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1.
Nano Lett ; 21(16): 7037-7043, 2021 Aug 25.
Artigo em Inglês | MEDLINE | ID: mdl-34374550

RESUMO

Unequal transmissions of spin waves along opposite directions provide useful functions for signal processing. So far, the realization of such nonreciprocal spin waves has been mostly limited at a gigahertz frequency in the coherent regime via microwave excitation. Here we show that, in a magnetic bilayer stack with chiral coupling, tunable nonreciprocal propagation can be realized in spin Hall effect-excited incoherent magnons, whose frequencies cover the spectrum from a few gigahertz up to terahertz. The sign of nonreciprocity is controlled by the magnetic orientations of the bilayer in a nonvolatile manner. The nonreciprocity is further verified by measurements of the magnon diffusion length, which is unequal along opposite transmission directions. Our findings enrich the knowledge on magnetic relaxation and diffusive transport and can lead to the design of a passive directional signal isolation device in the diffusive regime.

2.
Phys Rev Lett ; 123(24): 247206, 2019 Dec 13.
Artigo em Inglês | MEDLINE | ID: mdl-31922833

RESUMO

A quantitative investigation of the current-induced torque in antiferromagnets represents a great challenge due to the lack of an independent method for controlling Néel vectors. By utilizing an antiferromagnetic insulator with the Dzyaloshinskii-Moriya interaction α-Fe_{2}O_{3}, we show that the Néel vector can be controlled with a moderate external field, which is further utilized to calibrate the current-induced magnetic dynamics. We find that the current-induced magnetoresistance change in antiferromagnets can be complicated by resistive switching that does not have a magnetic origin. By excluding nonmagnetic switching and comparing the current-induced dynamics with the field-induced one, we determine the nature and magnitude of current-induced effects in Pt/α-Fe_{2}O_{3} bilayer films.

3.
Phys Rev Lett ; 121(5): 057701, 2018 Aug 03.
Artigo em Inglês | MEDLINE | ID: mdl-30118301

RESUMO

Owing to the difficulty in detecting and manipulating the magnetic states of antiferromagnetic materials, studying their switching dynamics using electrical methods remains a challenging task. By employing heavy-metal-rare-earth-transition-metal alloy bilayers, we experimentally study current-induced domain wall dynamics in an antiferromagnetically coupled system. We show that the current-induced domain wall mobility reaches a maximum at the angular momentum compensation point. With experiment and modeling, we further reveal the internal structures of domain walls and the underlying mechanisms for their fast motion. We show that the chirality of the ferrimagnetic domain walls remains the same across the compensation points, suggesting that spin orientations of specific sublattices rather than net magnetization determine Dzyaloshinskii-Moriya interaction in heavy-metal-ferrimagnet bilayers. The high current-induced domain wall mobility and the robust domain wall chirality in compensated ferrimagnetic material opens new opportunities for high-speed spintronic devices.

4.
Phys Rev Lett ; 119(7): 077702, 2017 Aug 18.
Artigo em Inglês | MEDLINE | ID: mdl-28949690

RESUMO

The strongly spin-momentum coupled electronic states in topological insulators (TI) have been extensively pursued to realize efficient magnetic switching. However, previous studies show a large discrepancy of the charge-spin conversion efficiency. Moreover, current-induced magnetic switching with TI can only be observed at cryogenic temperatures. We report spin-orbit torque switching in a TI-ferrimagnet heterostructure with perpendicular magnetic anisotropy at room temperature. The obtained effective spin Hall angle of TI is substantially larger than the previously studied heavy metals. Our results demonstrate robust charge-spin conversion in TI and provide a direct avenue towards applicable TI-based spintronic devices.

5.
Nat Nanotechnol ; 18(9): 1000-1004, 2023 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-37264089

RESUMO

Advancing the development of spin-wave devices requires high-quality low-damping magnetic materials where magnon spin currents can efficiently propagate and effectively interact with local magnetic textures. Here we show that magnetic domain walls can modulate spin-wave transport in perpendicularly magnetized channels of Bi-doped yttrium iron garnet. Conversely, we demonstrate that the magnon spin current can drive domain-wall motion in the Bi-doped yttrium iron garnet channel device by means of magnon spin-transfer torque. The domain wall can be reliably moved over 15-20 µm distances at zero applied magnetic field by a magnon spin current excited by a radio-frequency pulse as short as 1 ns. The required energy for driving the domain-wall motion is orders of magnitude smaller than those reported for metallic systems. These results facilitate low-switching-energy magnonic devices and circuits where magnetic domains can be efficiently reconfigured by magnon spin currents flowing within magnetic channels.

6.
Adv Mater ; 34(4): e2103870, 2022 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-34793612

RESUMO

Volumetric optical imaging of magnetic fields is challenging with existing magneto-optical materials, motivating the search for dyes with strong magnetic field interactions, distinct emission spectra, and an ability to withstand high photon flux and incorporation within samples. Here, the magnetic field effect on singlet-exciton fission is exploited to demonstrate spatial imaging of magnetic fields in a thin film of rubrene. Doping rubrene with the high-quantum yield dye dibenzotetraphenylperiflanthene (DBP) is shown to enable optically pumped, slab waveguide lasing. This laser is magnetic-field-switchable: when operated just below the lasing threshold, application of a 0.4 T magnetic field switches the device between nonlasing and lasing modes, accompanied by an intensity modulation of +360%. This is thought to be the first demonstration of a magnetically switchable laser, as well as the largest magnetically induced change in emission brightness in a singlet-fission material to date. These results demonstrate that singlet-fission materials are promising materials for magnetic sensing applications and could inspire a new class of magneto-optical modulators.

7.
Adv Mater ; 33(22): e2008555, 2021 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-33899284

RESUMO

While being electrically insulating, magnetic insulators can behave as good spin conductors by carrying spin current with excited spin waves. So far, magnetic insulators are utilized in multilayer heterostructures for optimizing spin transport or to form magnon spin valves for reaching controls over the spin flow. In these studies, it remains an intensively visited topic as to what the corresponding roles of coherent and incoherent magnons are in the spin transmission. Meanwhile, understanding the underlying mechanism associated with spin transmission in insulators can help to identify new mechanisms that can further improve the spin transport efficiency. Here, by studying spin transport in a magnetic-metal/magnetic-insulator/platinum multilayer, it is demonstrated that coherent magnons can transfer spins efficiently above the magnon bandgap of magnetic insulators. Particularly the standing spin-wave mode can greatly enhance the spin flow by inducing a resonant magnon transmission. Furthermore, within the magnon bandgap, a shutdown of spin transmission due to the blocking of coherent magnons is observed. The demonstrated magnon transmission enhancement and filtering effect provides an efficient method for modulating spin current in magnonic devices.

8.
Nat Nanotechnol ; 15(7): 563-568, 2020 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-32483320

RESUMO

Antiferromagnets (AFMs) possess great potential in spintronics because of their immunity to external magnetic disturbance, the absence of a stray field or the resonance in the terahertz range1,2. The coupling of insulating AFMs to spin-orbit materials3-7 enables spin transport via AFM magnons. In particular, spin transmission over several micrometres occurs in some AFMs with easy-axis anisotropy8,9. Easy-plane AFMs with two orthogonal, linearly polarized magnon eigenmodes own unique advantages for low-energy control of ultrafast magnetic dynamics2. However, it is commonly conceived that these magnon modes are less likely to transmit spins because of their vanishing angular momentum9-11. Here we report experimental evidence that an easy-plane insulating AFM, an α-Fe2O3 thin film, can efficiently transmit spins over micrometre distances. The spin decay length shows an unconventional temperature dependence that cannot be captured considering solely thermal magnon scatterings. We interpret our observations in terms of an interference of two linearly polarized, propagating magnons in analogy to the birefringence effect in optics. Furthermore, our devices can realize a bi-stable spin-current switch with a 100% on/off ratio under zero remnant magnetic field. These findings provide additional tools for non-volatile, low-field control of spin transport in AFM systems.

9.
Adv Mater ; 31(2): e1805361, 2019 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-30412315

RESUMO

Ferrimagnetic materials combine the advantages of the low magnetic moment of an antiferromagnet and the ease of realizing magnetic reading of a ferromagnet. Recently, it was demonstrated that compensated ferrimagnetic half metals can be realized in Heusler alloys, where high spin polarization, zero magnetic moment, and low magnetic damping can be achieved at the same time. In this work, by studying the spin-orbit torque induced switching in the Heusler alloy Mn2 Ru1- x Ga, it is found that efficient current-induced magnetic switching can be realized in a nearly compensated sample with strong perpendicular anisotropy and large film thickness. This work demonstrates the possibility of employing compensated Heusler alloys for fast, energy-efficient spintronic devices.

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