Photoinduced melting of a stripe-type charge-order and metallic domain formation in a layered BEDT-TTF-based organic salt.
Phys Rev Lett
; 98(9): 097402, 2007 Mar 02.
Article
em En
| MEDLINE
| ID: mdl-17359195
ABSTRACT
Photoinduced melting of charge-order (CO) in [bis(ethylenedithiolo)]-tetrathiafulvalene (BEDT-TTF) salts was investigated by femotosecond spectroscopy. Comparative studies on two polytypes exhibiting large [theta-(BEDT-TTF)2RbZn(SCN)_{4}] and small [alpha-(BEDT-TTF)2I3] molecular rearrangements through the CO transition were performed. Ultrafast melting of CO for both compounds demonstrates the major contribution of the electronic instability which is due to Coulomb interaction. The roles of the molecular rearrangements on the formation of the CO and the metallic domain are discussed on the basis of low-frequency lattice dynamics.
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01-internacional
Base de dados:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Ano de publicação:
2007
Tipo de documento:
Article