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We demonstrate that in partially ionized plasmas, Coulomb scattering can be significantly perturbed by electron collisions with neutral gas particles, and that this effect can be incorporated in the Coulomb collision terms of the Boltzmann equation by a modification of the classical Coulomb logarithm. We show that Boltzmann transport calculations using this modified Coulomb logarithm are in excellent agreement, for a sensitive model problem and a wide range of conditions, with particle simulations describing the many-body Coulomb interactions from first principles.
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Dynamic characteristics of strongly coupled classical one-component Coulomb and Yukawa plasmas are obtained within the nonperturbative model-free moment approach without any data input from simulations so that the dynamic structure factor (DSF) satisfies the first three nonvanishing sum rules automatically. The DSF, dispersion, decay, sound speed, and other characteristics of the collective modes are determined using exclusively the static structure factor calculated from various theoretical approaches including the hypernetted chain approximation. A good quantitative agreement with molecular dynamics simulation data is achieved.
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The dynamics of the ion structure in warm dense matter is determined by molecular dynamics simulations using an effective ion-ion potential. This potential is obtained from ab initio simulations and has a strong short-range repulsion added to a screened Coulomb potential. Models based on static or dynamic local field corrections are found to be insufficient to describe the data. An extended Mermin approach, a hydrodynamic model, and the method of moments with local constraints are capable of reproducing the numerical results but have rather limited predictive powers as they all need some numerical data as input. The method of moments is found to be the most promising.
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Unlike α- and γ-mode operation, electrons accelerated by strong drift and ambipolar electric fields in the plasma bulk and at the sheath edges are found to dominate the ionization in strongly electronegative discharges. These fields are caused by a low bulk conductivity and local maxima of the electron density at the sheath edges, respectively. This drift-ambipolar mode is investigated by kinetic particle simulations, experimental phase-resolved optical emission spectroscopy, and an analytical model in CF(4). Mode transitions induced by voltage and pressure variations are studied.
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We investigate the Ar(+)-Fe asymmetric charge transfer (ACT) reaction using a combination of plasma diagnostics methods and a kinetic model of the afterglow plasma, which allow monitoring of the temporal evolution of the densities of different species. The iron vapor is created inside a discharge cell by cathode sputtering; its density is measured by atomic absorption spectroscopy. The rate coefficient of the reaction is evaluated from the emission intensity decay of Fe(+)∗ lines pumped by the ACT process in the He-Ar-Fe and Ar-Fe afterglow plasmas. The measurements yield a rate coefficient k = 7.6( ± 3.0) × 10(-9) cm(3) s(-1) at T = 300 K.
Assuntos
Argônio/química , Ferro/química , Hélio/química , Íons/química , Cinética , Espectrofotometria Atômica , VácuoRESUMO
The existence of plasma oscillations at multiples of the magnetoplasmon frequency in a strongly coupled two-dimensional magnetized Yukawa plasma is reported, based on extensive molecular dynamics simulations. These modes are the analogues of Bernstein modes which are renormalized by strong interparticle correlations. Their properties are theoretically explained by a dielectric function incorporating the combined effect of a magnetic field, strong correlations and finite temperature.
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A classical dusty plasma experiment was performed using two different dust grain sizes to form a strongly coupled asymmetric bilayer (two closely spaced interacting monolayers) of two species of charged dust particles. The observation and analysis of the thermally excited particle oscillations revealed the collective mode structure and dispersion (wave propagation) in this system; in particular, the existence of the theoretically predicted k=0 energy (frequency) gap was verified. Equilibrium molecular-dynamics simulations were performed to emulate the experiment, assuming Yukawa-type interparticle interaction. The simulations and analytic calculations based both on lattice summation and on the quasilocalized charge approximation approach are in good agreement with the experimental findings and help in identifying and characterizing the observed phenomena.
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The existence of coefficients for diffusion, viscosity, and thermal conductivity is examined for two-dimensional (2D) liquids. Equilibrium molecular dynamics simulations are performed using a Yukawa potential and the long-time behavior of autocorrelation functions is tested. Advances reported here as compared to previous 2D Yukawa liquid simulations include an assessment of the thermal conductivity, using a larger system size to allow meaningful examination of longer times, and development of improved analysis methods. We find that the transport coefficient exists for diffusion at high temperature and viscosity at low temperature, but not in the opposite limits. The thermal conductivity coefficient does not appear to exist at high temperature. Further advances in computing power could improve these assessments by allowing even larger system sizes and longer time series.
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The self-diffusion phenomenon in a two-dimensional dusty plasma at extremely strong (effective) magnetic fields is studied experimentally and by means of molecular dynamics simulations. In the experiment the high magnetic field is introduced by rotating the particle cloud and observing the particle trajectories in a corotating frame, which allows reaching effective magnetic fields up to 3000 T. The experimental results confirm the predictions of the simulations: (i) superdiffusive behavior is found at intermediate timescales and (ii) the dependence of the self-diffusion coefficient on the magnetic field is well reproduced.
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We present molecular-dynamics calculations of the shear viscosity of three-dimensional strongly coupled Yukawa liquids which are frequently used as a model system of complex plasmas. The results obtained using two independent nonequilibrium simulation methods are critically compared with each other and with earlier published data for a wide range of plasma coupling (Gamma) and screening (kappa) parameters. The non-Newtonian behavior of the liquid, manifested as a decrease of the shear viscosity with increasing shear rate (shear thinning), and the validity of the Stokes-Einstein relation at high coupling strength are also demonstrated.
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The emergence and vanishing of superdiffusion in quasi-two-dimensional Yukawa systems are investigated by molecular dynamics simulations. Using both the asymptotic behavior of the mean-squared displacement of the particles and the long-time tail of the velocity autocorrelation function as indicators of superdiffusion, we confirm the existence of a transition from normal diffusion to superdiffusion in systems changing from a three-dimensional to a two-dimensional character. A connection between superdiffusion and dimensionality is established by the behavior of the projected pair distribution function.
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A magnetic field was recently shown to enhance field-parallel heat conduction in a strongly correlated plasma whereas cross-field conduction is reduced. Here we show that in such plasmas, the magnetic field has the additional effect of inhibiting the isotropization process between field-parallel and cross-field temperature components, thus leading to the emergence of strong and long-lived temperature anisotropies when the plasma is locally perturbed. An extended heat equation is shown to describe this process accurately.
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In a two-dimensional (2D) dusty plasma composed of superparamagnetic, charged dust grains and immersed in an external magnetic field B, the grains interact via both Yukawa and magnetic dipole-dipole potentials. Because the grains' magnetic dipole moments are induced by B, the dipole moments all lie along B. When B is tilted with respect to the normal to the dust layer, the interaction between the grains becomes anisotropic. In our previous paper [Hartmann et al., Phys. Rev. E 89, 043102 (2014)PLEEE81539-375510.1103/PhysRevE.89.043102], we studied the character of waves in such a system, confined strictly to two dimensions, without any spatial extension in the direction perpendicular to the layer. We analyzed how the dispersion of waves depends on the direction of propagation and the relative strengths of the magnetic dipole and Yukawa potentials. In this paper, we consider a more realistic quasi-2D system where the grains are confined by an external potential and can undergo small oscillations perpendicular to the layer. We analyze the effect of the strength of the confining potential on the in-plane correlations and on the wave propagation. In addition to the in-plane compressional and transverse waves, there now appears an out-of-plane transverse wave generated by the oscillation of the grains in the confining potential. The theoretical approach uses the quasi-localized charge approximation paralleled by molecular dynamics simulations.
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A "scanning" drift tube apparatus, capable of mapping of the spatiotemporal evolution of electron swarms, developing between two plane electrodes under the effect of a homogeneous electric field, is presented. The electron swarms are initiated by photoelectron pulses and the temporal distributions of the electron flux are recorded while the electrode gap length (at a fixed electric field strength) is varied. Operation of the system is tested and verified with argon gas; the measured data are used for the evaluation of the electron bulk drift velocity. The experimental results for the space-time maps of the electron swarms - presented here for the first time - also allow clear observation of deviations from hydrodynamic transport. The swarm maps are also reproduced by particle simulations.
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The influence of an external homogeneous magnetic field on the quasilocalization of the particles-characterized quantitatively by cage correlation functions-in strongly coupled three-dimensional Yukawa systems is investigated via molecular dynamics computer simulations over a wide domain of the system parameters (coupling and screening strengths, and magnetic field). The caging time is found to be enhanced by the magnetic field B. The anisotropic migration of the particles in the presence of magnetic field is quantified via computing directional correlation functions, which indicate a more significant increase of localization in the direction perpendicular to B, while a moderate increase is also found along the B field lines. Associating the particles' escapes from the cages with jumps of a characteristic length, a connection is found with the diffusion process: the diffusion coefficients derived from the decay time of the directional correlation functions in both the directions perpendicular to and parallel with B are in very good agreement with respective diffusion coefficients values obtained from their usual computation based on the mean-squared displacement of the particles.
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Properties of two-dimensional strongly coupled Yukawa systems are explored through molecular dynamics simulations. An effective coupling coefficient gamma* for the liquid phase is introduced on the basis of the constancy of the first peak amplitude of the pair-correlation functions. Thermodynamic quantities are calculated from the pair-correlation function. The solid-liquid transition of the system is investigated through the analysis of the bond-angular order parameter. The static structure function satisfies consistency relation, attesting to the reliability of the computational method. The response is shown to be governed by the correlational part of the inverse compressibility. An analysis of the velocity autocorrelation demonstrates that this latter also exhibits a universal behavior.
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In a classical ideal plasma, a magnetic field is known to reduce the heat conductivity perpendicular to the field, whereas it does not alter the one along the field. Here we show that, in strongly correlated plasmas that are observed at high pressure and/or low temperature, a magnetic field reduces the perpendicular heat transport much less and even enhances the parallel transport. These surprising observations are explained by the competition of kinetic, potential, and collisional contributions to the heat conductivity. Our results are based on first-principle molecular dynamics simulations of a one-component plasma.
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The accuracy of secondary-electron emission coefficients, that are used as input data of discharge models, seriously influences the calculated discharge characteristics. As it is very difficult to consider all possible electron emission processes of a cold cathode separately, in most of the recent models an apparent secondary coefficient gamma is applied, which is often assumed to be constant, even for a wide range of discharge conditions. In contrast with this common assumption, the present calculations-based on a heavy-particle hybrid model-show that in abnormal glow discharges gamma varies considerably with changing discharge conditions: a factor of 3 change of gamma has been found in the range of reduced current densities (0.04 mA cm(-2) Torr(-2)< or =j/p(2)< or =4 mA cm(-2) Torr(-2)) covered in this study. The present simulations also confirm that ionization by heavy particles plays a significant role in the ion production at the abnormal cathode fall. Moreover, it is shown, that the fast heavy particles reflected from the cathode surface play the dominant role in the gas heating.
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The thermal conductivity of strongly coupled Yukawa liquids, being relevant to dusty plasmas, is calculated from nonequilibrium molecular dynamics simulations. The calculations cover a wide range of plasma coupling (Gamma) and screening (kappa) parameters and yield data which are generally in good agreement with the results of recent independent calculations. An improved analytical formula, relating the thermal conductivity to the reduced temperature and to the screening length, is proposed.
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The structure of strongly coupled charged particle bilayers was investigated using molecular dynamics simulation, in a wide range of the plasma coupling parameter Gamma=20-100. The simulations showed the existence of a series of structural transformations, controlled by the separation of the layers. At high values of Gamma a pronounced long-range order was found to develop at intermediate layer separations, with staggered square lattice configuration. The results show a fair agreement with those obtained by hypernetted chain calculations, in terms of intralayer and interlayer pair correlation functions and structure functions.