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1.
Phys Rev Lett ; 130(12): 126401, 2023 Mar 24.
Artigo em Inglês | MEDLINE | ID: mdl-37027842

RESUMO

The recently discovered layered kagome metals of composition AV_{3}Sb_{5} (A=K, Rb, Cs) exhibit a complex interplay among superconductivity, charge density wave order, topologically nontrivial electronic band structure and geometrical frustration. Here, we probe the electronic band structure underlying these exotic correlated electronic states in CsV_{3}Sb_{5} with quantum oscillation measurements in pulsed fields up to 86 T. The high-field data reveal a sequence of magnetic breakdown orbits that allows the construction of a model for the folded Fermi surface of CsV_{3}Sb_{5}. The dominant features are large triangular Fermi surface sheets that cover almost half the folded Brillouin zone. These sheets have not yet been detected in angle resolved photoemission spectroscopy and display pronounced nesting. The Berry phases of the electron orbits have been deduced from Landau level fan diagrams near the quantum limit without the need for extrapolations, thereby unambiguously establishing the nontrivial topological character of several electron bands in this kagome lattice superconductor.

2.
J Phys Chem Lett ; 14(19): 4504-4509, 2023 May 18.
Artigo em Inglês | MEDLINE | ID: mdl-37158696

RESUMO

We propose a novel method for enantioselective electron paramagnetic resonance (EPR) spectroscopy based on magneto-chiral anisotropy. We elaborate a theoretical model to estimate the strength of this effect and propose a dedicated interferometer setup for its experimental observation.

3.
J Phys Chem Lett ; 8(8): 1851-1855, 2017 Apr 20.
Artigo em Inglês | MEDLINE | ID: mdl-28393517

RESUMO

We have accurately determined the exciton binding energy and reduced mass of single crystals of methylammonium lead triiodide using magneto-reflectivity at very high magnetic fields. The single crystal has excellent optical properties with a narrow line width of ∼3 meV for the excitonic transitions and a 2s transition that is clearly visible even at zero magnetic field. The exciton binding energy of 16 ± 2 meV in the low-temperature orthorhombic phase is almost identical to the value found in polycrystalline samples, crucially ruling out any possibility that the exciton binding energy depends on the grain size. In the room-temperature tetragonal phase, an upper limit for the exciton binding energy of 12 ± 4 meV is estimated from the evolution of 1s-2s splitting at high magnetic field.

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