotropy ratio of third harmonic generation in a semiconductor using a terahertz free electron laser.
Opt Lett ; 49(18): 5039-5042, 2024 Sep 15.
Article in En | MEDLINE | ID: mdl-39270224
ABSTRACT
The nonlinear susceptibility in the terahertz region is expected to have a non-negligible imaginary part originating from the momentum-dependent scattering time of free carriers, but it has been scarcely reported. By utilizing an intense 4 THz beam from a terahertz free electron laser, we investigated the azimuth angle dependence of the third harmonic generation (THG) from semiconductors. The observed angular anisotropy of THG revealed the contribution of the imaginary part of the nonlinear susceptibility originating from the momentum-scattering time relation in addition to its real part originating from the band nonparabolicity. The results provide a deeper understanding of nonlinear optics in the terahertz region.

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Opt Lett Year: 2024 Document type: Article

Full text: 1 Collection: 01-internacional Database: MEDLINE Language: En Journal: Opt Lett Year: 2024 Document type: Article