Pollution revealed by stable lead isotopes in recent snow from the northern and central Tibetan Plateau.
Ecotoxicol Environ Saf
; 263: 115296, 2023 Sep 15.
Article
em En
| MEDLINE
| ID: mdl-37517310
Lead (Pb) isotopes are less fractionated than those from different sources, and thus were used to trace the sources of Pb in the environment. To investigate the sources of Pb in the atmosphere of the Tibetan Plateau, stable Pb isotopes (206Pb, 207Pb and 208Pb) in acidified snow pit samples collected from five glaciers (i.e., Qiyi-QY, Meikuang-MK, Yuzhufeng-YZF, Hariqin-HRQ and Xiaodongkemadi-XDKMD) in May 2016 of the northern and central Tibetan Plateau were measured. The results showed narrow ranges of 1.158-1.187 for 206Pb/207Pb and 2.450-2.489 for 208Pb/207Pb respectively. The 206Pb/207Pb ratios in all samples were obviously lower than the environmental background value of 1.196, indicating the primary contributions of anthropogenic sources. At least 60% of Pb was contributed by various human activities, which was supported by the Pb isotopes in the snow pit samples from the QY, MK, YZF, HRQ and XDKMD glaciers. By comparing Pb isotope data, we found that the primary anthropogenic sources are coal combustion, mining and smelting activities in northwestern China and mixed emissions from cities located in western China and close to the glaciers. These sources contributed to the Pb in the northern glaciers (QY and MK) in particular. Coal combustion in India probably contributes to the central glaciers (HRQ and XDKMD). Another potential source could be parts of central Asia (e.g., Kyrgyzstan and Uzbekistan) through long range transport. The above potential source areas of contaminants were traced further by the air mass back-trajectory tracing method.
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Texto completo:
1
Coleções:
01-internacional
Contexto em Saúde:
2_ODS3
Base de dados:
MEDLINE
Assunto principal:
Neve
/
Chumbo
Limite:
Humans
País/Região como assunto:
Asia
Idioma:
En
Revista:
Ecotoxicol Environ Saf
Ano de publicação:
2023
Tipo de documento:
Article