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1.
Proc Natl Acad Sci U S A ; 117(2): 913-922, 2020 01 14.
Artigo em Inglês | MEDLINE | ID: mdl-31740597

RESUMO

Oil and gas well leakage is of public concern primarily due to the perceived risks of aquifer contamination and greenhouse gas (GHG) emissions. This study examined well leakage data from the British Columbia Oil and Gas Commission (BC OGC) to identify leakage pathways and initially quantify incident rates of leakage and GHG emissions from leaking wells. Three types of leakage are distinguished: "surface casing vent flow" (SCVF), "outside the surface casing leakage" (OSCL), and "cap leakage" (CL). In British Columbia (BC), the majority of reported incidents involve SCVF of gases, which does not pose a risk of aquifer contamination but does contribute to GHG emissions. Reported liquid leakage of brines and hydrocarbons is rarer. OSCL and CL of gas are more serious problems due to the risk of long-term leakage from abandoned wells; some were reported to be leaking gas several decades after they were permanently abandoned. According to the requirements of provincial regulation, 21,525 have been tested for leakage. In total, 2,329 wells in BC have had reported leakage during the lifetime of the well. This represents 10.8% of all wells in the assumed test population. However, it seems likely that wells drilled and/or abandoned before 2010 have unreported leakage. In BC, the total GHG emission from gas SCVF is estimated to reach about 75,000 t/y based on the existing inventory calculation; however, this number is likely higher due to underreporting.


Assuntos
Gases de Efeito Estufa/análise , Campos de Petróleo e Gás , Poluentes Químicos da Água/análise , Poluição do Ar , Colúmbia Britânica , Monitoramento Ambiental , Geologia , Água Subterrânea , Gás Natural , Permeabilidade , Poços de Água
2.
J Environ Manage ; 246: 275-282, 2019 Sep 15.
Artigo em Inglês | MEDLINE | ID: mdl-31181476

RESUMO

This paper presents the various tools and data sources in British Columbia (Canada) that can be used by environmental consultants to assess the potential of cross-contamination between shale gas formation fluids and shallow aquifers from hydraulic fracturing and related oil and gas activities. A systematic approach for evaluating the potential of cross-contamination using these data sources is applied to a specific case study at an undisclosed location in the northeastern part of the province. This approach includes defining and then evaluating the basic criteria for assessing the potential of cross-contamination. These criteria are: a leak source; a driving force such as buoyancy or head differential and a leakage pathway. This study has revealed that there is a potential of cross-contamination due to hydraulic fracturing activities and wellbore integrity issues. Wellbore integrity can be compromised by induced seismic events or by unintentional communication with offset hydraulic fractured wells. Induced seismicity is linked to the activity of hydraulic fracturing as well as to the deep disposal of wastewater.


Assuntos
Água Subterrânea , Fraturamento Hidráulico , Colúmbia Britânica , Gás Natural , Campos de Petróleo e Gás , Poços de Água
3.
Sci Total Environ ; 912: 169188, 2024 Feb 20.
Artigo em Inglês | MEDLINE | ID: mdl-38081423

RESUMO

This study highlights concerns regarding the reliability of groundwater nitrate data used in official surveys, such as within the EU-mandated Water Framework Directive (WFD). The focus is on the Campo de Cartagena - Mar Menor hydrosystem in Spain, a region known for its intensively irrigated watershed and eutrophicated lagoon, where monitoring the evolution of nitrate contamination in surface and groundwater is crucial but challenging due to the risk of inconsistent characterization leading to erratic remediation measures. The study employed an experimental approach in private wells that belong to a longstanding official nitrate survey network marked by irregular sampling practices. Importantly, these wells lacked comprehensive design documentation and were frequently used by farmers. The study aimed to evaluate the representativity of dissolved nitrate measurements in such an emblematic case, while investigating the source of the water using geochemical and isotope tracers. This assessment considered the effects of different sampling techniques (bailer or pumping) and sampling parameters (depth and time), acknowledging actual practices. The research highlights several key findings. Firstly, the bailer sampling method proved to account for a substantial portion of the observed variation in nitrate content. Secondly, in some cases, pumping introduced contributions from different water horizons, complicating the interpretation of nitrate data. Thirdly, alterations in the sampling protocol had a notable impact on the resulting nitrate measurements. Furthermore, the study emphasized a critical issue: the lack of analytical uncertainty estimation in official surveys introduces significant bias in result interpretation, with discrepancies exceeding 100 mg/L in four of the six wells analyzed. This underscores the pressing need for improved sampling protocols, dedicated borehole infrastructure and precise data interpretation. Given the potential unreliability of some official groundwater nitrate data shared under EU or other regulations, with corresponding economic and environmental impacts, the study recommends meticulous verification before transmitting data.

4.
Sci Total Environ ; 864: 160964, 2023 Mar 15.
Artigo em Inglês | MEDLINE | ID: mdl-36539081

RESUMO

Identifying groundwater wells performing riverbank filtration (RBF) is crucial to ensure safe drinking water through vulnerability assessment plans adapted to these hybrid water sources. Nonetheless, RBF is often unintentional or insufficiently documented and official inventories are scarce. We developed a user-friendly geochemical and isotopic framework for the in-situ identification of RBF facilities. It includes an interpretation abacus for non-specialists. While most studies using tracers are site-specific and/or based on discrete samples, we propose a novel multi-site characterization where time-series of EC, δ2H and δ18O are directly used as proxies of surface water infiltration at the watershed-scale. The basic statement is that time varying signal of raw water from a groundwater pumping facility reveals a significant induced infiltration of surface water. The framework was applied on nearly 2000 samples from 40 pumping wells and 4 neighboring rivers (<500 m), collected through collaborative sampling on a weekly to monthly basis for 18 months. Despite proximity to surface water, two-third of the complete dataset (19 facilities) were revealed not to benefit from significant contribution of surface water, demonstrating location criteria to be insufficient to identify RBF sites. Permanent RBF was evidenced at 5 facilities, where year-long seasonal variation of tracers in raw groundwater highlighted a continuous high proportion of infiltrated surface water. Unexpectedly, time-series also unveiled a third category: occasional RBF, where induced infiltration occurred only when specific hydrodynamic conditions were met (4 facilities). This study also provided concrete illustrations on how climate change may impact the efficiency of RBF to naturally attenuate microbiological contaminants and how geochemical and isotopic time-series considerably help at anticipating the evolution of contaminant attenuation capacity of RBF sites. Finally, by highlighting the existence of occasional RBF, this study tackles the common oversimplification that groundwater facilities can be binarily and classified either as RBF or groundwater.

5.
Sci Total Environ ; 750: 141429, 2021 Jan 01.
Artigo em Inglês | MEDLINE | ID: mdl-32853932

RESUMO

Bank filtration is a popular pre-treatment method to produce drinking water as it benefits from the natural capacity of the sediments to attenuate contaminants. Under flood conditions, bank filtration systems are known to be vulnerable to contamination, partly because flow patterns may evolve at short timescales and result in a rapid evolution of the origin and travel times of surface water in the aquifer. However, high frequency monitoring for water quality is not common practice yet, and water quality management decisions for the operation of bank filtration systems are typically based on weekly to monthly assays. The aim of this study is to illustrate how monitoring strategies of environmental tracers at flood-affected sites can be optimized and to demonstrate how tracer-based evidence can help to define adequate pumping strategies. Data acquisition spanned two intense flood events at a two-lake bank filtration site. Based on bacteriological indicators, the bank filtration system was shown to be resilient to the yearly recurring flood events but more vulnerable to contamination during the intense flood events. The origin of the bank filtrate gradually evolved from a mixture between the two lakes towards a contribution of floodwater and one lake only. Automatized measurements of temperature and electrical conductivity at observation wells allowed to detect changes in the groundwater flow patterns at a daily timescale, while the regulatory monthly monitoring for indicator bacteria did not fully capture the potential short timescale variability of the water quality. The recovery to pre-flood conditions was shown to be accelerated for the wells operating at high rates (i.e., ≥1000 m3/day), partly because of floodwater storage in the vicinity of the less active wells. These results establish new perspectives to anticipate water quality changes through selected pumping schemes, which depend on and must be adapted to site-specific water quality issues.

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