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Dynamics and fluctuations of minimally structured glass formers.
Charbonneau, Patrick; Hu, Yi; Morse, Peter K.
Afiliação
  • Charbonneau P; Department of Chemistry, <a href="https://ror.org/00py81415">Duke University</a>, Durham, North Carolina 27708, USA.
  • Hu Y; Department of Physics, <a href="https://ror.org/00py81415">Duke University</a>, Durham, North Carolina 27708, USA.
  • Morse PK; Department of Chemistry, <a href="https://ror.org/00py81415">Duke University</a>, Durham, North Carolina 27708, USA.
Phys Rev E ; 109(5-1): 054905, 2024 May.
Article em En | MEDLINE | ID: mdl-38907402
ABSTRACT
The mean-field theory (MFT) of simple structural glasses, which is exact in the limit of infinite spatial dimensions, d→∞, offers theoretical insight as well as quantitative predictions about certain features of d=3 systems. In order to more systematically relate the behavior of physical systems to MFT, however, various finite-d effects need to be accounted for. Although some efforts along this direction have already been undertaken, theoretical and technical challenges hinder progress. A general approach to sidestep many of these difficulties consists of simulating minimally structured models whose behavior smoothly converges to that described by the MFT as d increases, so as to permit a controlled dimensional extrapolation. Using this approach, we here extract the small fluctuations around the dynamical MFT captured by a standard liquid-state observable, the non-Gaussian parameter α_{2}. The results provide insight into the physical origin of these fluctuations as well as a quantitative reference with which to compare observations for more realistic glass formers.

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Phys Rev E Ano de publicação: 2024 Tipo de documento: Article

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Phys Rev E Ano de publicação: 2024 Tipo de documento: Article