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When the Coulomb repulsion between electrons dominates over their kinetic energy, electrons in two-dimensional systems are predicted to spontaneously break continuous-translation symmetry and form a quantum crystal1. Efforts to observe2-12 this elusive state of matter, termed a Wigner crystal, in two-dimensional extended systems have primarily focused on conductivity measurements on electrons confined to a single Landau level at high magnetic fields. Here we use optical spectroscopy to demonstrate that electrons in a monolayer semiconductor with density lower than 3 × 1011 per centimetre squared form a Wigner crystal. The combination of a high electron effective mass and reduced dielectric screening enables us to observe electronic charge order even in the absence of a moiré potential or an external magnetic field. The interactions between a resonantly injected exciton and electrons arranged in a periodic lattice modify the exciton bandstructure so that an umklapp resonance arises in the optical reflection spectrum, heralding the presence of charge order13. Our findings demonstrate that charge-tunable transition metal dichalcogenide monolayers14 enable the investigation of previously uncharted territory for many-body physics where interaction energy dominates over kinetic energy.
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One of the first theoretically predicted manifestations of strong interactions in many-electron systems was the Wigner crystal1-3, in which electrons crystallize into a regular lattice. The crystal can melt via either thermal or quantum fluctuations4. Quantum melting of the Wigner crystal is predicted to produce exotic intermediate phases5,6 and quantum magnetism7,8 because of the intricate interplay of Coulomb interactions and kinetic energy. However, studying two-dimensional Wigner crystals in the quantum regime has often required a strong magnetic field9-11 or a moiré superlattice potential12-15, thus limiting access to the full phase diagram of the interacting electron liquid. Here we report the observation of bilayer Wigner crystals without magnetic fields or moiré potentials in an atomically thin transition metal dichalcogenide heterostructure, which consists of two MoSe2 monolayers separated by hexagonal boron nitride. We observe optical signatures of robust correlated insulating states at symmetric (1:1) and asymmetric (3:1, 4:1 and 7:1) electron doping of the two MoSe2 layers at cryogenic temperatures. We attribute these features to bilayer Wigner crystals composed of two interlocked commensurate triangular electron lattices, stabilized by inter-layer interaction16. The Wigner crystal phases are remarkably stable, and undergo quantum and thermal melting transitions at electron densities of up to 6 × 1012 per square centimetre and at temperatures of up to about 40 kelvin. Our results demonstrate that an atomically thin heterostructure is a highly tunable platform for realizing many-body electronic states and probing their liquid-solid and magnetic quantum phase transitions4-8,17.
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Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is 1/τtrâ=â2πλT, where λ is a dimensionless strength of the electron-phonon coupling. The fact that measured values satisfy λââ²â1 has been noted in the context of a possible "Planckian" bound on transport. However, since the electron-phonon scattering is quasielastic in this regime, no such Planckian considerations can be relevant. We present and analyze Monte Carlo results on the Holstein model which show that a different sort of bound is at play: a "stability" bound on λ consistent with metallic transport. We conjecture that a qualitatively similar bound on the strength of residual interactions, which is often stronger than Planckian, may apply to metals more generally.
Assuntos
Elétrons , Metais , Movimento Celular , Método de Monte Carlo , FônonsRESUMO
We propose local electromagnetic noise spectroscopy as a versatile and noninvasive tool to study Wigner crystal phases of strongly interacting two-dimensional electronic systems. In-plane imaging of the local noise is predicted to enable single-site resolution of the electron crystal when the sample-probe distance is less than the interelectron separation. At larger sample-probe distances, noise spectroscopy encodes information about the low-energy Wigner crystal phonons, including the dispersion of the transverse shear mode, the pinning resonance due to disorder, and optical modes emerging, for instance, in bilayer crystals. We discuss the potential utility of local noise probes in analyzing the rich set of phenomena expected to occur in the vicinity of the melting transition.
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Scattering experiments have revolutionized our understanding of nature. Examples include the discovery of the nucleus [R. G. Newton, Scattering Theory of Waves and Particles (1982)], crystallography [U. Pietsch, V. Holý, T. Baumback, High-Resolution X-Ray Scattering (2004)], and the discovery of the double-helix structure of DNA [J. D. Watson, F. H. C. Crick, Nature 171, 737-738]. Scattering techniques differ by the type of particles used, the interaction these particles have with target materials, and the range of wavelengths used. Here, we demonstrate a two-dimensional table-top scattering platform for exploring magnetic properties of materials on mesoscopic length scales. Long-lived, coherent magnonic excitations are generated in a thin film of yttrium iron garnet and scattered off a magnetic target deposited on its surface. The scattered waves are then recorded using a scanning nitrogen vacancy center magnetometer that allows subwavelength imaging and operation under conditions ranging from cryogenic to ambient environment. While most scattering platforms measure only the intensity of the scattered waves, our imaging method allows for spatial determination of both amplitude and phase of the scattered waves, thereby allowing for a systematic reconstruction of the target scattering potential. Our experimental results are consistent with theoretical predictions for such a geometry and reveal several unusual features of the magnetic response of the target, including suppression near the target edges and a gradient in the direction perpendicular to the direction of surface wave propagation. Our results establish magnon scattering experiments as a platform for studying correlated many-body systems.
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Twisted bilayer graphene (TBG) exhibits extremely low Fermi velocities for electrons, with the speed of sound surpassing the Fermi velocity. This regime enables the use of TBG for amplifying vibrational waves of the lattice through stimulated emission, following the same principles of operation of free-electron lasers. Our Letter proposes a lasing mechanism relying on the slow-electron bands to produce a coherent beam of acoustic phonons. We propose a device based on undulated electrons in TBG, which we dub the phaser. The device generates phonon beams in a terahertz (THz) frequency range, which can then be used to produce THz electromagnetic radiation. The ability to generate coherent phonons in solids breaks new ground in controlling quantum memories, probing quantum states, realizing nonequilibrium phases of matter, and designing new types of THz optical devices.
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The extremely overdoped cuprates are generally considered to be Fermi liquid metals without exotic orders, whereas the underdoped cuprates harbor intertwined states. Contrary to this conventional wisdom, using Cu L_{3}-edge and O K-edge resonant x-ray scattering, we reveal a charge order (CO) correlation in overdoped La_{2-x}Sr_{x}CuO_{4} (0.35≤x≤0.6) beyond the superconducting dome. This CO has a periodicity of â¼6 lattice units with correlation lengths of â¼20 lattice units. It shows similar in-plane momentum and polarization dependence and dispersive excitations as the CO of underdoped cuprates, but its maximum intensity differs along the c direction and persists up to 300 K. This CO correlation cannot be explained by the Fermi surface instability and its origin remains to be understood. Our results suggest that CO is prevailing in the overdoped metallic regime and requires a reassessment of the picture of overdoped cuprates as weakly correlated Fermi liquids.
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Strongly correlated metals often display anomalous transport, including T-linear resistivity above the Mott-Ioffe-Regel limit. We introduce a tractable microscopic model for bad metals, by restoring in the well-known Hubbard model-with hopping t and on-site repulsion U-a "screened Coulomb" interaction between charge densities that decays exponentially with spatial separation. This interaction lifts the extensive degeneracy in the spectrum of the t=0 Hubbard model, allowing us to fully characterize the small t electric, thermal, and thermoelectric transport in our strongly correlated model. Throughout the phase diagram we observe T-linear resistivity above the Mott-Ioffe-Regel limit, together with strong violation of the Wiedemann-Franz law and a large thermopower that can undergo sign change.
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Strange metals-ubiquitous in correlated quantum materials-transport electrical charge at low temperatures but not by the individual electronic quasiparticle excitations, which carry charge in ordinary metals. In this work, we consider two-dimensional metals of fermions coupled to quantum critical scalars, the latter representing order parameters or fractionalized particles. We show that at low temperatures (T), such metals generically exhibit strange metal behavior with a T-linear resistivity arising from spatially random fluctuations in the fermion-scalar Yukawa couplings about a nonzero spatial average. We also find a T ln(1/T) specific heat and a rationale for the Planckian bound on the transport scattering time. These results are in agreement with observations and are obtained in the large N expansion of an ensemble of critical metals with N fermion flavors.